Recent advances in light energy conversion with biomimetic vesicle membranes.

Abstract

Lipid bilayer membranes are ubiquitous in natural chemical conversions. They enable for self-assembly and compartmentalization of reaction partners and it becomes increasingly evident that a thorough fundamental understanding of these concepts is highly desirable for chemical reactions and solar energy conversion with artificial systems. This minireview focusses on selected case studies from recent years, most of which were inspired by either membrane-facilitated light harvesting or respective charge transfer. The main focus is on highly biomimetic liposomes with artificial chromophores, and some cases for polymer-membranes will be made. Furthermore, we categorized these studies into energy transfer and electron transfer, with phospholipid vesicles, and polymer membranes for light-driven reactions.