In situ X-ray tomography densification of firn: The role of mechanics and diffusion processes

Abstract

Abstract One of the most efficient proxy methods for paleoclimatology consists of obtaining data previously preserved within polar ice cores. Models for past climate reconstruction are based in particular on the characterization of entrapped gases in ice closed pores. Improving the temporal accuracy of these models requires a better understanding of firn densification mechanisms. In particular, the interplay between viscoplastic deformation and diffusion processes for pore closure is not well understood. In this work, we describe the first in situ laboratory densification experiments on polar firn retrieved from Antarctica with live characterization by X-ray tomography. Our in situ tests allow for the first time to approximately access the process of pore closure in ice, which takes thousands of years to occur in Antarctica, from visualizations and quantitative analyses of short time laboratory experiments. The parameters of pore separation and closure and the microstructural changes that accompany them are monitored. We show that densification of polar firn and pore closure could be replicated at higher strain rate and warmer temperature. Experiments allow the viscoplastic part of the firn deformation to be decoupled from the diffusion mechanisms that occur at high temperature. Our results show that density alone is not sufficient to predict the close-off density at which gases get entrapped. More generally, the method laid out here may find useful application in the domain of high temperature powder compaction, for which pore closure and grain growth are significant process parameters.