Featured Researches

Mesoscale And Nanoscale Physics

Highly tunable quadruple quantum dot in a narrow bandgap semiconductor InAs nanowire

Quantum dots (QDs) made from semiconductors are among the most promising platforms for the developments of quantum computing and simulation chips, and have advantages over other platforms in high density integration and in compatibility to the standard semiconductor chip fabrication technology. However, development of a highly tunable semiconductor multiple QD system still remains as a major challenge. Here, we demonstrate realization of a highly tunable linear quadruple QD (QQD) in a narrow bandgap semiconductor InAs nanowire with fine finger gate technique. The QQD is studied by electron transport measurements in the linear response regime. Characteristic two-dimensional charge stability diagrams containing four groups of resonant current lines of different slopes are found for the QQD. It is shown that these current lines can be individually assigned as arising from resonant electron transport through the energy levels of different QDs. Benefited from the excellent gate tunability, we also demonstrate tuning of the QQD to regimes where the energy levels of two QDs, three QDs and all the four QDs are energetically on resonance, respectively, with the fermi level of source and drain contacts. A capacitance network model is developed for the linear QQD and the simulated charge stability diagrams based on the model show good agreements with the experiments. Our work presents a solid experimental evidence that narrow bandgap semiconductor nanowires multiple QDs could be used as a versatile platform to achieve integrated qubits for quantum computing and to perform quantum simulations for complex many-body systems.

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Mesoscale And Nanoscale Physics

Hinge Spin Polarization in Magnetic Topological Insulators Revealed by Resistance Switch

We report on the possibility to detect hinge spin polarization in magnetic topological insulators by resistance measurements. By implementing a three-dimensional model of magnetic topological insulators into a multi-terminal device with ferromagnetic contacts near the top surface, local spin features of the chiral edge modes are unveiled. We find local spin polarization at the hinges that inverts sign between top and bottom surfaces. At the opposite edge, the topological state with inverted spin polarization propagates in the reverse direction. Large resistance switch between forward and backward propagating states is obtained, driven by the matching between the spin polarized hinges and the ferromagnetic contacts. This feature is general to the ferromagnetic, antiferromagnetic and canted-antiferromagnetic phases, and enables the design of spin-sensitive devices, with the possibility of reversing the hinge spin polarization of the currents.

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Mesoscale And Nanoscale Physics

Hydrodynamical study of Terahertz emission in magnetized graphene field-effect transistors

Several hydrodynamic descriptions of charge transport in graphene have been presented in the late years. We discuss a general hydrodynamic model governing the dynamics of a two-dimensional electron gas in a magnetized field-effect transistor in the slow drift regime. The Dyakonov--Shur instability is investigated including the effect of weak magnetic fields (i.e. away from Landau levels). We show that the gap on the dispersion relation prevents the instability to reach the lower frequencies thus imposing a limit on the Mach number of the electronic flow. Furthermore, we discuss that the presence of the external magnetic field decreases the growth rate of the instability, as well as the saturation amplitude. The numerical results from our simulations and the presented higher order dynamic mode decomposition support such reasoning.

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Mesoscale And Nanoscale Physics

Hyperpolarisation of external nuclear spins using nitrogen-vacancy centre ensembles

The nitrogen-vacancy (NV) centre in diamond has emerged as a candidate to non-invasively hyperpolarise nuclear spins in molecular systems to improve the sensitivity of nuclear magnetic resonance (NMR) experiments. Several promising proof of principle experiments have demonstrated small-scale polarisation transfer from single NVs to hydrogen spins outside the diamond. However, the scaling up of these results to the use of a dense NV ensemble, which is a necessary prerequisite for achieving realistic NMR sensitivity enhancement, has not yet been demonstrated. In this work, we present evidence for a polarising interaction between a shallow NV ensemble and external nuclear targets over a micrometre scale, and characterise the challenges in achieving useful polarisation enhancement. In the most favourable example of the interaction with hydrogen in a solid state target, a maximum polarisation transfer rate of ??500 spins per second per NV is measured, averaged over an area containing order 10 6 NVs. Reduced levels of polarisation efficiency are found for liquid state targets, where molecular diffusion limits the transfer. Through analysis via a theoretical model, we find that our results suggest implementation of this technique for NMR sensitivity enhancement is feasible following realistic diamond material improvements.

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Mesoscale And Nanoscale Physics

Imaging local discharge cascades for correlated electrons in WS2/WSe2 moiré superlattices

Transition metal dichalcogenide (TMD) moiré heterostructures provide an ideal platform to explore the extended Hubbard model1 where long-range Coulomb interactions play a critical role in determining strongly correlated electron states. This has led to experimental observations of Mott insulator states at half filling2-4 as well as a variety of extended Wigner crystal states at different fractional fillings5-9. Microscopic understanding of these emerging quantum phases, however, is still lacking. Here we describe a novel scanning tunneling microscopy (STM) technique for local sensing and manipulation of correlated electrons in a gated WS2/WSe2 moiré superlattice that enables experimental extraction of fundamental extended Hubbard model parameters. We demonstrate that the charge state of local moiré sites can be imaged by their influence on STM tunneling current, analogous to the charge-sensing mechanism in a single-electron transistor. In addition to imaging, we are also able to manipulate the charge state of correlated electrons. Discharge cascades of correlated electrons in the moiré superlattice are locally induced by ramping the STM bias, thus enabling the nearest-neighbor Coulomb interaction (UNN) to be estimated. 2D mapping of the moiré electron charge states also enables us to determine onsite energy fluctuations at different moiré sites. Our technique should be broadly applicable to many semiconductor moiré systems, offering a powerful new tool for microscopic characterization and control of strongly correlated states in moiré superlattices.

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Mesoscale And Nanoscale Physics

Imaging phonon-mediated hydrodynamic flow in WTe2 with cryogenic quantum magnetometry

In the presence of strong interactions, electrons in condensed matter systems can behave hydrodynamically thereby exhibiting classical fluid phenomena such as vortices and Poiseuille flow. While in most conductors large screening effects minimize electron-electron interactions, hindering the search for possible hydrodynamic candidate materials, a new class of semimetals has recently been reported to exhibit strong interactions. In this work, we study the current flow in the layered semimetal tungsten ditelluride (WTe2) by imaging the local magnetic field above it using a nitrogen-vacancy (NV) defect in diamond. Our cryogenic scanning magnetometry system allows for temperature-resolved measurement with high sensitivity enabled by the long defect spin coherence. We directly measure the spatial current profile within WTe2 and find it differs substantially from the uniform profile of a Fermi liquid, indicating hydrodynamic flow. Furthermore, our temperature-resolved current profile measurements reveal an unexpected non-monotonic temperature dependence, with hydrodynamic effects strongest at ~20 K. We further elucidate this behavior via ab initio calculations of electron scattering mechanisms, which are used to extract a current profile using the electronic Boltzmann transport equation. These calculations show quantitative agreement with our measurements, capturing the non-monotonic temperature dependence. The combination of experimental and theoretical observations allows us to quantitatively infer the strength of electron-electron interactions in WTe2. We show these strong electron interactions cannot be explained by Coulomb repulsion alone and are predominantly phonon-mediated. This provides a promising avenue in the search for hydrodynamic flow and strong interactions in high carrier density materials.

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Mesoscale And Nanoscale Physics

Imaging vibrations of locally gated, electromechanical few layer graphene resonators with a moving vacuum enclosure

Imaging the vibrations of nanomechanical resonators means measuring their flexural mode shapes from the dependence of their frequency response on in-plane position. Applied to two-dimensional resonators, this technique provides a wealth of information on the mechanical properties of atomically-thin membranes. We present a simple and robust system to image the vibrations of few layer graphene (FLG) resonators at room temperature and in vacuum with an in-plane displacement precision of ??.20 μ m. It consists of a sturdy vacuum enclosure mounted on a three-axis micropositioning stage and designed for free space optical measurements of vibrations. The system is equipped with ultra-flexible radio frequency waveguides to electrically actuate resonators. With it we characterize the lowest frequency mode of a FLG resonator by measuring its frequency response as a function of position on the membrane. The resonator is suspended over a nanofabricated local gate electrode acting both as a mirror and as a capacitor plate to actuate vibrations at radio frequencies. From these measurements, we estimate the ratio of thermal expansion coefficient to thermal conductivity of the membrane, and we measure the effective mass of the lowest frequency mode. We complement our study with a globally gated resonator and image its first three vibration modes. There, we find that folds in the membrane locally suppress vibrations.

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Mesoscale And Nanoscale Physics

Impossibility of Increasing N e ´ el Temperature in Zigzag Graphene Nanoribbon by Electric Field and Carrier Doping

We investigated the dependence of N e ´ el temperature as a critical temperature on the electric field and hole-electron doping in the antiferromagnetically ordered zigzag graphene nanoribbon. The temperature was calculated by averaging the magnon energy in the Brillouin zone within the mean-field approximation. We employed the generalized Bloch theorem instead of the supercell approach to reduce the computational cost significantly to obtain the magnon spectrum. We showed that the N e ´ el temperature reduces when increasing both the electric field and the hole-electron doping, thus these treatments will never enhance the N e ´ el temperature.

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Mesoscale And Nanoscale Physics

Imprinting Tunable ? -Magnetism in Graphene Nanoribbons via Edge Extensions

Magnetic carbon nanostructures are currently under scrutiny for a wide spectrum of applications. Here, we theoretically investigate armchair graphene nanoribbons patterned with asymmetric edge extensions consisting of laterally fused naphtho groups, as recently fabricated via on-surface synthesis. We show that an individual edge extension acts as a spin- 1 2 center and develops a sizable spin-polarization of the conductance around the band edges. The Heisenberg exchange coupling between a pair of edge extensions is dictated by the position of the second naphtho group in the carbon backbone, thus enabling ferromagnetic, antiferromagnetic, or non-magnetic states. The periodic arrangement of edge extensions yields full spin-polarization at the band extrema, and the accompanying ferromagnetic ground state can be driven into non-magnetic or antiferromagnetic phases through external stimuli. Overall, our work reveals precise tunability of the ? -magnetism in graphene nanoribbons induced by naphtho groups, thereby establishing these one-dimensional architectures as suitable platforms for logic spintronics.

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Mesoscale And Nanoscale Physics

InP-based single-photon sources operating at telecom C-band with increased extraction efficiency

In this work we demonstrate a triggered single-photon source operating at the telecom C-band with photon extraction efficiency exceeding any reported values in this range. The non-classical light emission with low probability of the multiphoton events is realized with single InAs quantum dots (QDs) grown by molecular beam epitaxy and embedded directly in an InP matrix. Low QD spatial density on the order of 5x108 cm-2 to ~2x109 cm-2 and symmetric shape of these nanostructures together with spectral range of emission makes them relevant for quantum communication applications. The engineering of extraction efficiency is realized by combining a bottom distributed Bragg reflector consisting of 25 pairs of InP/In0.53Ga0.37Al0.1As layers and cylindrical photonic confinement structures. Realization of such technologically non-demanding approach even in a non-deterministic fashion results in photon extraction efficiency of (13.3+/-2)% into 0.4 numerical aperture detection optics at approx. 1560 nm emission wavelength, i.e., close to the center of the telecom C-band.

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