A. Papayannis

Aerosol lidar intercomparison in the framework of the EARLINET project. 3. Raman lidar algorithm for aerosol extinction, backscatter, and lidar ratio

An intercomparison of the algorithms used to retrieve aerosol extinction and backscatter starting from Raman lidar signals has been performed by 11 groups of lidar scientists involved in the European Aerosol Research Lidar Network (EARLINET). This intercomparison is part of an extended quality assurance program performed on aerosol lidars in the EARLINET. Lidar instruments and aerosol backscatter algorithms were tested separately. The Raman lidar algorithms were tested by use of synthetic lidar data, simulated at 355, 532, 386, and 607 nm, with realistic experimental and atmospheric conditions taken into account. The intercomparison demonstrates that the data-handling procedures used by all the lidar groups provide satisfactory results. Extinction profiles show mean deviations from the correct solution within 10% in the planetary boundary layer (PBL), and backscatter profiles, retrieved by use of algorithms based on the combined Raman elastic-backscatter lidar technique, show mean deviations from solutions within 20% up to 2 km. The intercomparison was also carried out for the lidar ratio and produced profiles that show a mean deviation from the solution within 20% in the PBL. The mean value of this parameter was also calculated within a lofted aerosol layer at higher altitudes that is representative of typical layers related to special events such as Saharan dust outbreaks, forest fires, and volcanic eruptions. Here deviations were within 15%.

Aerosol lidar intercomparison in the framework of the EARLINET project. 2.Aerosol backscatter algorithms

An intercomparison of aerosol backscatter lidar algorithms was performed in 2001 within the framework of the European Aerosol Research Lidar Network to Establish an Aerosol Climatology (EARLINET). The objective of this research was to test the correctness of the algorithms and the influence of the lidar ratio used by the various lidar teams involved in the EARLINET for calculation of backscatter-coefficient profiles from the lidar signals. The exercise consisted of processing synthetic lidar signals of various degrees of difficulty. One of these profiles contained height-dependent lidar ratios to test the vertical influence of those profiles on the various retrieval algorithms. Furthermore, a realistic incomplete overlap of laser beam and receiver field of view was introduced to remind the teams to take great care in the nearest range to the lidar. The intercomparison was performed in three stages with increasing knowledge on the input parameters. First, only the lidar signals were distributed; this is the most realistic stage. Afterward the lidar ratio profiles and the reference values at calibration height were provided. The unknown height-dependent lidar ratio had the largest influence on the retrieval, whereas the unknown reference value was of minor importance. These results show the necessity of making additional independent measurements, which can provide us with a suitable approximation of the lidar ratio. The final stage proves in general, that the data evaluation schemes of the different groups of lidar systems work well.

EARLINET observations of the 14-22-May long-range dust transport event during SAMUM 2006: validation of results from dust transport modelling

We observed a long-range transport event of mineral dust from North Africa to South Europe during the Saharan Mineral Dust Experiment (SAMUM) 2006. Geometrical and optical properties of that dust plume were determined with Sun photometer of the Aerosol Robotic Network (AERONET) and Raman lidar near the North African source region, and with Sun photometers of AERONET and lidars of the European Aerosol Research Lidar Network (EARLINET) in the far field in Europe. Extinction-to-backscatter ratios of the dust plume over Morocco and Southern Europe do not differ. Ångström exponents increase with distance from Morocco. We simulated the transport, and geometrical and optical properties of the dust plume with a dust transport model. The model results and the experimental data show similar times regarding the appearance of the dust plume over each EARLINET site. Dust optical depth from the model agrees in most cases to particle optical depth measured with the Sun photometers. The vertical distribution of the mineral dust could be satisfactorily reproduced, if we use as benchmark the extinction profiles measured with lidar. In some cases we find differences. We assume that insufficient vertical resolution of the dust plume in the model calculations is one reason for these deviations.

Optical, size and mass properties of mixed type aerosols in Greece and Romania as observed by synergy of lidar and sunphotometers in combination with model simulations: A case study

A coordinated experimental campaign aiming to study the aerosol optical, size and mass properties was organized in September 2012, in selected sites in Greece and Romania. It was based on the synergy of lidar and sunphotometers. In this paper we focus on a specific campaign period (23-24 September), where mixed type aerosols (Saharan dust, biomass burning and continental) were confined from the Planetary Boundary Layer (PBL) up to 4-4.5 km height. Hourly mean linear depolarization and lidar ratio values were measured inside the dust layers, ranging from 13 to 29 and from 44 to 65sr, respectively, depending on their mixing status and the corresponding air mass pathways over Greece and Romania. During this event the columnar Aerosol Optical Depth (AOD) values ranged from 0.13 to 0.26 at 532 nm. The Lidar/Radiometer Inversion Code (LIRIC) and the Polarization Lidar Photometer Networking (POLIPHON) codes were used and inter-compared with regards to the retrieved aerosol (fine and coarse spherical/spheroid) mass concentrations, showing that LIRIC generally overestimates the aerosol mass concentrations, in the case of spherical particles. For non-spherical particles the difference in the retrieved mass concentration profiles from these two codes remained smaller than ±20%. POLIPHON retrievals showed that the non-spherical particles reached concentrations of the order of 100-140 μg/m(3) over Romania compared to 50-75 μg/m(3) over Greece. Finally, the Dust Regional Atmospheric Model (DREAM) model was used to simulate the dust concentrations over the South-Eastern Europe.

Ground-, satellite-and simulation-based analysis of a strong dust event over Abastumani, Georgia, during May 2009

A strong dust event over Abastumani, Georgia, during May 2009 was studied using light detection and ranging (lidar), satellite and sun photometric measurements. High aerosol optical depth (AOD) values (0.45–0.57) at 500 nm were measured over the closest Aerosol Robotic Network (AERONET) site (Erdemli, Turkey), whereas over Georgia, the AOD measured by the Moderate Resolution Imaging Spectroradiometer (MODIS) was about 0.9 at 550 nm. The AERONET data analysis showed a mean aerosol effective radius of about 2.5 μm, whereas the mean value of the Ångström exponent (α) (wavelength pair 440/870 nm) was smaller than 1, indicating the dominance of large aerosols. The aerosol lidar over Abastumani showed the existence of a strong particle load from the near ground up to a height of 3.5 km. The BSC-DREAM8b forecast model showed that the dust aerosols travelled from the Saharan and the Arabic deserts to the studied area, even reaching southern Russia, covering a total distance of about 5500 km, in the height region from about 2 to 11.5 km.

EARLINET coordinated lidar observations of Saharan dust events on continental scale

EARLINET, the European Aerosol Research Lidar Network, is the best tool to investigate the horizontal and vertical transport of aerosols over Europe. Within the network, particular attention is devoted to Saharan dust events monitoring. An alert system has been established in order to perform devoted measurements in case of intrusions of desert particles on European continent. Starting from data collected within EARLINET since May 2000, a first statistical analysis of the aerosol vertical distribution on European scale during Saharan dust outbreaks, has been performed. These results highlights the fundamental role that EARLINET can have for the study of impact of Saharan dust on European scale. The current 5-year EU project EARLINET-ASOS, started in March 2006, will enhance the operation of the network through the improvement of the instruments and of the temporal coverage, and of the data analysis procedures.

An overview from hygroscopic aerosols to cloud droplets: The HygrA-CD campaign in the Athens basin

The international experimental campaign Hygroscopic Aerosols to Cloud Droplets (HygrA-CD), organized in the Greater Athens Area (GAA), Greece from 15 May to 22 June 2014, aimed to study the physico-chemical properties of aerosols and their impact on the formation of clouds in the convective Planetary Boundary Layer (PBL). We found that under continental (W-NW-N) and Etesian (NE) synoptic wind flow and with a deep moist PBL (~2-2.5km height), mixed hygroscopic (anthropogenic, biomass burning and marine) particles arrive over the GAA, and contribute to the formation of convective non-precipitating PBL clouds (of ~16-20μm mean diameter) with vertical extent up to 500m. Under these conditions, high updraft velocities (1-2ms-1) and cloud condensation nuclei (CCN) concentrations (~2000cm-3 at 1% supersaturation), generated clouds with an estimated cloud droplet number of ~600cm-3. Under Saharan wind flow conditions (S-SW) a shallow PBL (<1-1.2km height) develops, leading to much higher CCN concentrations (~3500-5000cm-3 at 1% supersaturation) near the ground; updraft velocities, however, were significantly lower, with an estimated maximum cloud droplet number of ~200cm-3 and without observed significant PBL cloud formation. The largest contribution to cloud droplet number variance is attributed to the updraft velocity variability, followed by variances in aerosol number concentration.

Evaluation of CALIPSO’s Aerosol Classification Scheme During the ACEMED Experimental Campaign Over Greece: The Case Study of 9th of September 2011

In order to assess the validity of CALIPSO’s aerosol classification scheme, an experimental campaign called ACEMED (Evaluation of CALIPSO’s aerosol classification scheme over Eastern Mediterranean) has been organized over Greece on September 2011. In this study, we concentrate on the characterization of the aerosol load over Greece on 9th of September, using advanced in-situ aircraft instrumentation (onboard the FAAM-Bae146 aircraft of the UK Met Office). The analytical evaluation of CALIPSO’s aerosol-type classification scheme that is performed using synchronous/collocated satellite/airborne measurements, show a qualitatively reasonable performance of the CALIPSO’s aerosol classification scheme in the complex aerosol environment of the case under study, where smoke, continental, urban and dust aerosol components are present.

From Hygroscopic Aerosols to Cloud Droplets: The HygrA-CD Campaign in the Athens Basin—An Overview

The international experimental campaign Hygroscopic Aerosols to Cloud Droplets (HygrA-CD), organized in the Greater Athens Area (GAA), Greece from 15 May to 22 June 2014 provided an unprecedented record of data on aerosols, clouds and meteorology. HygrA-CD brought together different active/passive remote sensing and in situ instrumentation/teams for the purpose of fostering our understanding on the physico-chemical properties of aerosols and their impact on the cloud formation in the lower troposphere, with emphasis on the top of the Planetary Boundary Layer (PBL). The use of well-established numerical weather prediction and atmospheric modeling, such as the Flexible particle (FLEXPART) dispersion model and the Weather Research and Forecasting (WRF) model enabled us to simulate air mass back-trajectories and atmospheric variables in the PBL, such as PBL height (PBLH), relative humidity, wind fields etc. This paper presents the major findings and highlights of the HygrA-CD campaign.

Forest Fire Aerosols: Vertically Resolved Optical and Microphysical Properties and Mass Concentration from Lidar Observations

The influence of smoke on the aerosol loading in the free troposphere from EARLINET observations are examined in this paper. Several cases during 2001–2011 were identified over Thessaloniki and Athens, Greece, when very high aerosol optical depth values in the free troposphere were observed with a UV-Raman lidar. Particle dispersion modeling (FLEXPART) and satellite hot spot fire detection (ATSR) showed that these high free tropospheric aerosol optical depths are mainly attributed to the advection of smoke plumes from biomass burning regions. The biomass burning regions were found to extend across Russia in the latitudinal belt between 45°N and 55°N, as well as in Eastern Europe. The highest frequency of agricultural fires occurred during the summer season (mainly in August). Emphasis is also given on the 2007 wild fires surrounding Athens and earlier studies performed in the frame of EARLINET. The data collected allowed the optical and microphysical characterization of the smoke aerosols that arrived over Greece, where limited information has so far been available and in synergy with AERΟNET and CALIPSO observation a first attempt is made for the vertically resolved mass concentration of the smoke plumes.