A. Srinivasa Rao

Third order optical nonlinear studies and its use to estimate thickness of sandwiched films of tetra-phenyl porphyrin derivatives

Third-order nonlinear optical properties of tetra-phenyl porphyrin (H2TPP) derivatives viz., H2TPP(OH)4 and Zn(II)TPP doped in boric acid glass thin films were measured using single beam Z-scan and forward degenerate four-wave mixing (DFWM) techniques. Excited state lifetimes and absorption cross-sections were estimated from these experiments. Thickness of the porphyrin doped sandwich glass films were determined using DFWM technique for the first time. The values of nonlinear refractive index (n2) obtained for these systems are are found to be sensitive to the nature of substituents in porphyrin molecule. These results are interpreted in terms of delocalized π electrons contributing to the third-order optical nonlinearity.

Nonlinear frequency doubling characteristics of asymmetric vortices of tunable, broad orbital angular momentum spectrum

We report on a simple experimental scheme to generate and control the orbital angular momentum (OAM) spectrum of the asymmetric vortex beams in a nonlinear frequency conversion process. Using a spiral phase plate (SPP) and adjusting the transverse shift of the SPP with respect to the incident Gaussian beam axis, we have transformed the symmetric (intensity distribution) optical vortex of order l into an asymmetric vortex beam of measured broad spectrum of OAM modes of orders l, l − 1, l − 2, …, 0 (Gaussian mode). While the position of the SPP determines the distribution of the OAM modes, we have also observed that the modal distribution of the vortex beam changes with the shift of the SPP of all orders and finally results in a Gaussian beam (l = 0). Using single-pass frequency doubling of the asymmetric vortices, we have transferred the pump OAM spectra, l, l − 1, l − 2, …, 0, into the broad spectra of higher order OAM modes, 2l, 2l − 1, 2l − 2, …, 0 at green wavelength, owing to OAM conservation in nonli...

On-axis intensity modulation-free, segmented, zero-order Bessel beams with tunable ranges

We propose and experimentally demonstrate a novel experimental scheme to generate high on-axis peak intensity, segmented, smooth, zero-order quasi-Bessel beams with tunable ranges. Illuminating the axicon with hollow Gaussian beams (HGBs) of different orders, we have generated Bessel beams of varying ranges at different positions away from the axicon. The presence of a dark core at the center of the HGBs removes the effect of imperfection in the axicon tip. As a result, the entire power of the input beam is transformed into a zero-order Bessel beam without any on-axis intensity modulation. We observe the decrease in range and increase in on-axis peak intensity of the zero-order Bessel beam with the order of HGBs. Controlling the superposition of the HGBs of different orders to the axicon, we have demonstrated the increase in the range of the Bessel beam. The current technique can also produce Bessel beams of different intensity distributions, including single-peak or multiple-peak Bessel beams. Using single-pass second-harmonic generation in nonlinear crystals of different lengths, we have further verified the increase of on-axis peak intensity of the Bessel beam with the order of the HGBs and the increase in the range of the Bessel beam due to the superposed HGBs.