Alessandro Principi

Highly confined low-loss plasmons in graphene–boron nitride heterostructures

Graphene plasmons were predicted to possess simultaneous ultrastrong field confinement and very low damping, enabling new classes of devices for deep-subwavelength metamaterials, single-photon nonlinearities, extraordinarily strong light-matter interactions and nano-optoelectronic switches. Although all of these great prospects require low damping, thus far strong plasmon damping has been observed, with both impurity scattering and many-body effects in graphene proposed as possible explanations. With the advent of van der Waals heterostructures, new methods have been developed to integrate graphene with other atomically flat materials. In this Article we exploit near-field microscopy to image propagating plasmons in high-quality graphene encapsulated between two films of hexagonal boron nitride (h-BN). We determine the dispersion and plasmon damping in real space. We find unprecedentedly low plasmon damping combined with strong field confinement and confirm the high uniformity of this plasmonic medium. The main damping channels are attributed to intrinsic thermal phonons in the graphene and dielectric losses in the h-BN. The observation and in-depth understanding of low plasmon damping is the key to the development of graphene nanophotonic and nano-optoelectronic devices.

Drude weight, plasmon dispersion, and ac conductivity in doped graphene sheets

We demonstrate that the plasmon frequency and Drude weight of the electron liquid in a doped graphene sheet are strongly renormalized by electron-electron interactions even in the long-wavelength limit. This effect is not captured by the random-phase approximation (RPA), commonly used to describe electron fluids, and is due to coupling between the center-of-mass motion and the pseudospin degree of freedom of the graphene’s masslessDiracfermions.Bymakinguseofdiagrammaticperturbationtheorytofirstorderintheelectron-electron interaction, we show that this coupling enhances both the plasmon frequency and the Drude weight relative to the RPA value. We also show that interactions are responsible for a significant enhancement of the optical conductivity at frequencies just above the absorption threshold. Our predictions can be checked by far-infrared spectroscopy or inelastic light scattering.

Plasmon losses due to electron-phonon scattering: The case of graphene encapsulated in hexagonal boron nitride

Graphene sheets encapsulated between hexagonal Boron Nitride (hBN) slabs display superb electronic properties due to very limited scattering from extrinsic disorder sources such as Coulomb impurities and corrugations. Such samples are therefore expected to be ideal platforms for highly-tunable low-loss plasmonics in a wide spectral range. In this Article we present a theory of collective electron density oscillations in a graphene sheet encapsulated between two hBN semi-infinite slabs (hBN/G/hBN). Graphene plasmons hybridize with hBN optical phonons forming hybrid plasmon-phonon (HPP) modes. We focus on scattering of these modes against graphenes acoustic phonons and hBN optical phonons, two sources of scattering that are expected to play a key role in hBN/G/hBN stacks. We find that at room temperature the scattering against graphenes acoustic phonons is the dominant limiting factor for hBN/G/hBN stacks, yielding theoretical inverse damping ratios of hybrid plasmon-phonon modes of the order of

Revealing the electronic band structure of trilayer graphene on SiC: An angle-resolved photoemission study

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Acoustic terahertz graphene plasmons revealed by photocurrent nanoscopy

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Intrinsic lifetime of Dirac plasmons in graphene

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Violation of the Wiedemann-Franz Law in Hydrodynamic Electron Liquids.

, with a weak dependence on carrier density and a strong dependence on illumination frequency. We confirm that the plasmon lifetime is not directly correlated with the mobility: in fact, it can be anti-correlated.

Impact of disorder on Dirac plasmon losses

In recent times, trilayer graphene has attracted wide attention owing to its stacking and electric-field-dependent electronic properties. However, a direct and well-resolved experimental visualization of its band structure has not yet been reported. In this paper, we present angle-resolved photoemission spectroscopy data which show with high resolution the electronic band structure of trilayer graphene obtained on alpha-SiC(0001) and beta-SiC(111) via hydrogen intercalation. Electronic bands obtained from tight-binding calculations are fitted to the experimental data to extract the interatomic hopping parameters for Bernal and rhombohedral stacked trilayers. Low-energy electron microscopy measurements demonstrate that the trilayer domains extend over areas of tens of square micrometers, suggesting the feasibility of exploiting this material in electronic and photonic devices. Furthermore, our results suggest that, on SiC substrates, the occurrence of a rhombohedral stacked trilayer is significantly higher than in natural bulk graphite. (Less)

Plasmons and Coulomb drag in Dirac/Schroedinger hybrid electron systems

Terahertz (THz) fields are widely used for sensing, communication and quality control. In future applications, they could be efficiently confined, enhanced and manipulated well below the classical diffraction limit through the excitation of graphene plasmons (GPs). These possibilities emerge from the strongly reduced GP wavelength, λp, compared with the photon wavelength, λ0, which can be controlled by modulating the carrier density of graphene via electrical gating. Recently, GPs in a graphene/insulator/metal configuration have been predicted to exhibit a linear dispersion (thus called acoustic plasmons) and a further reduced wavelength, implying an improved field confinement, analogous to plasmons in two-dimensional electron gases (2DEGs) near conductive substrates. Although infrared GPs have been visualized by scattering-type scanning near-field optical microscopy (s-SNOM), the real-space imaging of strongly confined THz plasmons in graphene and 2DEGs has been elusive so far-only GPs with nearly free-space wavelengths have been observed. Here we demonstrate real-space imaging of acoustic THz plasmons in a graphene photodetector with split-gate architecture. To that end, we introduce nanoscale-resolved THz photocurrent near-field microscopy, where near-field excited GPs are detected thermoelectrically rather than optically. This on-chip detection simplifies GP imaging as sophisticated s-SNOM detection schemes can be avoided. The photocurrent images reveal strongly reduced GP wavelengths (λp ≈ λ0/66), a linear dispersion resulting from the coupling of GPs with the metal gate below the graphene, and that plasmon damping at positive carrier densities is dominated by Coulomb impurity scattering.

Accessing Phonon Polaritons in Hyperbolic Crystals by Angle-Resolved Photoemission Spectroscopy

Dirac plasmons in a doped graphene sheet have recently been shown to enable confinement of light to ultrasmall volumes. In this work we calculate the intrinsic lifetime of a Dirac plasmon in a doped graphene sheet by analyzing the role of electron-electron interactions beyond the random phase approximation. The damping mechanism at work is intrinsic since it operates also in disorder-free samples and in the absence of lattice vibrations. We demonstrate that graphenes sublattice-pseudospin degree of freedom suppresses intrinsic plasmon losses with respect to those that occur in ordinary two-dimensional electron liquids. We relate our findings to a microscopic calculation of the homogeneous dynamical conductivity at energies below the single-particle absorption threshold.