Alexander Sinyuk

Application of spheroid models to account for aerosol particle nonsphericity in remote sensing of desert dust

[ 1] The possibility of using shape mixtures of randomly oriented spheroids for modeling desert dust aerosol light scattering is discussed. For reducing calculation time, look-up tables were simulated for quadrature coefficients employed in the numerical integration of spheroid optical properties over size and shape. The calculations were done for 25 bins of the spheroid axis ratio ranging from similar to 0.3 ( flattened spheroids) to similar to 3.0 ( elongated spheroids) and for 41 narrow size bins covering the size parameter range from similar to 0.012 to similar to 625. The look-up tables were arranged into a software package, which allows fast, accurate, and flexible modeling of scattering by randomly oriented spheroids with different size and shape distributions. In order to evaluate spheroid model and explore the possibility of aerosol shape identification, the software tool has been integrated into inversion algorithms for retrieving detailed aerosol properties from laboratory or remote sensing polarimetric measurements of light scattering. The application of this retrieval technique to laboratory measurements by Volten et al. ( 2001) has shown that spheroids can closely reproduce mineral dust light scattering matrices. The spheroid model was utilized for retrievals of aerosol properties from atmospheric radiation measured by AERONET ground-based Sun/sky-radiometers. It is shown that mixtures of spheroids allow rather accurate fitting of measured spectral and angular dependencies of observed intensity and polarization. Moreover, it is shown that for aerosol mixtures with a significant fraction of coarse-mode particles ( radii >= similar to 1 mu m), the nonsphericity of aerosol particles can be detected as part of AERONET retrievals. The retrieval results indicate that nonspherical particles with aspect ratios similar to 1.5 and higher dominate in desert dust plumes, while in the case of background maritime aerosol spherical particles are dominant. Finally, the potential of using AERONET derived spheroid mixtures for modeling the effects of aerosol particle nonsphericity in other remote sensing techniques is discussed. For example, the variability of lidar measurements ( extinction to backscattering ratio and signal depolarization ratio) is illustrated and analyzed. Also, some potentially important differences in the sensitivity of angular light scattering to parameters of nonspherical versus spherical aerosols are revealed and discussed.

Local analysis of MISR surface BRF and albedo over GSFC and mongu AERONET sites

We have developed an atmospheric correction algorithm to retrieve the surface bidirectional reflectance factor (BRF) and albedo from Multiangle Imaging SpectroRadiometer (MISR) measurements for small areas around Aerosol Robotic Network (AERONET) sunphotometer sites, using AERONET aerosol and column water vapor information. Our goal is to develop an indirect validation method for MISR surface reflectance products over heterogeneous land. Our algorithm makes independent retrievals with both the Li Sparse-Ross Thick kernel BRF model and the modified Rahman-Pinty-Verstraete BRF model used in the Moderate Resolution Imaging Spectroradiometer and MISR land algorithms, respectively. In this study, we report the first results of processing MISR Collection 4 data for 2003-2004 for two sites, Mongu, Zambia, and Greenbelt, MD. We found that MISR generally provides accurate retrievals of BRF and albedo in both clear and hazy atmospheric conditions, correctly reproducing the parameter time series and spatial distribution. We found that the MISR BRF, on average, is less anisotropic in the visible bands. The difference is greatest in the blue band, but decreases with increasing wavelength such that it is negligible in the near-IR band. This discrepancy originates in part in the MISR aerosol retrieval algorithm over heterogeneous land, which tends to select an aerosol model that favors spectrally invariant shapes of surface BRF. The other part of the discrepancy comes from the surface hemispherical-directional reflectance factor retrieval algorithm where the iteration loop that removes the diffuse atmospheric transmittance is currently turned off. Our initial results suggest that the MISR surface albedo is on average lower than our retrievals by about 0.005 in the green and red bands. In the near-IR, it agreed with our retrievals with the modified Rahman-Pinty-Verstraete model for the Mongu site, but was systematically lower over the Greenbelt site by about 0.016. When significant aerosol absorption is present (Mongu), the albedo discrepancy is additionally biased by the difference between the MISR and AERONET retrievals of aerosol absorption

Aerosol properties from multi-spectral and multi-angular aircraft 4STAR observations: expected advantages and challenges

The airborne Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) is developed to retrieve aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. The necessarily compact design of the 4STAR may cause noticeable apparent enhancement of sky radiance at small scattering angles. We assess the sensitivity of expected 4STAR-based aerosol retrieval to such enhancement by applying the operational AERONET retrieval code and synthetic 4STAR-like data. Also, we assess the sensitivity of the broadband radiative fluxes and the direct aerosol radiative forcing to uncertainties in aerosol retrievals associated with the sky radiance enhancement. Our sensitivity study results suggest that the 4STARbased aerosol retrieval has limitations in obtaining detailed information on particle size distribution and scattering phase function. However, these limitations have small impact on the retrieved bulk optical parameters, such as the asymmetry factor (up to 4%, or ±0.02) and single-scattering albedo (up to 2%, or ±0.02), and the calculated direct aerosol radiative forcing (up to 6%, or 2 Wm-2).

Aerosol and Surface Properties Characterization from Joint Inversion of Ground-Based and Satellite Observations

A method for simultaneously retrieving aerosol and surface parameters from ground based and satellite observations collocated in space and time is presented. The improvements in aerosol and surface reflectance characterization are discussed.