Alexey Kavokin

Spontaneous formation and optical manipulation of extended polariton condensates

Long-lived polariton condensates can propagate well beyond the area of their initial excitation while still maintaining spatial coherence. This enables direct and controllable manipulation of the condensate wavefunction.

Mie Resonances, Infrared Emission, and the Band Gap of InN

Mie resonances due to scattering or absorption of light in InN-containing clusters of metallic In may have been erroneously interpreted as the infrared band gap absorption in tens of papers. Here we show by direct thermally detected optical absorption measurements that the true band gap of InN is markedly wider than the currently accepted 0.7 eV. Microcathodoluminescence studies complemented by the imaging of metallic In have shown that bright infrared emission at 0.7-0.8 eV arises in a close vicinity of In inclusions and is likely associated with surface states at the metal/InN interfaces.

Observation of half-quantum vortices in an exciton-polariton condensate

Quantum Division The notion of quantum mechanics is that variables are expressed as integer values. In quantum fluids, for instance, vortices are quantized in terms of the polarization and phase shifts observed as multiples of 2π, that is, full rotations of each variable around the vortex core. Theoretical work has predicted that in some instances there should be half-quantum vortices, where circumventing the vortex core is characterized by just π rotations of the phase and polarization. By observing exciton-polariton condensates Lagoudakis et al. (p. 974) present evidence for the existence of these long-predicted half-quantum vortices. Evidence is presented for the existence of half-quantum vortices in exciton-polariton condensates. Singly quantized vortices have already been observed in many systems, including the superfluid helium, Bose-Einstein condensates of dilute atomic gases, and condensates of exciton-polaritons in the solid state. Two-dimensional superfluids carrying spin are expected to demonstrate a different type of elementary excitations referred to as half-quantum vortices, characterized by a π rotation of the phase and a π rotation of the polarization vector when circumventing the vortex core. We detect half-quantum vortices in an exciton-polariton condensate by means of polarization-resolved interferometry, real-space spectroscopy, and phase imaging. Half-quantum vortices coexist with single-quantum vortices in our sample.

Room-temperature polariton lasers based on GaN microcavities

The critical temperature for Bose condensation of exciton polaritons in an AlGaN microcavity containing 9 GaN quantum wells is calculated to be T5460 K. We have modeled the kinetics of polaritons in such a microcavity device using the two-dimensional Boltzmann equation. Room-temperature lasing is found with a threshold as small as 100 mW. The kinetic blocking of polariton relaxation that prevents formation of the Bose-condensed phase of polaritons at low temperatures disappears at high temperatures, especially in n-doped samples. Thus, GaN microcavities are excellent candidates for realization of room-temperature polariton lasers.

Giant exciton-light coupling in ZnO quantum dots

We investigate the strength of the coupling of the electronic states with the electromagnetic field in ZnO nanospheres, taking into account the retardation effect. We show that the coupling strength is particularly strong: the bulk properties are so enhanced that the radiative decay time can reach some 200 ps for quantum dot sizes of some 30 nm.

Spontaneous coherence in a cold exciton gas

If bosonic particles are cooled down below the temperature of quantum degeneracy, they can spontaneously form a coherent state in which individual matter waves synchronize and combine. Spontaneous coherence of matter waves forms the basis of a number of fundamental phenomena in physics, including superconductivity, superfluidity and Bose–Einstein condensation. Spontaneous coherence is the key characteristic of condensation in momentum space. Excitons—bound pairs of electrons and holes—form a model system to explore the quantum physics of cold bosons in solids. Cold exciton gases can be realized in a system of indirect excitons, which can cool down below the temperature of quantum degeneracy owing to their long lifetimes. Here we report measurements of spontaneous coherence in a gas of indirect excitons. We found that spontaneous coherence of excitons emerges in the region of the macroscopically ordered exciton state and in the region of vortices of linear polarization. The coherence length in these regions is much larger than in a classical gas, indicating a coherent state with a much narrower than classical exciton distribution in momentum space, characteristic of a condensate. A pattern of extended spontaneous coherence is correlated with a pattern of spontaneous polarization, revealing the properties of a multicomponent coherent state. We also observed phase singularities in the coherent exciton gas. All these phenomena emerge when the exciton gas is cooled below a few kelvin.

Optical Tamm states for the fabrication of polariton lasers

We propose to embed the ultrathin layer of an organic or inorganic material at the boundary between two specially designed periodic dielectric structures in order to achieve the strong coupling between Frenkel or Wannier-Mott excitons and optical Tamm states localized at the interface. This would allow the fabrication of polariton lasers without microcavities that could be easier from the technological point of view. Analytical formulas are given for the energies of optical Tamm states and the constant of their coupling to excitons.

Exciton-polariton mediated superconductivity.

We revisit the exciton mechanism of superconductivity in the framework of microcavity physics, replacing virtual excitons as a binding agent of Cooper pairs by excitations of an exciton-polariton Bose-Einstein condensate. We consider a model microcavity where a quantum well with a two-dimensional electron gas is sandwiched between two undoped quantum wells, where a polariton condensate is formed. We show that the critical temperature for superconductivity dramatically increases with the condensate population, opening a new route towards high-temperature superconductivity.

Exciton mediated self-organization in glass driven by ultrashort light pulses

We propose an exciton-polariton-mediated self-organization effect in transparent SiO2 glass under intense femtosecond light irradiation. Interference and dipole-dipole interaction of polaritons causes formation of gratings of dielectric polarization. Due to an ultrafast exciton self-localization into a quasicrystal structure, the polariton gratings remain frozen in glass and a permanent three-dimensional image of exciton-polariton gas is created. We show that coherent effects in propagation of exciton-polaritons can serve as a tool for nanostructuring and fabrication of 5-dimensional optical memories in glass, opening new horizons for polaritronics.

Room-temperature Tamm-plasmon exciton-polaritons with a WSe2 monolayer.

Solid-state cavity quantum electrodynamics is a rapidly advancing field, which explores the frontiers of light–matter coupling. Metal-based approaches are of particular interest in this field, as they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit. Transition metal dichalcogenides are ideally suited as the active material in cavity quantum electrodynamics, as they interact strongly with light at the ultimate monolayer limit. Here, we implement a Tamm-plasmon-polariton structure and study the coupling to a monolayer of WSe2, hosting highly stable excitons. Exciton-polariton formation at room temperature is manifested in the characteristic energy–momentum dispersion relation studied in photoluminescence, featuring an anti-crossing between the exciton and photon modes with a Rabi-splitting of 23.5 meV. Creating polaritonic quasiparticles in monolithic, compact architectures with atomic monolayers under ambient conditions is a crucial step towards the exploration of nonlinearities, macroscopic coherence and advanced spinor physics with novel, low-mass bosons.