Annapoorna Akella

Digital holographic storage system incorporating optical fixing

Digital holograms have been written in stoichiometric Pr:LiNbO(3) in a two-color recording scheme, demonstrating what is to our knowledge the first all-optical nondestructive readout of digital data. Using writing light at 800nm and gating light at 476 nm, we stored and retrieved 256-kbit digital data pages with a raw bit-error rate BER of <10(-4) .

Synthesis and characterization of photochromic organic films for holographic recording

Polymer films doped with 2-(5, 5-dimethyl-3-styryl-cyclohex-2-enylidene)-malononitrile chromophore and various sensitizers have been prepared and characterized. The material exhibits high sensitivity in the red region (S=0.26 cm(2)/J at lambda=633 nm), a large dynamic range (Dn=-0.05) , and large transient two-beam coupling gain (G=110 cm(-1)) . Self-diffraction effects, such as energy and phase coupling, and photoinduced scattering are studied.

One-color one-beam pumping of Er(3+)-doped ZBLAN glasses for a three-dimensional two-step excitation display.

We demonstrate a one-color one-beam pumping method for a three-dimensional two-step excitation fluorescent display with Er(3+) -doped ZBLAN glass. A localized green fluorescent spot is obtained by use of a focused pump-light beam at 979 nm. The quantum efficiency of the two-step excitation fluorescence is investigated in a time-dependent analysis and an experiment with a pulsed pump light.

Two-photon holographic recording in aluminosilicate glass containing silver particles.

Recording of holographic gratings by 532-nm laser pulses in photochromic bulk aluminosilicate glass containing silver particles is demonstrated. A diffraction efficiency of 1.5% is achieved for readout at the same wavelength. The speed of grating formation as a function of pulse energy suggests that two-photon excitation is responsible for the recording. The light causes bleaching of an absorption peak near 417nm, which corresponds to the excitation of surface plasmons on the silver, and broad darkening throughout the visible to the near infrared. A likely mechanism for the photochromic effect is discussed.

New fluoroindate glass compositions

Abstract New multicomponent InF 3 -based bulk glasses have been investigated. The molar composition of the base glass is 28% InF 3 –20% ZnF 2 –16.5% BaF 2 –12% GaF 3 –9% PbF 2 –6% NaCl–5% SrF 2 –3% CaF 2 –0.5% PrF 3 . A number of variations of the base glass were prepared and their refractive indices and densities measured. Resistance to crystallization allowed the preparation of large pieces of the base glass. The infrared and Raman spectra show that the base composition has a longer wavelength multiphonon edge at 10 μm and a phonon energy of 509 cm −1 , in comparison with 8 μm and 574 cm −1 for ZBLAN, which reveals that the present glasses have a lower phonon energy and a greater transparency in the infrared than ZBLAN. Reduction of PbF 2 concentration in the base composition provided glasses with smaller refractive indices than the base glass.

Properties of compositional volume grating formation with photoinitiated cationic-ring-opening polymerization

We investigated compositional volume grating formation in the Polaroid medium that utilizes the cationic-ring-opening photoinitiated polymerization process, and compared our conclusions with the current physical model describing polymer holographic recording. We identified the effects of diffusion and polymerization during illumination, as well as significant postexposure grating development. Holographic recording in this medium allows for final strong gratings with high recording sensitivity (S approximately 2 cm/mJ), that were not limited at the higher recording intensities (I less than or equal to 250 mW/cm2) corresponding to photon (exposure) limited recording. The results of the present analysis allow for more comprehensive physical description of grating formation in the photoinitiated CROP process, and evaluation of the polymer recording process in a nonvolatile holographic storage system.