Arati Prakash

Spin Seebeck effect through antiferromagnetic NiO

We report temperature-dependent spin Seebeck measurements on Pt/YIG bilayers and Pt/NiO/YIG trilayers, where YIG (yttrium iron garnet,

Magnon-drag thermopower and Nernst coefficient in Fe, Co and Ni

{\mathrm{Y}}_{3}\mathrm{F}{\mathrm{e}}_{5}{\mathrm{O}}_{12}

Dirac dispersion generates unusually large Nernst effect in Weyl semimetals

) is an insulating ferrimagnet and NiO is an antiferromagnet at low temperatures. The thickness of the NiO layer is varied from 0 to 10 nm. In the Pt/YIG bilayers, the temperature gradient applied to the YIG stimulates dynamic spin injection into the Pt, which generates an inverse spin Hall voltage in the Pt. The presence of a NiO layer dampens the spin injection exponentially with a decay length of 2 \ifmmode\pm\else\textpm\fi{} 0.6 nm at 180 K. The decay length increases with temperature and shows a maximum of 5.5 \ifmmode\pm\else\textpm\fi{} 0.8 nm at 360 K. The temperature dependence of the amplitude of the spin Seebeck signal without NiO shows a broad maximum of 6.5 \ifmmode\pm\else\textpm\fi{} 0.5 \ensuremath{\mu}V/K at 20 K. In the presence of NiO, the maximum shifts sharply to higher temperatures, likely correlated to the increase in decay length. This implies that NiO is most transparent to magnon propagation near the paramagnet-antiferromagnet transition. We do not see the enhancement in spin current driven into Pt reported in other papers when 1--2 nm NiO layers are sandwiched between Pt and YIG.

BiSb and spin-related thermoelectric phenomena

Magnon drag is shown to dominate the thermopower of elemental Fe from 2 to 80 K and of elemental Co from 150 to 600 K; it is also shown to contribute to the thermopower of elemental Ni from 50 to 500 K. Two theoretical models are presented for magnon-drag thermopower. One is a hydrodynamic theory based purely on nonrelativistic, Galilean, spin-preserving electron-magnon scattering. The second is based on spin-motive forces, where the thermopower results from the electric current pumped by the dynamic magnetization associated with a magnon heat flux. In spite of their very different microscopic origins, the two give similar predictions for pure metals at low temperature, allowing us to semiquantitatively explain the observed thermopower of elemental Fe and Co without adjustable parameters. We also find that magnon drag may contribute to the thermopower of Ni. A spin-mixing model is presented that describes the magnon-drag contribution to the anomalous Nernst effect in Fe, again enabling a semiquantitative match to the experimental data without fitting parameters. Our paper suggests that particle nonconserving processes may play an important role in other types of drag phenomena and also gives a predicative theory for improving metals as thermoelectric materials.

Thermal spin transport and energy conversion

Weyl semimetals expand research on topologically protected transport by adding bulk Berry monopoles with linearly dispersing electronic states and topologically robust, gapless surface Fermi arcs terminating on bulk node projections. Here, we show how the Nernst effect, combining entropy with charge transport, gives a unique signature for the presence of Dirac bands. The Nernst thermopower of NbP (maximum of 800 microV K-1 at 9 T, 109 K) exceeds its conventional thermopower by a hundredfold and is significantly larger than the thermopower of traditional thermoelectric materials. The Nernst effect has a pronounced maximum near T_M=90 +/- 20 K=mu_0/kB (mu_0 is chemical potential at T=0 K). A self-consistent theory without adjustable parameters shows that this results from electrochemical potential pinning to the Weyl point energy at T>=TM, driven by charge neutrality and Dirac band symmetry. Temperature and field dependences of the Nernst effect, an even function of the charge polarity, result from the intrinsically bipolar nature of the Weyl fermions. Through this study, we offer an understanding of the temperature dependence of the position of the electrochemical potential vis-a-vis the Weyl point, and we show a direct connection between topology and the Nernst effect, a potentially robust experimental tool for investigating topological states and the chiral anomaly.

Nernst Effect in the Weyl Semimetal NbP

This article reviews the factors limiting the figure of merit zT of conventional thermoelectrics especially at cryogenic temperatures and then highlights modern approaches used to increase zT below 200 K. Two type of materials are discussed. The first are BiSb alloys, relatively conventional thermoelectrics in which the zT is enhanced by using resonant levels. The second is the spin- Seebeck effect (SSE), a new solid-state energy conversion technology. Classical thermoelectric and SSE physics are combined to provide new concepts, like magnon-drag, in which we hope to increase the performance of solid-state coolers by exploiting the spin degree of freedom.