Armando Reale

Diffraction of x rays in capillary optics.

Propagation of x rays generated by a small-diameter incoherent source through the capillary waveguide that satisfies the multimode condition is studied with the Fresnel-Kirchhoff diffraction theory. The strong influence of diffraction on the propagation is demonstrated. The diffraction phenomenon is manifested by the appearance of diffraction fringes in both the guide channel and the far-field zone of the capillary output. Experimental data that confirm such behavior of the x-ray radiation is also presented. The results confirm the interference effects recently observed in some experiments on the grazing reflections of x rays in single- and multiple-capillary optics.

Large-field high-resolution x-ray monochromatic microscope based on spherical crystals and high-repetition-rate laser-produced plasmas

The combination of a table-top laser produced plasma X-ray source and spherically bent crystals for the soft X-ray region is used in traditional X-ray microscopy schemes. The X-ray source is well localized both spatially (approximately 20 micrometer) and temporally (1 ps - 10 ns, it depends on the used laser) and it is spectrally tunable in a relatively wide range (6 - 19 angstrom). High quality monochromatic ((delta) (lambda) /(lambda) approximately 10-5 - 10-3) images with high spatial resolution (up to approximately 4 micrometer) and in a large field of view (few mm) are presented. For many applications, these low-cost compact systems can offer a simple alternative to the larger installations which are usually used. It was demonstrated that the spherically bent crystals can be efficiently used in a wide ((Theta) equals 40 - 90 degrees) range of reflection angles, thus allowing wide wavelength selection. A very efficient concentration of monochromatic X-Ray radiation into different spot shapes (line, circle spot, etc) is demonstrated.

X-ray contact microscopy using a plasma source generated by long and short (120-ns and 10-ns) excimer laser pulses

Soft x-ray contact microscopy (SXCM), using a pulsed x-ray source, offers the possibility of imaging the ultrastructure of living biological systems at sub-50nm resolution. We have developed a pulsed plasma x-ray source for this application, generated by the large volume XeCl laser Hercules. Various unstable optical resonator configurations were employed to achieve a high laser intensity to increase the conversion efficiency to water window x-rays (280-530eV). Optimum plasma conditions for SXCM are discussed, including the effect of pulse duration on image resolution. Soft x-ray contact images of Chlamydomonas dysosmos (unicellular alga) and the cyanobacteria Leptolyngbya are shown. In addition, the potential of producing a movie film of the development of x-ray images within the photoresist (acting as the recording medium) is discussed, following the resist development while viewing by atomic force microscopy.

Lithium fluoride coloration by laser-plasma soft x-rays: a promising tool for x-ray microscopy and photonics

A new imaging detector for EUV or soft-X-ray radiation based on optically stimulated luminescence (OSL) of lithium fluoride (LiF) films or crystals is presented. The first micro-radiography images of biological samples and of meshes obtained on LiF using a laser-plasma source or an X-ray laser are shown, and (up to now) a resolution better than one micron is demonstrated. The dependence of the coloration density vs the deposited X-ray dose is considered and the advantages of this new diagnostic technique for both coherent and non-coherent EUV sources, compared with CCDs detectors, photographic films and photoresists are discussed. This new detector is extremely suitable for laser plasmas and for X-ray lasers sources.

Novel portable high-luminosity monochromatically tunable x-ray microscope

A novel experimental setup for transmission x-ray microscopy is presented. It is based on the use of a point isotropic x- ray source and a single spherical crystal. The x-ray beam intensity is modulated by the object attenuation, then monochromatized and enlarged using a spherical crystal and, lastly, imaged using a detector downstream of the crystal. We demonstrate by ray tracing technique and experimental testing that this system allows microscopy studies with image resolution better than the dimensions of the source, high magnification ratios, and great field of view. Microscopes using this model ca be easily built using different micro x-ray sources, like conventional x-ray tube generators, x-rays emitted by laser generated plasmas or synchrotron radiation. Utilization of spherically bent crystals to obtain high-resolution, large field, monochromatic images in a wide range of Bragg angles is demonstrated for the first time. High quality monochromatic images with high magnification about 15-35 times and spatial resolution over a large field of view were obtained. Some possible applications and preliminary experimental verification of the feasibility of the setup are also presented.

Atmospheric-pressure soft x-ray source for contact microscopy and radiobiology applications

A large volume non-conventional XeCl excimer laser (HERCULES) emitting long pulses (from 10 ns up to 120 ns at a wavelength of 308 nm) has been used to drive a soft x-ray plasma source. The x-rays pulse duration and the energy conversion efficiency in different spectral regions have been measured; x-rays emission lasting up to 100 ns has been obtained in the 70 eV region. The dependence of x-ray pulse duration on the size of the laser spot is discussed. The x- ray source can be operated both in vacuum and in helium at atmospheric pressure. This allows irradiating over a large area both for contact microscopy of living specimens (up to 1 mm2 windows) and for radiobiology (up to some cm2 windows). The experimental results obtained for these two applications as well as for radiographic images of living insects are discussed.

Double-pulse excitation of x-ray capillary lasers

We propose to enhance the gain of Ne-like ion capillary lasers by the utilization of two discharge pulses. A first pulse working in the pinch regime mode is designed to create the cold-plasma column with the required ionization degree, followed by a second fast high-voltage pulse to do the effective collision excitation. The second pulse, which heats the electrons to a kinetic temperature Te greater than Tecold in times shorter than the ionization time, increases the laser gain. In the two stage pumping scheme, both the amplitude of each of the pulses and the delay between them can be adjusted for independent control of the ionization degree and excitation rate. Numerical estimations performed for the low-Z-ion (Na+1, . . ., Ar+8) lasers with the double pulse pumping predict enhancement in gain by a factor of approximately 10. In addition, the extension of two-stage electrical pumping to the high-Z-ion collision and recombination laser schemes is discussed. Description of the experimental set-up constructed for such experiments and some related measurement data are also presented.

Characteristics of a soft x-ray plasma source for different pumping laser configurations and spectral analysis

A large volume long pulse excimer laser ((lambda) equals 308 nm) is used to generate a soft x- ray plasma source with long heating time at a power density in the order of 1012 - 1014 W/cm2. The characteristics of the plasma source for different laser pulse time evolution in the range 10-120 ns and for different target materials are investigated. In particular the most suitable source conditions (spectral energy distribution, time duration, etc.) for specific applications are analyzed.

Highly efficient x-ray imaging and backlighting schemes based on spherically bent crystals

New approaches of a spectrally tunable backlighting schemes based on a spherically bent crystal are considered. In a contrary to the traditional backlighting scheme, in which the investigated objects should be placed between the backlighter and the crystal, for the considered schemes an object is placed downstream of the crystal, before the tangential or after the sagittal focus and an image of the object is recorded at the distance from the object corresponded to the needed magnification. The magnification is defined by the ratio of the distances form the sagittal focus to the detector and from the object to the sagittal focus. A ray tracing modeling and experimental images of test meshes, obtained at an incidence angles of the backlighter radiation of 10° and 22°, are presented. It is demonstrated that, at incident angles up to 22°, a linear transformation of the obtained astigmatic images allows to reconstruct them with an accuracy (5 - 15%). A spatial resolution around 10 μm in a field of view of some mm2 is achieved, for the spectral range around 9 Å. It is also demonstrated that spherically bent crystals could be used for X-ray imaging of a self emitting plasma structures with a spatial resolution at least 50 μm in a field of view of some square millimeters for angles of incidence up to 22°.

Far-field, near-field and interference patterns imaging in LiF crystals from a 46.9-nm capillary discharge pumped soft-x-ray laser

The recent progress in the development of the tabletop soft x-ray lasers pumped by capillary discharges has opened the possibility of the widespread use of these coherent sources for applications. In this paper, we present the latest results achieved in our laboratory concerning the optimization of a 46.9nm capillary discharge pumped soft x-ray laser and the imaging of the laser beam on Lithium Fluoride (LiF, films), which appears to be a new promising x-ray detector. The use of LiF allows a high spatial resolution (smaller than 1μm) on large areas, high-contrast imaging and simple manipulation. The laser, which is pumped by 18-20kA, 150-180ns long current pulses at a repetition rate of 0.1Hz, is produced in 3.2mm diameter up to 45cm length alumina capillary tubes filled with Ar at the initial gas pressure of 300-600mTorr. At the capillary lengths examined, the laser is operating in the saturation regime giving an output energy of about 300μJ per pulse and high coherence degree.