Atsuyuki Sorimachi

Thyroid doses for evacuees from the Fukushima nuclear accident

A primary health concern among residents and evacuees in affected areas immediately after a nuclear accident is the internal exposure of the thyroid to radioiodine, particularly I-131, and subsequent thyroid cancer risk. In Japan, the natural disasters of the earthquake and tsunami in March 2011 destroyed an important function of the Fukushima Daiichi Nuclear Power Plant (F1-NPP) and a large amount of radioactive material was released to the environment. Here we report for the first time extensive measurements of the exposure to I-131 revealing I-131 activity in the thyroid of 46 out of the 62 residents and evacuees measured. The median thyroid equivalent dose was estimated to be 4.2 mSv and 3.5 mSv for children and adults, respectively, much smaller than the mean thyroid dose in the Chernobyl accident (490 mSv in evacuees). Maximum thyroid doses for children and adults were 23 mSv and 33 mSv, respectively.

The time variation of dose rate artificially increased by the Fukushima nuclear crisis

A car-borne survey for dose rate in air was carried out in March and April 2011 along an expressway passing northwest of the Fukushima Dai-ichi Nuclear Power Station which released radionuclides starting after the Great East Japan Earthquake on March 11, 2011, and in an area closer to the Fukushima NPS which is known to have been strongly affected. Dose rates along the expressway, i.e. relatively far from the power station were higher after than before March 11, in some places by several orders of magnitude, implying that there were some additional releases from Fukushima NPS. The maximum dose rate in air within the high level contamination area was 36 μGy h−1, and the estimated maximum cumulative external dose for evacuees who came from Namie Town to evacuation sites (e.g. Fukushima, Koriyama and Nihonmatsu Cities) was 68 mSv. The evacuation is justified from the viewpoint of radiation protection.

Preliminary results of simultaneous radon and thoron tests in Ottawa

Ottawa is the capital city of Canada. In the previous cross Canada radon survey, Ottawa was not included. There is great interest to know radon level as well as thoron concentration in Ottawa homes. Therefore, radon/thoron discrimination detectors developed at the National Institute of Radiological Sciences in Japan were deployed in 93 houses for a period of 3 months. As expected, thoron is present in Ottawa homes. Radon concentrations ranged from 8 to 1525 Bq m(-3) while thoron concentrations varied from 5 to 924 Bq m(-3). The arithmetic mean of radon and thoron concentrations were found to be 110 +/- 168 and 56 +/- 123 Bq m(-3), respectively.

International intercomparisons of integrating radon detectors in the NIRS radon chamber.

An international intercomparison of integrating detectors was conducted at NIRS (National Institute of Radiological Science, Japan) with a 24.4 m(3) inner volume walk-in radon chamber that has systems to control radon concentration, temperature and humidity. During the first intercomparison (05.2007) four groups participated from four countries and for the second intercomparison (10.2007) 17 participants were involved from 11 countries. Most of detectors are in good agreement with each other when compared to the radon level provided by the radon chamber. It appeared that the 70% of detectors are unified within the 20% margin of uncertainty.

Activity concentrations of environmental samples collected in Fukushima Prefecture immediately after the Fukushima nuclear accident

Radionuclide concentrations in environmental samples such as surface soils, plants and water were evaluated by high purity germanium detector measurements. The contribution rate of short half-life radionuclides such as 132I to the exposure dose to residents was discussed from the measured values. The highest values of the 131I/137Cs activity ratio ranged from 49 to 70 in the environmental samples collected at Iwaki City which is located to the south of the F1-NPS. On the other hand, the 132I/131I activity ratio in the same environmental samples had the lowest values, ranging from 0.01 to 0.02. By assuming that the 132I/131I activity ratio in the atmosphere was equal to the ratio in the environmental samples, the percent contribution to the thyroid equivalent dose by 132I was estimated to be less than 2%. Moreover, the contribution to the thyroid exposure by 132I might be negligible if 132I contamination was restricted to Iwaki City.

Estimation of internal exposure of the thyroid to 131I on the basis of 134Cs accumulated in the body among evacuees of the Fukushima Daiichi Nuclear Power Station accident

Namie Town was heavily contaminated by the Fukushima Daiichi Nuclear Power Station accident. The thyroid equivalent dose for residents who lived in Namie was estimated using results of whole body counting examinations which were carried out by the Japan Atomic Energy Agency a few months after the nuclear accident. Photon peaks of (131)I and (134)Cs were previously measured by the authors using a NaI(Tl) scintillation spectrometer and that information was used to estimate the (131)I/(134)Cs activity ratio of total intake in the present study. The maximum values of (131)I/(134)Cs activity ratio corresponding to thyroid uptake factors of 0.3, 0.1 and 0.03 were evaluated to be 0.9, 2.6 and 8.7, respectively. The maximum value of the (131)I/(134)Cs activity ratio was used to obtain the most conservative thyroid equivalent dose estimation. The maximum internal exposure of the thyroid to (131)I on the basis of (134)Cs accumulated in the body measured by the whole body counter was estimated to be 18mSv. This value was much smaller than 50mSv that the International Atomic Energy Agency recommends as the dose at which exposed persons should take stable iodine tablets.

LONG-TERM MEASUREMENTS OF THORON, ITS AIRBORNE PROGENY AND RADON IN 205 DWELLINGS IN IRELAND

Long-term (circa 3 months) simultaneous measurements of indoor concentrations of thoron gas, airborne thoron progeny and radon were made using passive alpha track detectors in 205 dwellings in Ireland during the period 2007-09. Thoron progeny concentrations were measured using passive deposition monitors designed at the National Institute of Radiological Sciences (NIRS), Japan, whereas thoron gas concentrations were measured using Raduet detectors (Radosys, Budapest). Radon concentrations were measured in these dwellings by means of NRPB/SSI type alpha track radon detectors as normally used by the Radiological Protection Institute of Ireland (RPII). The concentration of thoron gas ranged from <1 to 174 Bq m(-3) with an arithmetic mean (AM) of 22 Bq m(-3). The concentration of radon gas ranged from 4 to 767 Bq m(-3) with an AM of 75 Bq m(-3). For radon, the estimated annual doses were 0.1 (min), 19.2 (max) and 1.9 (AM) mSv y(-1). The concentration of thoron progeny ranged from <0.1 to 3.8 Bq m(-3) [equilibrium equivalent thoron concentration (EETC)] with an AM of 0.47 Bq m(-3) (EETC). The corresponding estimated annual doses were 2.9 (max) and 0.35 (mean) mSv y(-1). In 14 or 7% of the dwellings, the estimated doses from thoron progeny exceeded those from radon.

Generation and control of thoron emanated from lantern mantles

This paper describes the performance of a thoron ((220)Rn) flowthrough source made of a commercially available lantern mantle. This (220)Rn source is easy to construct and operate and has a negligible radon ((222)Rn) gas generated when the air was passed through the source. We studied the (220)Rn concentration generated from the lantern mantles in terms of the variability in concentration associated with both the total weight of the lantern mantles used in the source and the air flow rate used in the experimental chamber. We found that the concentration of (220)Rn generated in air ranged from 0.9 to 150 kBq m(-3) and exponentially depended on the absolute humidity. The (220)Rn concentration increased linearly with increasing total weight of the lantern mantles, but variations in the rate of air flow passed through the source had no influence on the observed (220)Rn concentration.

Simultaneous 222Rn and 220Rn measurements in Winnipeg, Canada

Naturally occurring isotopes of radon in indoor air are identified as the second leading cause of lung cancer after tobacco smoking. Winnipeg had the highest radon ((222)Rn) concentration among 18 Canadian cities surveyed in the past. There is great interest to know the current radon as well as thoron ((220)Rn) concentrations in Winnipeg homes. Therefore, radon-thoron discrimination detectors were deployed in 117 houses for a period of 3 months. The results confirmed that thoron is present at detectable levels in about half of the Winnipeg homes and radon remains significantly higher than the national average. In this study, radon concentrations ranged from 20 to 483 Bq m(-3) with a geometric mean of 112 Bq m(-3) and a geometric standard deviation of 2.07. It is estimated that 20% of Winnipeg homes could have radon concentrations above the Canadian indoor radon guideline of 200 Bq m(-3). This conclusion is similar to the previous estimation made 20 y ago. Thoron concentrations were below the detection limit in 60 homes. Among the homes with detectable thoron concentrations, the values varied from 5 to 297 Bq m(-3), the geometric mean and standard deviation were 21 Bq m(-3) and 2.53, respectively.

Preliminary indoor thoron measurements in high radiation background area of southeastern coastal Orissa, India

This paper presents the preliminary results of radon and thoron measurements in the houses of Chhatrapur area of southeastern coast of Orissa, India. This area is one of the high radiation background radiation areas in India, which consists of monazite sand as the source of thoron. Both active and passive methods were employed for the measurements. Radon and thoron concentrations were measured in the houses of Chhatrapur area using twin cup radon dosemeters, RAD7 and radon-thoron discriminative detector (Raduet). Thoron progeny concentration was also measured in the houses using deposition rate measurements. Radon and thoron concentrations in the houses of study area were found to vary from 8 to 47 Bq m(-3) and the below detection level to 77 Bq m(-3), respectively. While thoron progeny concentration in these houses ranges between 0.17 and 4.24 Bq m(-3), preliminary investigation shows that the thoron concentration is higher than radon concentration in the houses of the study area. The thoron progeny concentration was found to be comparatively higher, which forms a base for further study in the area. The comparison between the results of various techniques is presented in this paper.