Avi Pe'er

A High Phase-Space-Density Gas of Polar Molecules

A quantum gas of ultracold polar molecules, with long-range and anisotropic interactions, not only would enable explorations of a large class of many-body physics phenomena but also could be used for quantum information processing. We report on the creation of an ultracold dense gas of potassium-rubidium (40K87Rb) polar molecules. Using a single step of STIRAP (stimulated Raman adiabatic passage) with two-frequency laser irradiation, we coherently transfer extremely weakly bound KRb molecules to the rovibrational ground state of either the triplet or the singlet electronic ground molecular potential. The polar molecular gas has a peak density of 1012 per cubic centimeter and an expansion-determined translational temperature of 350 nanokelvin. The polar molecules have a permanent electric dipole moment, which we measure with Stark spectroscopy to be 0.052(2) Debye (1 Debye = 3.336 × 10–30 coulomb-meters) for the triplet rovibrational ground state and 0.566(17) Debye for the singlet rovibrational ground state.

Two Photon Absorption and Coherent Control with Broadband Down-Converted Light

We experimentally demonstrate two-photon absorption with broadband down-converted light (squeezed vacuum). Although incoherent and exhibiting the statistics of a thermal noise, broadband down-converted light can induce two-photon absorption with the same sharp temporal behavior as femtosecond pulses, while exhibiting the high spectral resolution of the narrow band pump laser. Using pulse-shaping methods, we coherently control two-photon absorption in rubidium, demonstrating spectral and temporal resolutions that are 3-5 orders of magnitude below the actual bandwidth and temporal duration of the light itself. Such properties can be exploited in various applications such as spread-spectrum optical communications, tomography, and nonlinear microscopy.

Temporal shaping of entangled photons

We experimentally demonstrate shaping of the two-photon wave function of entangled-photon pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the second-order correlation function of the photons exactly like a coherent ultrashort pulse. To observe the shaping we perform sum-frequency generation with an ultrahigh flux of entangled photons. At the appropriate conditions, sum-frequency generation performs as a coincidence detector with an ultrashort response time (approximately 100 fs), enabling a direct observation of the two-photon wave function. This property also enables us to demonstrate background-free, high-visibility two-photon interference oscillations.

Nonlinear interactions with an ultrahigh flux of broadband entangled photons.

We experimentally demonstrate sum-frequency generation with entangled photon pairs, generating as many as 40,000 photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a linear intensity dependence of the nonlinear process. The key element in our scheme is the generation of an ultrahigh flux of entangled photons while maintaining their nonclassical properties. This is made possible by generating the down-converted photons as broadband as possible, orders of magnitude wider than the pump. This approach can be applied to other nonlinear interactions, and may become useful for various quantum-measurement tasks.

Direct frequency comb spectroscopy

We summarize recent developments in direct frequency-comb spectroscopy that allowed high-resolution, broad-bandwidth measurements of multiple atomic and molecular resonances using only a phase-stabilized femtosecond laser, opening the way for merging precision spectroscopy with coherent control.

Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb

We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within the framework of coherent control in the perturbative regime, while coherent accumulation of many pulse pairs enables near unity transfer efficiency with a high spectral selectivity, thus forming a powerful combination of pump-dump control schemes and the precision of the frequency comb. Simulations verify the feasibility and robustness of this concept, with the aim to form deeply bound, ultracold molecules.

Control of Four-Level Quantum Coherence via Discrete Spectral Shaping of an Optical Frequency Comb

We present experiments demonstrating high-resolution and wide-bandwidth coherent control of a four-level atomic system in a diamond configuration. A femtosecond frequency comb is used to excite a specific pair of two-photon transitions in cold 87Rb. The optical-phase-sensitive response of the closed-loop diamond system is studied by controlling the phase of the comb modes with a pulse shaper. Finally, the pulse shape is optimized resulting in a 256% increase in the two-photon transition rate by forcing constructive interference between the mode pairs detuned from an intermediate resonance.

Piecewise Adiabatic Population Transfer in a Molecule via a Wave Packet

We propose a class of schemes for robust population transfer between quantum states that utilize trains of coherent pulses, thus forming a generalized adiabatic passage via a wave packet. We study piecewise stimulated Raman adiabatic passage with pulse-to-pulse amplitude variation, and piecewise chirped Raman passage with pulse-to-pulse phase variation, implemented with an optical frequency comb. In the context of production of ultracold ground-state molecules, we show that with almost no knowledge of the excited potential, robust high-efficiency transfer is possible.

Optical code-division multiple access using broad-band parametrically generated light

A novel approach for an optical direct-sequence spread spectrum is presented. It is based on the complementary processes of broad-band parametric down-conversion and up-conversion. With parametric down-conversion, a narrow-band continuous-wave (CW) optical field is transformed into two CW broad-band white-noise fields that are complex conjugates of each other. These noise fields are exploited as the key and conjugate key in optical direct-sequence spread spectrum. The inverse process of parametric up-conversion is then used for multiplying the key by the conjugate key at the receiver in order to extract the transmitted data. A complete scheme for optical code-division multiple access (OCDMA) based on this approach is presented. The salient feature of the approach presented in this paper is that an ideal white-noise key is automatically generated, leading to high-capacity versatile code-division multiple-access configurations.

Optical correlation with totally incoherent light.

An optical correlator that can operate with totally incoherent light is presented. Such a correlator can be designed to compensate completely for the inherent chromatic aberrations by resorting to elements with specialized, possibly impractical, dispersion characteristics. Nevertheless, a practical configuration that exploits available achromatic lenses and Fresnel zone plates was designed, built, and tested experimentally. The results reveal that detectable correlation peaks can be obtained with totally incoherent white light. The designs, experimental procedures, and results are presented.