Axel Griesmaier

Bose-Einstein Condensation of Chromium

We report on the generation of a Bose-Einstein condensate in a gas of chromium atoms, which have an exceptionally large magnetic dipole moment and therefore underlie anisotropic long-range interactions. The preparation of the chromium condensate requires novel cooling strategies that are adapted to its special electronic and magnetic properties. The final step to reach quantum degeneracy is forced evaporative cooling of 52Cr atoms within a crossed optical dipole trap. At a critical temperature of T(c) approximately 700 nK, we observe Bose-Einstein condensation by the appearance of a two-component velocity distribution. We are able to produce almost pure condensates with more than 50,000 condensed 52Cr atoms.

Observation of Dipole-Dipole Interaction in a Degenerate Quantum Gas

We have investigated the expansion of a Bose-Einstein condensate of strongly magnetic chromium atoms. The long-range and anisotropic magnetic dipole-dipole interaction leads to an anisotropic deformation of the expanding chromium condensate which depends on the orientation of the atomic dipole moments. Our measurements are consistent with the theory of dipolar quantum gases and show that a chromium condensate is an excellent model system to study dipolar interactions in such gases.

d-wave collapse and explosion of a dipolar bose-einstein condensate.

We investigate the collapse dynamics of a dipolar condensate of 52Cr atoms when the s-wave scattering length characterizing the contact interaction is reduced below a critical value. A complex dynamics, involving an anisotropic, d-wave symmetric explosion of the condensate, is observed. The atom number decreases abruptly during the collapse. We find good agreement between our experimental results and those of a numerical simulation of the three-dimensional Gross-Pitaevskii equation, including contact and dipolar interactions as well as three-body losses. The simulation indicates that the collapse induces the formation of two vortex rings with opposite circulations.

Strong dipolar effects in a quantum ferrofluid

Symmetry-breaking interactions have a crucial role in many areas of physics, ranging from classical ferrofluids to superfluid 3He and d-wave superconductivity. For superfluid quantum gases, a variety of new physical phenomena arising from the symmetry-breaking interaction between electric or magnetic dipoles are expected. Novel quantum phases in optical lattices, such as chequerboard or supersolid phases, are predicted for dipolar bosons. Dipolar interactions can also enrich considerably the physics of quantum gases with internal degrees of freedom. Arrays of dipolar particles could be used for efficient quantum information processing. Here we report the realization of a chromium Bose–Einstein condensate with strong dipolar interactions. By using a Feshbach resonance, we reduce the usual isotropic contact interaction, such that the anisotropic magnetic dipole–dipole interaction between 52Cr atoms becomes comparable in strength. This induces a change of the aspect ratio of the atom cloud; for strong dipolar interactions, the inversion of ellipticity during expansion (the usual ‘smoking gun’ evidence for a Bose–Einstein condensate) can be suppressed. These effects are accounted for by taking into account the dipolar interaction in the superfluid hydrodynamic equations governing the dynamics of the gas, in the same way as classical ferrofluids can be described by including dipolar terms in the classical hydrodynamic equations. Our results are a first step in the exploration of the unique properties of quantum ferrofluids.

Stabilization of a purely dipolar quantum gas against collapse

For the first time, a purely dipolar quantum gas has been prepared experimentally. Different regimes have been explored; in some, the gas is stable, whereas in others it collapses due to the strong dipole–dipole interaction between the constituent atoms.

Comparing Contact and Dipolar Interactions in a Bose-Einstein Condensate

We have measured the relative strength epsilon dd of the magnetic dipole-dipole interaction compared with the contact interaction in a dipolar chromium Bose-Einstein condensate. We analyze the asymptotic velocities of expansion of the condensate with different orientations of the atomic magnetic moments. By comparing the experimental results with numerical solutions of the hydrodynamic equations for dipolar condensates, we obtain epsilon dd = 0.159+/-0.034. We use this result to determine the s-wave scattering length a = (5.08+/-1.06 x 10(-9)) m = (96+/-20) a0 of 52Cr. This is fully consistent with our previous measurements on the basis of Feshbach resonances and therefore confirms the validity of the theoretical approach used to describe the dipolar Bose-Einstein condensate.

Observation of Feshbach Resonances in an Ultracold Gas of 52Cr

We have observed Feshbach resonances in collisions between ultracold 52Cr atoms. This is the first observation of collisional Feshbach resonances in an atomic species with more than one valence electron. The zero nuclear spin of 52Cr and thus the absence of a Fermi-contact interaction leads to regularly spaced resonance sequences. By comparing resonance positions with multichannel scattering calculations we determine the s-wave scattering length of the lowest (2S+1)Sigma(+)(g) potentials to be 112(14) a(0), 58(6) a(0), and -7(20) a(0) for S=6, 4, and 2, respectively, where a(0)=0.0529 nm.

Expansion dynamics of a dipolar Bose-Einstein condensate

Our recent measurements on the expansion of a chromium dipolar condensate after release from an optical trapping potential are in good agreement with an exact solution of the hydrodynamic equations for dipolar Bose gases. We report here the theoretical method used to interpret the measurement data as well as more details of the experiment and its analysis. The theory reported here is a tool for the investigation of different dynamical situations in time-dependent harmonic traps.

Demagnetization cooling of a gas

Adiabatic demagnetization is an efficient technique for cooling solid samples by several orders of magnitude in a single cooling step. In gases, the required coupling between dipolar moments and motion is typically too weak, but in dipolar gases—of high-spin atoms or heteronuclear molecules with strong electric dipole moments, for example—the method should be applicable. Here, we demonstrate demagnetization cooling of a gas of ultracold 52Cr atoms. Demagnetization is driven by inelastic dipolar collisions, which couple the motional degrees of freedom to the spin degree. In this way, kinetic energy is converted into magnetic work, with a consequent temperature reduction of the gas. Optical pumping is used to magnetize the system and drive continuous demagnetization cooling. We can increase the phase-space density of our sample by up to one order of magnitude, with almost no atom loss, suggesting that the method could be used to achieve quantum degeneracy via optical means.

Continuous loading of a conservative potential trap from an atomic beam.

We demonstrate the fast accumulation of 52Cr atoms in a conservative potential from a guided atomic beam. Without laser cooling on a cycling transition, a dissipative step involving optical pumping allows us to load atoms at a rate of 2×10(7)  s(-1) in the trap. Within less than 100 ms we reach the collisionally dense regime, from which we produce a Bose-Einstein condensate with subsequent evaporative cooling. This constitutes a new approach to degeneracy where Bose-Einstein condensation can be reached without a closed cycling transition, provided that a slow beam of particles can be produced.