B. Bartenlian

Nanoscale Magnetic Domains in Mesoscopic Magnets

The basic magnetic properties of three-dimensional nanostructured materials can be drastically different from those of a continuous film. High-resolution magnetic force microscopy studies of magnetic submicrometer-sized cobalt dots with geometrical dimensions comparable to the width of magnetic domains reveal a variety of intricate domain patterns controlled by the details of the dot geometry. By changing the thickness of the dots, the width of the geometrically constrained magnetic domains can be tuned. Concentric rings and spirals with vortex configurations have been stabilized, with particular incidence in the magnetization reversal process as observed in the ensemble-averaged hysteresis loops.

Two-chamber AFM: probing membrane proteins separating two aqueous compartments

Biological membranes compartmentalize and define physical borders of cells. They are crowded with membrane proteins that fulfill diverse crucial functions. About one-third of all genes in organisms code for, and the majority of drugs target, membrane proteins. To combine structure and function analysis of membrane proteins, we designed a two-chamber atomic force microscopy (AFM) setup that allows investigation of membranes spanned over nanowells, therefore separating two aqueous chambers. We imaged nonsupported surface layers (S layers) of Corynebacterium glutamicum at sufficient resolution to delineate a 15 Å–wide protein pore. We probed the elastic and yield moduli of nonsupported membranes, giving access to the lateral interaction energy between proteins. We combined AFM and fluorescence microscopy to demonstrate the functionality of proteins in the setup by documenting proton pumping by Halobacterium salinarium purple membranes.

Spin-wave quantization and dynamic coupling in micron-size circular magnetic dots

We report on the observation of spin-wave quantization in square arrays of micron-size circular magnetic Ni80Fe20 dots by means of Brillouin light-scattering spectroscopy. For a large wave-vector interval several discrete, dispersionless modes with a frequency splitting of up to 2.5 GHz were observed. The modes are identified as magnetostatic surface spin waves laterally quantized due to in-plane confinement in each single dot. The frequencies of the lowest observed modes decrease with increasing distance between the dots, thus indicating an essential dynamic magnetic dipole interaction between the dots at small interdot distances.

Soft UV nanoimprint lithography-designed highly sensitive substrates for SERS detection

AbstractWe report on the use of soft UV nanoimprint lithography (UV-NIL) for the development of reproducible, millimeter-sized, and sensitive substrates for SERS detection. The used geometry for plasmonic nanostructures is the cylinder. Gold nanocylinders (GNCs) showed to be very sensitive and specific sensing surfaces. Indeed, we demonstrated that less than 4 ×106 avidin molecules were detected and contributed to the surface-enhanced Raman scattering (SERS) signal. Thus, the soft UV-NIL technique allows to obtain quickly very sensitive substrates for SERS biosensing on surfaces of 1 mm 2.

Brillouin light scattering investigations of structured permalloy films

The static and spin wave properties of regular square lattices of magnetic dots of 0.5–2 μm dot diameter and 1–4 μm periodicity patterned in permalloy films have been investigated by Brillouin light scattering. The samples have been structured using x-ray lithography and ion beam etching. The Brillouin light scattering spectra reveal both surface and bulk spin wave modes. The spin wave frequencies can be well described taking into account the demagnetization factor of each single dot. For the samples with smallest dot separation of 0.1 μm a fourfold in-plane magnetic anisotropy with the easy axis directed along the pattern diagonal is observed, indicating anisotropic coupling between the dots.

MAGNETIZATION REVERSAL IN PATTERNED CO(0001) ULTRATHIN FILMS WITH PERPENDICULAR MAGNETIC ANISOTROPY

Using x‐ray lithography we have patterned dot arrays in Au/Co/Au(111) sandwiches based on ultrathin Co layers with perpendicular anisotropy. Large area arrays of dots with diameters of 1 and 2 μm have been obtained, keeping mostly undamaged the ultrathin Co layer. Hysteresis loops of the arrays depend drastically on the dot diameter. Magneto‐optical domain visualization experiments confirm a magnetization reversal mechanism based on a large distribution of nucleation fields in the film, with complete reversal of the magnetization of one dot through the domain wall propagation after a local nucleation process. This could give information on the magnetization reversal processes in Au/Co/Au(111) continuous films.

Spin wave quantization in laterally confined magnetic structures (invited)

An overview of the current status of the study of spin wave excitations in arrays of magnetic dots and wires is given. We describe both the status of theory and recent inelastic light scattering experiments addressing the most important issues; the quantization of localized spin waves due to the in-plane confinement of spin waves in elements, dipolar coupling between the quantized modes, and the localization of the modes within rectangular elements due to an inhomogeneous demagnetizing field.

Light diffraction effects in the magneto-optical properties of 2D arrays of magnetic dots of Au/Co/Au(111) films with perpendicular magnetic anisotropy

Using X-ray lithography and ion beam etching we have patterned micrometer-sized square lattices of round dots, out of Au/Co/Au(111) films with perpendicular easy magnetization axes. The magneto-optical Kerr rotation shows strong variations versus the diffraction order, the light polarization direction and the ratio of film to background reflectance, particularly when the lattice spacing is high compared with the dot size. This reveals an important interplay between diffraction and magneto-optics.

Integration of short gold nanoparticles chain on SOI waveguide toward compact integrated bio-sensors

We demonstrate the integration of short metal nanoparticle chains (L ≈700 nm) supporting localized surface plasmons in Silicon On Insulator (SOI) waveguides at telecom wavelengths. Nanoparticles are deposited on the waveguide top and excited through the evanescent field of the TE waveguide modes. Finite difference time domain calculations and waveguide transmission measurements reveal that almost all the TE mode energy can be transferred to nanoparticle chains at resonance. It is also shown that the transmission spectrum is very sensitive to the molecular environment of nanoparticles, thus opening the way towards ultra-compact sensors in guided plasmonics on SOI. An experimental demonstration is reported with octadecanthiol molecules for a detection volume as small as 0.26 attoliter.

Inverse giant magnetoresistance (invited)

Inverse giant magnetoresistance (GMR) is obtained in multilayers alternating two ferromagnetic layers F1 and F2 with different asymmetry of spin scattering, α1≳1 and α2<1. This is clearly demonstrated in the simple spin‐valve system with perpendicular magnetization Fe1−xVx/Au/Co. With respect to Fe, the FeV alloys with x=0.18 and 0.29 exhibit an inversion of the spin scattering coefficients (αFe≳1, αFeV<1) due to the change of the densities of states at the Fermi level. The inverse MR of FeV/Au/Co is studied as a function of FeV layer thickness and temperature and compared to calculations based on the Camley–Barnas model. The data show that the inverse GMR is due to the bulk scattering within the FeV layer, which coexists with a substantial interface scattering favoring normal GMR.