B. Marczewska

Photoluminescence of gamma-, proton- and alpha-irradiated LiF detectors

Lithium fluoride (LiF), one of the most pervasive alkali halides in optical device research, is routinely used in optical data storage and radiation protection. LiF crystals may contain different aggregate defects produced by several types of ionizing radiation, with the number of defects being proportional to the cumulative radiation dose. Stimulation of irradiated LiF detectors by heating or with blue light causes thermoluminescence (TL) or photoluminescence (PL), respectively. We developed a new PL reader equipped with a blue light-emitting diode for stimulation and a Hamamatsu photomultiplier for registering green emissions, dedicated to examining LiF detectors as well as more broadly investigating TL/PL emission from standard LiF detectors irradiated with gamma rays, 60 MeV protons and alpha particles. The results confirmed very high efficiency PL signal from alpha-irradiated LiF detectors corresponding to their low efficiency after gamma irradiation, and vice versa for TL readout. Combining the TL and PL readouts permits us to discriminate between how different kinds of radiation affect efficiency in LiF detectors.

LITHIUM FLUORIDE CRYSTALS AS FLUORESCENT NUCLEAR TRACK DETECTORS

Radiophotoluminescence signal of LiF crystals was found to be sufficiently strong to visualize tracks of a single charged particle. This was achieved with a wide-field fluorescent microscope equipped with a ×100 objective and LiF single crystals grown with the Czochralski method at IFJ PAN. The tracks of alpha particles, protons, as well as products of 6Li(n,α)3H reaction with thermal neutrons (moderated Pu/Be source), were observed. These encouraging results are the first steps towards practical use of LiF as fluorescent nuclear track detectors. The most promising dosimetric application seems to be neutron measurements.

IMAGING OF PROTON BRAGG PEAKS IN LiF

Lithium fluoride (LiF) is one of the most common thermoluminescent phosphors routinely used in radiation protection services. Another advantageous property of LiF is radiophotoluminescence, whose occurs after its irradiation due to the creation of color centers. Excitation of LiF samples with a blue light causes the emission of photoluminescence, which spectrum consists of two peaks at ~520 and ~670 nm. The work was focused on imaging of Bragg peaks of proton beams routinely applied at the proton eye radiotherapy facility operating at the Institute of Nuclear Physics Polish Academy of Sciences (IFJ PAN) in Krakow by the measurement of the fluorescence light in LiF crystals excited with a 445 nm blue light after their previous irradiation with the proton beams of energies of 28, 30, 40 and 50 MeV. The range of proton beams in LiF crystals for different energies was calculated by Monte Carlo simulations.

Optical and thermal pre-readout treatments to reduce the influence of fading on LiMgPO4 OSL measurements

TL (Thermoluminescent) and OSL (Optically Stimulated Luminescence) techniques are both luminescent techniques widely applied in several areas into radiation dosimetry. The main difference between them are related to the employed stimulus (thermal or optical) for luminescent emission, as well as the advantages of each technique. Due to simplicity and not to be required heating, the OSL technique has been continuously improved and new researches in materials to be used with this technique have grown in the last decades. Nowadays the main problems in the application of the developed new materials are the poor stability and loss of OSL signal over time (fading). In this study, we performed a sequence of thermal (preheat) and optical (OSL with infra-red light stimulus) pre-readout treatments immediately before OSL readouts of LiMgPO4 based detectors (LMP), aiming the applicability of novel materials, contributing to find solutions to minimize the influence of fading. Moreover, it was demonstrated that the influence of fading is minimized and the stability of OSL signal from LMP is achieved using just optical process, without heating the material.

OSL dosimetric properties and efficiency of Brazilian natural calcium fluoride pellets

Calcium fluoride (CaF2), in both natural and synthetic forms, has been exhaustively studied and explored as thermoluminescent (TL) detector. However its sensitivity to ambient light points to the applicability of CaF2 as OSL (Optically Stimulated Luminescence) detector, increasing the research about its luminescent properties. Although some properties to employ CaF2 detectors with OSL technique have been already demonstrated, there is a lack of some essential information as the OSL response to different types and energy of ionizing radiation. In order to extend the use of Brazilian natural CaF2 with OSL technique, we evaluated the efficiency and dosimetric properties of cold pressed CaF2:NaCl pellets. The CaF2 detectors presented good reproducibility and negligible fading of the signal over one month after irradiation. The dose response using OSL, TL and residual TL showed linear behavior for different radiation beams (protons, photons and alpha and beta particles), being equivalent to the results obtained with BeO and MTS (LiF) detectors through OSL and TL technique respectively. Moreover, differences were observed in OSL efficiency according the beam type and energy; CaF2 detectors presented a higher OSL and TL sensitivities to protons, photons and beta particles than to alpha particles. The energy response to photons obtained using OSL and residual TL intensities present an over response at lower photon energy similar to TL energy response. In addition, differences in the OSL curve shapes were observed according to radiation type and energy, pointing to the possibility of applying this material in mixed radiation fields and to estimate average LET (Linear Energy Transfer).

OSL properties of lithium aluminate crystals grown with Micro-Pulling-Down technique

Selected optically stimulated luminescence properties of lithium aluminate crystals are presented within this work. Crystals were grown using Micro-Pulling-Down technique. The growth parameters and XRD analysis of obtained samples are demonstrated. OSL decay curves, thermal stability and fading of samples prepared under different conditions are compared.

TL and OSL properties of LiMgPO 4 :Tb,B

LiMgPO4 (LMP) phosphor is a new highly sensitive material for TL and OSL dosimetry. The objective of the work was to investigate the dosimetric properties of this material. LMP phosphor doped with Tb and B was irradiated with beta rays and alpha particles. Thermoluminescence (TL) and optically stimulated luminescence (OSL) measurements were performed for LMP powders in comparison with Al2O3:C detector (Landauer). The phosphate which was made in our laboratory exhibits a main TL peak at 150°C. The synthesized LiMgPO4:Tb,B is a highly sensitive OSL material for dosimetric applications.