Ben De Clercq

Plasmons reveal the direction of magnetization in nickel nanostructures.

We have applied the surface-sensitive nonlinear optical technique of magnetization-induced second harmonic generation (MSHG) to plasmonic, magnetic nanostructures made of Ni. We show that surface plasmon contributions to the MSHG signal can reveal the direction of the magnetization. Both the plasmonic and the magnetic nonlinear optical responses can be tuned; our results indicate novel ways to combine nanophotonics, nanoelectronics, and nanomagnetics and suggest the possibility for large magneto-chiral effects in metamaterials.

Plasmon-Enhanced Sub-Wavelength Laser Ablation: Plasmonic Nanojets

In response to the incident lights electric field, the electron density oscillates in the plasmonic hotspots producing an electric current. Associated Ohmic losses raise the temperature of the material within the plasmonic hotspot above the melting point. A nanojet and nanosphere ejection can then be observed precisely from the plasmonic hotspots.

U-Shaped Switches for Optical Information Processing at the Nanoscale

4–6 ] In such devices, light waves would be used instead of electrons. The possibility arises from the fact that light waves can couple to collective excitations of electrons at the surfaces of metallic nanostructures, a prop-erty referred to as surface plasmon resonance. Because these optically induced resonances occur at the surfaces and interfaces of the nanostructures, they can readily be investigated with a surface- and interface-specifi c optical technique, such as second-harmonic generation (SHG). SHG is a nonlinear optical technique that, within the dipole approximation, is forbidden in materials with a center of symmetry. Consequently, SHG is highly sensitive to regions with broken symmetry, such as surfaces (or interfaces), and it has been successfully applied to the study of plasmonic nano-materials with different geometries.

The role of chiral local field enhancements below the resolution limit of Second Harmonic Generation microscopy

While it has been demonstrated that, above its resolution limit, Second Harmonic Generation (SHG) microscopy can map chiral local field enhancements, below that limit, structural defects were found to play a major role. Here we show that, even below the resolution limit, the contributions from chiral local field enhancements to the SHG signal can dominate over those by structural defects. We report highly homogeneous SHG micrographs of star-shaped gold nanostructures, where the SHG circular dichroism effect is clearly visible from virtually every single nanostructure. Most likely, size and geometry determine the dominant contributions to the SHG signal in nanostructured systems.

Diffusion of myelin oligodendrocyte glycoprotein in living OLN-93 Cells investigated by raster-scanning image correlation spectroscopy (RICS)

Many membrane proteins and lipids are partially confined in substructures ranging from tens of nanometers to micrometers in size. Evidence for heterogeneities in the membrane of oligodendrocytes, i.e. the myelin-producing cells of the central nervous system, is almost exclusively based on detergent methods. However, as application of detergents can alter the membrane phase behaviour, it is important to investigate membrane heterogeneities in living cells. Here, we report on the first investigations of the diffusion behavior of the myelin-specific protein MOG (myelin oligodendrocyte glycoprotein) in OLN-93 as studied by the recently developed RICS (raster-scanning image correlation spectroscopy) technique. We implemented RICS on a standard confocal laser-scanning microscope with one-photon excitation and analog detection. Measurements on FITC-dextran were used to evaluate the performance of the system and the data analysis procedure.

Second harmonic hotspots at the edges of the unit cells in G-shaped gold nanostructures

We report our latest results on second harmonic generation (SHG) microscopy from arrays of G-shaped chiral gold nanostructures. The nanostructures are arranged in unit cells composed of four Gs, each rotated at 90° with respect to its neighbors. As it has already been demonstrated, for linearly polarized light, these unit cells yield a pattern of four SHG hotspots. However, upon increasing the pitch of the nanostructured arrays, extra hotspots can be observed at the edges of the unit cells. While the origin of these extra hotspots remains to be elucidated, their position indicates a relationship to coupling behavior between the unit cells.