Benjamin A. Lindley

On the Use of Reduced-Moderation LWRs for Transuranic Isotope Burning in Thorium Fuel—I: Assembly Analysis

Multiple recycle of transuranic (TRU) isotopes in thermal reactors results in degradation of the plutonium (Pu) fissile quality with buildup of higher actinides (e.g., Am, Cm, Cf), some of which are thermal absorbers. These phenomena lead to increasing amounts of Pu feed being required to sustain criticality and accordingly larger TRU content in the multirecycled fuel inventory, ultimately resulting in a positive moderator temperature coefficient (MTC) and void reactivity coefficient. Because of the favorable impact fostered by use of thorium (Th) on these coefficients, the feasibility of Th-TRU multiple recycle in reduced-moderation pressurized water reactors (PWRs) and boiling water reactors (BWRs) has been investigated. In this paper, Part I of two companion papers, the analysis is limited to a single assembly, with full-core models presented in Part II. Spatial separation of TRU from bred uranium is found to greatly improve neutronic performance. A large reduction in moderation is necessary to allow full actinide recycle. This will pose thermal-hydraulic challenges, which are discussed in Part II. In addition, the harder neutron spectrum resulting from the reduced moderation also reduces the control rod worth, while there is a neutronic incentive to use increased mechanical shim to maintain a negative MTC. It may therefore be desirable to increase the number of rod cluster control assemblies. Superior burnup is achievable in a reduced-moderation BWR as a larger reduction in moderation is feasible, although the incineration rate is reduced relative to a PWR due to a higher conversion ratio.

Transmutation of thermocouples in thermal and fast nuclear reactors

Thermocouples are the most commonly used sensors for temperature measurement in nuclear reactors. Their role is fundamental for the control of current nuclear reactors and for the development of the nuclear technology needed for the implementation of GEN IV nuclear reactors. When used for in-core measurements thermocouples are strongly affected not only by high temperatures, but also by intense neutron fluxes. As a result of the interaction with neutrons, the thermoelements of the thermocouples undergo transmutation, which produces a time dependent change in composition in the thermoelements and, as a consequence, a time dependent drift in the thermocouple signal. Thermocouple drift can be very significant for in-pile temperature measurements and may render the temperature sensors unreliable after exposure to nuclear radiation for relatively short times compared to the life required for temperature sensors in nuclear applications. In this work, undertaken as part of the European project METROFISSION, the change in composition occurring in irradiated thermocouples has been calculated using the software ORIGEN 2.2. Several thermocouples have been considered, including Nickel based thermocouples (type K and type N), Tungsten based thermocouples (W-5%Re vs W-26%Re and W3%Re vs W-25%Re), Platinum based thermocouples (type S and Platinum vs Palladium) and Molybdenum vs Niobium thermocouples. The transmutation induced by both thermal flux and fast flux has been calculated. Thermocouples undergo more pronounced transmutation in thermal fluxes rather than in fast fluxes, as the neutron cross section of an element is higher for thermal energies. Nickel based thermocouples have a minimal change in composition, while Platinum based and Tungsten based thermocouples experience a very significant transmutation. The use of coatings deposited on the sheath of a thermocouple has been considered as a mean to reduce the neutron flux the thermoelements inside the thermocouple sheath are subject to. Boron containing coatings have been chosen as potential candidates. The effect of the coatings on the neutron flux affecting the thermoelements has been calculated using the software WIMS. The results for both thermal and fast reactors are reported in this paper.

Analysis of advanced PWR loading schemes for transuranic incineration in thorium

It is difficult to perform multiple recycle of transuranic (TRU) isotopes in PWRs as the moderator temperature coefficient (MTC) tends to become positive after a few recycles and the core may have positive reactivity when fully voided. Due to the favorable impact on the MTC and void coefficient fostered by use of thorium (Th), the possibility of performing Th-TRU multiple-recycle in reduced-moderation PWRs (RMPWRs) is under consideration. The simplest way to reduce the moderation in a PWR is to increase the fuel pin diameter. This configuration improves the trade-off between achievable burn-up and MTC, but is ultimately limited by thermal-hydraulic constraints. Heterogeneous recycle with the bred uranium (U3) and the TRU are arranged in separate pins was found to be neutronically preferable to a homogeneous configuration. Spatial separation also enables the U3 and TRU to be refueled on different batch schemes. These techniques allow satisfactory discharge burn-up while ensuring negative MTC and fully voided reactivity, with the pin diameter of a standard PWR increased from 9.5 mm to 11 mm. Reactivity control is a key challenge due to the reduced worth of neutron absorbers and their detrimental effect on the void coefficients, especially when diluted, as is the case for soluble boron. It seems necessary to control the core using control rods to keep the fully voided reactivity negative. A preliminary analysis indicates that this is feasible.Copyright

Nuclear data libraries assessment for modelling a small fluoride salt-cooled, high-temperature reactor

Nuclear data consists of measured or evaluated probabilities of various fundamental physical interactions involving the nuclei of atoms and their properties. Most fluoride salt-cooled high-temperature reactor (FHR) studies that were reviewed do not give detailed information on the data libraries used in their assessments. Therefore, the main objective of this data libraries comparison study is to investigate whether there are any significant discrepancies between main data libraries, namely ENDF/B-VII, JEFF-3.1 and JEF-2.2. Knowing the discrepancies, especially its magnitude, is important and relevant for readers as to whether further cautions are necessary for any future verification or validation processes when modelling an FHR. The study is performed using AMEC’s reactor physics software tool, WIMS. The WIMS calculation is simply a 2-D infinite lattice of fuel assembly calculation. The comparison between the data libraries in terms of infinite multiplication factor, kinf and pin power map are presented...