C. Grivas

Nanodroplets deposited in microarrays by femtosecond Ti:sapphire laser-induced forward transfer

The authors present the deposition of nanoscale droplets of Cr using femtosecond Ti:sapphire laser-induced forward transfer. Deposits around 300nm in diameter, significantly smaller than any previously reported, are obtained from a 30nm thick source film. Deposit size, morphology, and adhesion to a receiver substrate as functions of applied laser fluence are investigated. The authors show that deposits can be obtained from previously irradiated areas of the source material film with negligible loss of deposition quality, allowing subspot size period microarrays to be produced without the need to move the source film.

Single-mode tunable laser emission in the single-exciton regime from colloidal nanocrystals

Whispering-gallery-mode resonators have been extensively used in conjunction with different materials for the development of a variety of photonic devices. Among the latter, hybrid structures, consisting of dielectric microspheres and colloidal core/shell semiconductor nanocrystals as gain media, have attracted interest for the development of microlasers and studies of cavity quantum electrodynamic effects. Here we demonstrate single-exciton, single-mode, spectrally tuned lasing from ensembles of optical antenna-designed, colloidal core/shell CdSe/CdS quantum rods deposited on silica microspheres. We obtain single-exciton emission by capitalizing on the band structure of the specific core/shell architecture that strongly localizes holes in the core, and the two-dimensional quantum confinement of electrons across the elongated shell. This creates a type-II conduction band alignment driven by coulombic repulsion that eliminates non-radiative multi-exciton Auger recombination processes, thereby inducing a large exciton–bi-exciton energy shift. Their ultra-low thresholds and single-mode, single-exciton emission make these hybrid lasers appealing for various applications, including quantum information processing.

Micro-channels machined in microstructured optical fibers by femtosecond laser

Micro-channels were fabricated in hollow-core photonic bandgap fiber (HC-PBGF) and suspended-core holey fiber (SC-HF) by femtosecond Ti:sapphire laser irradiation. Gaseous access was demonstrated via these engineered ports to the core of HC-PBGF and the hollow cladding of SC-HF. Femtosecond laser micro-machining caused no additional transmission loss in HC-PBGFs. This allowed a novel gas cell to be produced, in which gaseous access was provided solely through two micro-channels. Acetylene diffusion was also confirmed through a micro-channel leading to a single cladding airhole in SC-HF. This further highlighted the fabrication techniques precision, selectivity, and potential for developing fiber-based micro-fluidic devices.

TI:SAPPHIRE PLANAR WAVEGUIDE LASER GROWN BY PULSED LASER DEPOSITION

We document the lasing performance of a waveguiding layer of Ti:sapphire, of ~12-mum thickness, grown by pulsed laser deposition from a 0.12-wt.% Ti(2)O(3) Ti:sapphire single-crystal target onto an undoped z-cut sapphire substrate. Lasing around 800 nm is observed when the waveguide layer is pumped by an argon-ion laser running on all-blue-green lines, with an absorbed power threshold of 0.56 W, with high-reflectivity (R>98%) mirrors. With a 5% pump duty cycle and a T=35% output coupler, a slope efficiency of 26% with respect to absorbed power is obtained, giving quasi-cw output powers in excess of 350 mW.

Growth of Ti:sapphire single crystal thin films by pulsed laser deposition

This paper documents the growth of single crystal Ti:sapphire thin films, typically 10µm thick, on undoped sapphire substrates using Pulsed Laser Deposition from a Ti:sapphire single crystal target with a doping level of 0.1 % wt Ti2O3. These thin films are shown to have very high crystal quality using Ion Beam Channelling and X-Ray Diffraction Techniques. The degree of titanium incorporation into the films is investigated using Inductively Coupled Plasma Mass Spectrometry and Particle Induced X-ray Emission. These techniques show that levels of up to 0.08% wt Ti2O3 are present in the deposited layers.

Shadowgraphic studies of triazene assisted laser-induced forward transfer of ceramic thin films

The laser-induced forward transfer process of solid ceramic donor materials (gadolinium gallium oxide and ytterbium doped yttrium aluminium oxide) was studied using triazene polymer as a sacrificial layer by means of a time-resolved nanosecond-shadowgraphy technique. The dependence of the ablation dynamics and quality of the ejected donor material on the laser fluence and thickness of the sacrificial and donor layers were investigated and discussed.

Performance of Ar/sup +/-milled Ti:sapphire rib waveguides as single transverse-mode broadband fluorescence sources

Rib waveguides have been fabricated in pulsed-laser-deposited Ti:sapphire layers using photolithographic patterning and subsequent Ar/sup +/-beam milling. Fluorescence output powers up to 300 /spl mu/W have been observed from the ribs following excitation by a 3-W multiline argon laser. Mode intensity profiles show high optical confinement and the measured beam propagation factors M/sub x//sup 2/ and M/sub y//sup 2/ of 1.12 and 1.16, respectively, indicate single transverse-mode fluorescence emission. Loss measurements using the self-pumped phase conjugation technique have yielded comparable values (1.7 dB/cm) for the ribs and the unstructured planar waveguide counterparts. The combination of optimum modal properties and strong optical confinement, together with sufficient levels of fluorescence output, make the single-moded Ti:sapphire rib waveguides a very interesting candidate as a fluorescence source for optical coherence tomography applications.

Performance of a low loss pulsed laser deposited Nd:Gd3Ga5O12 waveguide laser at 1.06µm and 0.94µm

We report the laser performance of a low-propagation-loss neodymium-doped Gd(3)Ga(5)O(12) (Nd:GGG) waveguide fabricated by pulsed-laser deposition. An 8- mum -thick crystalline Nd:GGG film grown upon an undoped Y(3)Al(5)O(12) substrate lases at 1.060 and 1.062 microm when pumped by a Ti:sapphire laser operating at 740 or 808nm.Using a 2.2% output coupler, we observed a 1060-nm laser threshold of 4mW and a slope efficiency of 20%. Laser action was also achieved, for what we believe is the first time in Nd:GGG, on the quasi-three-level 937-nm transition. With a 2% output coupler at this wavelength a laser threshold of 17mW and a 20% slope efficiency were obtained. This demonstration of low propagation loss combined with the fact that these waveguides have a very high numerical aperture (0.75) makes pulsed-laser-deposited thin films attractive for high-power diode-pumped devices.

Microstructured KY(WO4)2:Gd3+, Lu3+, Yb3+ channel waveguide laser

Epitaxially grown, 2.4-microm-thin layers of KY(WO(4))(2):Gd(3+), Lu(3+), Yb(3+), which exhibit a high refractive index contrast with respect to the undoped KY(WO(4))(2) substrate, have been microstructured by Ar beam milling, providing 1.4-microm-deep ridge channel waveguides of 2 to 7 microm width, and overgrown by an undoped KY(WO(4))(2) layer. Channel waveguide laser operation was achieved with a launched pump power threshold of only 5 mW, a slope efficiency of 62% versus launched pump power, and 76 mW output power.

Tunable, continuous-wave Ti:sapphire channel waveguide lasers written by femtosecond and picosecond laser pulses

Fabrication and cw lasing at 798.25 nm is reported for femtosecond (fs) and picosecond (ps) laser-inscribed channel waveguides in Ti:sapphire crystals. Lasing in channels written by fs (ps) pulses was obtained above a threshold of 84 mW (189 mW) with a maximum output power and a slope efficiency of 143 mW (45 mW) and 23.5% (7.1%), respectively. The emission wavelength was tuned over a 170 nm range by using a birefringent filter in an external cavity.