C. Lemell

Direct measurement and analysis of the carrier-envelope phase in light pulses approaching the single-cycle regime

We demonstrate a solid-state device capable of providing direct information about the carrier-envelope (CE) phase of ultrashort (4 fs) laser pulses. The measurement is based on multi-photon-induced photoelectron emission from a gold surface. The amount of the charge emitted from the surface gives a clear indication of phase sensitivity, as predicted by our simulations and also by a simple intuitive model. This phenomenon was used to determine the CE phase value of each laser pulse in a mode-locked, unamplified, low-energy pulse train. The inability of the commonly used f -to-2f interferometric method to measure accurately extracavity drifts of the CE phase is discussed and contrasted with the direct phase measurement method proposed here. The evolution of the CE phase upon propagation of pulses comparable in duration to the optical cycle is analysed.

Electron rescattering at metal nanotips induced by ultrashort laser pulses

We report on the first investigation of plateau and cut-off structures in photoelectron spectra from nano-scale metal tips interacting with few-cycle near-infrared laser pulses. These hallmarks of electron rescattering, well-known from atom-laser interaction in the strong-field regime, appear at remarkably low laser intensities with nominal Keldysh parameters of the order of

Electron guiding through insulating nanocapillaries

\gtrsim 10

Simulation of attosecond streaking of electrons emitted from a tungsten surface

. Quantum and quasi-classical simulations reveal that a large field enhancement near the tip and the increased backscattering probability at a solid-state target play a key role. Plateau electrons are by an order of magnitude more abundant than in comparable atomic spectra, reflecting the high density of target atoms at the surface. The position of the cut-off serves as an in-situ probe for the locally enhanced electric field at the tip apex.

Interaction of ultrashort laser pulses with metal nanotips: a model system for strong-field phenomena

We simulate the electron transmission through insulating Mylar (polyethylene terephthalate, or PET) capillaries. We show that the mechanisms underlying the recently discovered electron guiding are fundamentally different from those for ion guiding. Quantum reflection and multiple near-forward scattering rather than the self-organized charge up are key to the transmission along the capillary axis irrespective of the angle of incidence. We find surprisingly good agreement with recent data. Our simulation suggests that electron guiding should also be observable for metallic capillaries.

Ab initio simulation of electrical currents induced by ultrafast laser excitation of dielectric materials.

First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an extended ultraviolet pump pulse and probed by a few-cycle near-infrared pulse found a time delay of about 100 as between photoelectrons from the conduction band and those from the

Phase diagram for nanostructuring CaF(2) surfaces by slow highly charged ions.

4f

Large optical field enhancement for nanotips with large opening angles

core level of tungsten. We present a microscopic simulation of the emission time and energy spectra employing a classical transport theory. Emission spectra and streaking images are well reproduced. Different contributions to the delayed emission of core electrons are identified: larger emission depth, slowing down by inelastic-scattering processes, and possibly, energy-dependent deviations from the free-electron dispersion. We find delay times near the lower bound of the experimental data.

Transmission of highly charged ions through microcapillaries

We discuss the interaction of ultrashort near-infrared laser pulses with sharp metal tips at moderate nominal intensities (I0 10 11 Wcm 2 ). As external electric fields are strongly enhanced at such tips (enhancement factor 10) our system turns out to be an ideal miniature laboratory to investigate strong-field effects at solid surfaces. We analyse the electron-energy spectra as a function of the strength of the laser field and the static extraction field and present an intuitive model for their interpretation. The size of the effective field acting on the metal electrons can be determined from the electron spectra. The latter are also reproduced by time-dependent density functional theory (TDDFT) simulations.

Ab initio multiscale simulation of high-order harmonic generation in solids

We theoretically investigate the generation of ultrafast currents in insulators induced by strong few-cycle laser pulses. Ab initio simulations based on time-dependent density functional theory give insight into the atomic-scale properties of the induced current signifying a femtosecond-scale insulator-metal transition. We observe the transition from nonlinear polarization currents during the laser pulse at low intensities to tunnelinglike excitation into the conduction band at higher laser intensities. At high intensities, the current persists after the conclusion of the laser pulse considered to be the precursor of the dielectric breakdown on the femtosecond scale. We show that the transferred charge sensitively depends on the orientation of the polarization axis relative to the crystal axis, suggesting that the induced charge separation reflects the anisotropic electronic structure. We find good agreement with very recent experimental data on the intensity and carrier-envelope phase dependence [A. Schiffrin et al., Nature (London) 493, 70 (2013).