C. M. Morris

A sudden collapse in the transport lifetime across the topological phase transition in (Bi1-xInx)2Se3

The quantum phase transition from a topological to a conventional insulator in In-doped Bi2Se3 occurs when the topological phase is destroyed by the hybridization of states on opposite surfaces. This is characterized by a sudden change in the transport lifetime, measured by means of optical spectroscopy.

Polarization modulation time-domain terahertz polarimetry

We present high precision measurements of polarization rotations in the frequency range from 0.1 to 2.5 THz using a polarization modulation technique. A motorized stage rotates a polarizer at ~ 80 Hz, and the resulting modulation of the polarization is measured by a lock-in technique. We achieve an accuracy of 0.050° (900 μrad) and a precision of 0.02° (350 μrad) for small rotation angles. A detailed mathematical description of the technique is presented, showing its ability to fully characterize elliptical polarizations from 0.1 to 2.5 THz.

High-Resolution Faraday Rotation and Electron-Phonon Coupling in Surface States of the Bulk-Insulating Topological Insulator Cu_{0.02}Bi_{2}Se_{3}.

We have utilized time-domain magnetoterahertz spectroscopy to investigate the low-frequency optical response of the topological insulator Cu_{0.02}Bi_{2}Se_{3} and Bi_{2}Se_{3} films. With both field and frequency dependence, such experiments give sufficient information to measure the mobility and carrier density of multiple conduction channels simultaneously. We observe sharp cyclotron resonances (CRs) in both materials. The small amount of Cu incorporated into the Cu_{0.02}Bi_{2}Se_{3} induces a true bulk insulator with only a single type of conduction with a total sheet carrier density of ~4.9×10^{12}/cm^{2} and mobility as high as 4000 cm^{2}/V·s. This is consistent with conduction from two virtually identical topological surface states (TSSs) on the top and bottom of the film with a chemical potential ~145 meV above the Dirac point and in the bulk gap. The CR broadens at high fields, an effect that we attribute to an electron-phonon interaction. This assignment is supported by an extended Drude model analysis of the zero-field Drude conductance. In contrast, in normal Bi_{2}Se_{3} films, two conduction channels were observed, and we developed a self-consistent analysis method to distinguish the dominant TSSs and coexisting trivial bulk or two-dimensional electron gas states. Our high-resolution Faraday rotation spectroscopy on Cu_{0.02}Bi_{2}Se_{3} paves the way for the observation of quantized Faraday rotation under experimentally achievable conditions to push the chemical potential in the lowest Landau level.

A hierarchy of bound states in the 1D ferromagnetic Ising chain CoNb

Kink bound states in the one-dimensional ferromagnetic Ising chain compound CoNb2O6 have been studied using high-resolution time-domain terahertz spectroscopy in zero applied magnetic field. When magnetic order develops at low temperature, nine bound states of kinks become visible. Their energies can be modeled exceedingly well by the Airy function solutions to a 1D Schrödinger equation with a linear confining potential. This sequence of bound states terminates at a threshold energy near 2 times the energy of the lowest bound state. Above this energy scale we observe a broad feature consistent with the onset of the two particle continuum. At energies just below this threshold we observe a prominent excitation that we interpret as a novel bound state of bound states--two pairs of kinks on neighboring chains.

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Abstract Recent experiments have uncovered evidence of low energy excitations in the bulk of SmB 6 that are perhaps associated with unconventional quasiparticles, bringing into question whether this Kondo “insulator” is truly insulating in the bulk. Recently, we demonstrated that SmB 6 possesses significant in-gap bulk ac conduction far in excess of typical disordered semiconductors. Whether such conduction is an intrinsic feature of SmB 6 , suggesting the formation of an exotic state, or residual conduction from impurities continues to be a topic of debate. Here, we further examine the origin of the ac optical conductivity of SmB 6 in light of recent experimental and theoretical developments. The optical conductivity of SmB 6 is shown to possess distinct regimes of either dominant free carrier or localized response contributions. The free carrier response is found to be in good qualitative agreement with previous literature, although quantitative differences are revealed and discussed. The localized response, which dominates at the lowest temperatures, is analyzed in the context of models of either in-gap impurity states or an exotic neutral Fermi surface. The charge density or effective mass of this low temperature in-gap conductivity is extracted through a conductivity sum rule analysis and found to be in general alignment with both models in the appropriate limits. Our results shed further light on the nature of the in-gap states of SmB 6 .

O

Standard time-domain THz spectroscopy (TDTS) in a transmission geometry was performed with a custom home-built THz spectrometer. In this technique an approximately single-cycle picosecond pulse of light is transmitted through the sample and the substrate. The complex transmission is obtained from Fourier transforming the time-domain sample pulse and ratioing it to a Fourier transformed substrate pulse.

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Kink bound states in the one-dimensional ferromagnetic Ising chain compound CoNb2O6 have been studied using high-resolution time-domain terahertz spectroscopy in zero applied magnetic field. When magnetic order develops at low temperature, nine bound states of kinks become visible. Their energies can be modeled exceedingly well by the Airy function solutions to a 1D Schrödinger equation with a linear confining potential. This sequence of bound states terminates at a threshold energy near 2 times the energy of the lowest bound state. Above this energy scale we observe a broad feature consistent with the onset of the two particle continuum. At energies just below this threshold we observe a prominent excitation that we interpret as a novel bound state of bound states--two pairs of kinks on neighboring chains.