C. W. Chou

Generation of nonclassical photon pairs for scalable quantum communication with atomic ensembles

Quantum information science attempts to exploit capabilities from the quantum realm to accomplish tasks that are otherwise impossible in the classical domain. Although sufficient conditions have been formulated for the physical resources required to achieve quantum computation and communication, there is a growing understanding of the power of quantum measurement combined with the conditional evolution of quantum states for accomplishing diverse tasks in quantum information science. For example, a protocol has recently been developed for the realization of scalable long-distance quantum communication and the distribution of entanglement over quantum networks. Here we report the first enabling step in the realization of this protocol, namely the observation of quantum correlations for photon pairs generated in the collective emission from an atomic ensemble. The nonclassical character of the fields is demonstrated by the violation of an inequality involving their normalized correlation functions. Compared to previous investigations of non-classical correlations for photon pairs produced in atomic cascades and in parametric down-conversion, our experiment is distinct in that the correlated photons are separated by a programmable time interval (of about 400 nanoseconds in our initial experiments).

Measurement induced entanglement for excitation stored in remote atomic ensembles

A critical requirement for diverse applications in quantum information science is the capability to disseminate quantum resources over complex quantum networks. For example, the coherent distribution of entangled quantum states together with quantum memory (for storing the states) can enable scalable architectures for quantum computation, communication and metrology. Here we report observations of entanglement between two atomic ensembles located in distinct, spatially separated set-ups. Quantum interference in the detection of a photon emitted by one of the samples projects the otherwise independent ensembles into an entangled state with one joint excitation stored remotely in 105 atoms at each site. After a programmable delay, we confirm entanglement by mapping the state of the atoms to optical fields and measuring mutual coherences and photon statistics for these fields. We thereby determine a quantitative lower bound for the entanglement of the joint state of the ensembles. Our observations represent significant progress in the ability to distribute and store entangled quantum states.

Single-photon generation from stored excitation in an atomic ensemble

Single photons are generated from an ensemble of cold Cs atoms via the protocol of Duan et al. [Nature (London), ()]]. Conditioned upon an initial detection from field 1 at 852 nm, a photon in field 2 at 894 nm is produced in a controlled fashion from excitation stored within the atomic ensemble. The single-quantum character of field 2 is demonstrated by the violation of a Cauchy-Schwarz inequality, namely w(1(2),1(2)|1(1))=0.24+/-0.05 not > or = 1, where w(1(2),1(2)|1(1)) describes the detection of two events (1(2),1(2)) conditioned upon an initial detection 1(1), with w-->0 for single photons.

Conditional control of the quantum states of remote atomic memories for quantum networking

Quantum networks hold the promise for revolutionary advances in information processing with quantum resources distributed over remote locations via quantum-repeater architectures. Quantum networks are composed of nodes for storing and processing quantum states, and of channels for transmitting states between them. The scalability of such networks relies critically on the ability to carry out conditional operations on states stored in separated quantum memories. Here, we report the first implementation of such conditional control of two atomic memories, located in distinct apparatuses, which results in a 28-fold increase of the probability of simultaneously obtaining a pair of single photons, relative to the case without conditional control. As a first application, we demonstrate a high degree of indistinguishability for remotely generated single photons by the observation of destructive interference of their wave packets. Our results demonstrate experimentally a basic principle for enabling scalable quantum networks, with applications also to linear optics quantum computation.

Direct Measurement of Decoherence for Entanglement between a Photon and Stored Atomic Excitation

Violations of a Bell inequality are reported for an experiment where one of two entangled qubits is stored in a collective atomic memory for a user-defined time delay. The atomic qubit is found to preserve the violation of a Bell inequality for storage times up to 21 micros, 700 times longer than the duration of the excitation pulse that creates the entanglement. To address the question of the security of entanglement-based cryptography implemented with this system, an investigation of the Bell violation as a function of the cross correlation between the generated nonclassical fields is reported, with saturation of the violation close to the maximum value allowed by quantum mechanics.

Temporal dynamics of photon pairs generated by an atomic ensemble.

The time dependence of nonclassical correlations is investigated for two fields (1,2) generated by an ensemble of cold cesium atoms via the protocol of Duan et al. [Nature (London) 414, 413 (2001)]]. The correlation function R(t1,t2) for the ratio of cross to autocorrelations for the (1,2) fields at times (t1,t2) is found to have a maximum value R(max=292+/-57, which significantly violates the Cauchy-Schwarz inequality R< or =1 for classical fields. Decoherence of quantum correlations is observed over taud approximately 175 ns, and is described by our model, as is a new scheme to mitigate this effect.

Cavity QED by the Numbers

The number of atoms trapped within the mode of an optical cavity is determined in real time by monitoring the transmission of a weak probe beam. Continuous observation of atom number is accomplished in the strong coupling regime of cavity quantum electrodynamics and functions in concert with a cooling scheme for radial atomic motion. The probe transmission exhibits sudden steps from one plateau to the next in response to the time evolution of the intracavity atom number, from N >= 3 to N = 2 to 1 to 0, with some trapping events lasting over 1 second.

Quantum Networking with Atomic Ensembles in the Single Excitation Regime

Quantum networks hold the promise for revolutionary advances in information processing with entanglement distributed over remote locations via quantum repeaters. We report two milestones in this direction: the conditional control of memories and the implementation of functional nodes.

Nonclassical photon pairs from a cold atomic ensemble for scalable quantum communication

We report a dramatic improvement of the degree of nonclassical correlation between photon pairs generated by a cold atomic ensemble. The temporal dependence of this correlation and the influence of decoherence are described