Ch. Spielmann

Compression of high-energy laser pulses below 5 fs.

High-energy 20-fs pulses generated by a Ti:sapphire laser system were spectrally broadened to more than 250 nm by self-phase modulation in a hollow fiber filled with noble gases and subsequently compressed in a broadband high-throughput dispersive system. Pulses as short as 4.5 fs with energy up to 20-microJ were obtained with krypton, while pulses as short as 5 fs with energy up to 70 microJ were obtained with argon. These pulses are, to our knowledge, the shortest generated to date at multigigawatt peak powers.

Amplitude and phase control of ultrashort pulses by use of an acousto-optic programmable dispersive filter: pulse compression and shaping

We demonstrate experimentally that an arbitrary phase and amplitude profile can be applied to an ultrashort pulse by use of an acousto-optic programmable dispersive filter (AOPDF). Our filter has a large group-delay range that extends over 3 ps and a 30% diffraction efficiency over 150 THz. Experiments were conducted on a kilohertz chirped-pulse amplification laser chain capable of generating 30-fs pulses without additional pulse shaping. Compensating for gain narrowing and residual phase errors with an AOPDF in place of the stretcher results in 17-fs transform-limited pulses. Arbitrary shaping of these 17-fs pulses is also demonstrated in both the temporal and the spectral domains.

Route to phase control of ultrashort light pulses

A feasibility study of controlling the carrier phase in ultrashort light-wave packets emitted by a sub-10-fs laser is reported. An experimental apparatus capable of exploring the phase sensitivity of nonlinear-optical interactions is presented.

Sub-10-fs mirror-dispersion-controlled Ti:sapphire laser

We demonstrate the generation of nearly bandwidth-limited 8-fs optical pulses near 0.8 microm from a self-mode-locked Ti:sapphire laser oscillator, using chirped dielectric mirrors for dispersion control. The mode-locking performance is described, and limitations are discussed.

Generation of 0.1-TW 5-fs optical pulses at a 1-kHz repetition rate

A compact all-solid-state femtosecond Ti:sapphire oscillator¿amplifier system using no grating-based pulse stretcher produces 20-fs, 1.5-mJ pulses at a 1-kHz repetition rate. The pulses are subsequently compressed in a hollow-fiber chirped-mirror compressor. The system delivers bandwidth-limited 5-fs, 0.5-mJ pulses at 780 nm in a diffraction-limited beam.

Kerr lens mode locking

Self-focusing in conjunction with an intracavity aperture creates a power-dependent amplitude modulation in laser oscillators, which allows passive mode locking. A simple analytical formalism yields closed-form expressions for the depth of passive amplitude modulation introduced by either the spatial gain profile or a hard aperture inserted in the resonator. Design issues for this mode-locking technique are discussed.

Laser technology: source of coherent kiloelectronvolt X-rays.

Generating X-rays that have the properties of laser light has been a long-standing goal for experimental science. Here we describe the emission of highly collimated, spatially coherent X-rays, at a wavelength of about 1 nanometre and at photon energies extending to 1.3 kiloelectronvolts, from atoms that have been ionized by a 5-femtosecond laser pulse. This means that a laboratory source of laser-like, kiloelectronvolt X-rays, which will operate on timescales relevant to many chemical, biological and materials problems, is now within reach.

Self-starting passive mode locking.

We investigate the evolution of continuous-wave laser oscillation from free-running to mode-locked operation assuming a nonlinear device with an intensity-dependent transmittivity or reflectivity to be the mode-locking element. An intensity threshold for self-starting passive mode locking is predicted and related to the linewidth of the first beat note of the power spectrum of the free-running laser output. Experimental results confirm the predictions of the theory.

Operation of a femtosecond Ti:sapphire solitary laser in the vicinity of zero group-delay dispersion

We report the operating characteristics of a self-mode-locked Ti:sapphire solitary laser at reduced group-delay dispersion. The generation of asymptotically equal to 12.3 fs near-sech(2) optical pulses at 775 nm is reported, together with experimental evidence for the dominant role of third-order dispersion (TOD) as a limiting factor to further pulse shortening in the oscillator. At reduced second-order dispersion excessive residual TOD is shown to lead to dispersive wave generation, and the position of the dispersive resonance is used to determine the ratio of the net second- and third-order intracavity dispersions. Since the magnitude of TOD rapidly decreases with increasing wavelength in prism-pair dispersion-compensated resonators, the oscillator presented has the potential for producing sub-10-fs pulses in the 800-nm wavelength region.

Mode locking in solitary lasers.

We present an analysis of passively mode-locked lasers in which pulse formation is dominated by the interplay between self-phase modulation and negative dispersion in separate cavity elements. Steady-state pulse parameters and stability issues are discussed. Stability in these solitary systems relies on some passive amplitude modulation, and the ultimate system performance is found to depend sensitively on the magnitude of amplitude modulation relative to that of phase modulation.