Chao-Xing Liu

Topology-Driven Magnetic Quantum Phase Transition in Topological Insulators

Simultaneous topological and magnetic quantum phase transitions are observed in thin films of Bi2(SexTe1-x)3 doped with chromium Topological insulators owe their exotic properties to the peculiarities of their band structure, and one can induce a transition between a topologically trivial and nontrivial material by chemical doping. Now, J. Zhang et al. (p. 1582) have gone a step further—simultaneously observing that a magnetic quantum transition as the ratio of Se and Te is varied in Bi2(SexTe1-x)3 thin films grown by molecular beam epitaxy and doped with magnetic Cr. Photoemission and transport experiments, as well as density functional calculations, imply that the topological transition induces magnetism The breaking of time reversal symmetry in topological insulators may create previously unknown quantum effects. We observed a magnetic quantum phase transition in Cr-doped Bi2(SexTe1-x)3 topological insulator films grown by means of molecular beam epitaxy. Across the critical point, a topological quantum phase transition is revealed through both angle-resolved photoemission measurements and density functional theory calculations. We present strong evidence that the bulk band topology is the fundamental driving force for the magnetic quantum phase transition. The tunable topological and magnetic properties in this system are well suited for realizing the exotic topological quantum phenomena in magnetic topological insulators.

Zero-Field Dissipationless Chiral Edge Transport and the Nature of Dissipation in the Quantum Anomalous Hall State

The quantum anomalous Hall (QAH) effect is predicted to possess, at a zero magnetic field, chiral edge channels that conduct a spin polarized current without dissipation. While edge channels have been observed in previous experimental studies of the QAH effect, their dissipationless nature at a zero magnetic field has not been convincingly demonstrated. By a comprehensive experimental study of the gate and temperature dependences of local and nonlocal magnetoresistance, we unambiguously establish the dissipationless edge transport. By studying the onset of dissipation, we also identify the origin of dissipative channels and clarify the surprising observation that the critical temperature of the QAH effect is 2 orders of magnitude smaller than the Curie temperature of ferromagnetism.

Above 400-K robust perpendicular ferromagnetic phase in a topological insulator

Topological surface states reveal proximity-induced ferromagnetism with perpendicular anisotropy persisting above 400 K. The quantum anomalous Hall effect (QAHE) that emerges under broken time-reversal symmetry in topological insulators (TIs) exhibits many fascinating physical properties for potential applications in nanoelectronics and spintronics. However, in transition metal–doped TIs, the only experimentally demonstrated QAHE system to date, the QAHE is lost at practically relevant temperatures. This constraint is imposed by the relatively low Curie temperature (Tc) and inherent spin disorder associated with the random magnetic dopants. We demonstrate drastically enhanced Tc by exchange coupling TIs to Tm3Fe5O12, a high-Tc magnetic insulator with perpendicular magnetic anisotropy. Signatures showing that the TI surface states acquire robust ferromagnetism are revealed by distinct squared anomalous Hall hysteresis loops at 400 K. Point-contact Andreev reflection spectroscopy confirms that the TI surface is spin-polarized. The greatly enhanced Tc, absence of spin disorder, and perpendicular anisotropy are all essential to the occurrence of the QAHE at high temperatures.

Unconventional superconductivity in bilayer transition metal dichalcogenides

Bilayer transition metal dichalcogenides (TMDs) belong to a class of materials with two unique features, the coupled spin-valley-layer degrees of freedom and the crystal structure that is globally centrosymmetric but locally noncentrosymmetric. In this Letter, we will show that the combination of these two features can lead to a rich phase diagram for unconventional superconductivity, including intralayer and interlayer singlet pairings and interlayer triplet pairings, in bilayer superconducting TMDs. In particular, we predict that the inhomogeneous Fulde-Ferrell-Larkin-Ovchinnikov state can exist in bilayer TMDs under an in-plane magnetic field. We also discuss the experimental relevance of our results and possible experimental signatures.

Observation of the Quantum Anomalous Hall Insulator to Anderson Insulator Quantum Phase Transition and its Scaling Behavior

Fundamental insight into the nature of the quantum phase transition from a superconductor to an insulator in two dimensions, or from one plateau to the next or to an insulator in the quantum Hall effect, has been revealed through the study of its scaling behavior. Here, we report on the experimental observation of a quantum phase transition from a quantum-anomalous-Hall insulator to an Anderson insulator in a magnetic topological insulator by tuning the chemical potential. Our experiment demonstrates the existence of scaling behavior from which we extract the critical exponent for this quantum phase transition. We expect that our work will motivate much further investigation of many properties of quantum phase transition in this new context.

Helicity dependent photocurrent in electrically gated (Bi 1−x Sb x ) 2 Te 3 thin films

Circularly polarized photons are known to generate a directional helicity-dependent photocurrent in three-dimensional topological insulators at room temperature. Surprisingly, the phenomenon is readily observed at photon energies that excite electrons to states far above the spin-momentum locked Dirac cone and the underlying mechanism for the helicity-dependent photocurrent is still not understood. Here we show a comprehensive study of the helicity-dependent photocurrent in (Bi1−xSbx)2Te3 thin films as a function of the incidence angle of the optical excitation, its wavelength and the gate-tuned chemical potential. Our observations allow us to unambiguously identify the circular photo-galvanic effect as the dominant mechanism for the helicity-dependent photocurrent. Additionally, we use an analytical model to relate the directional nature of the photocurrent to asymmetric optical transitions between the topological surface states and bulk bands. The insights we obtain are important for engineering opto-spintronic devices that rely on optical steering of spin and charge currents.Control of the directional photocurrent by polarized light in topological insulators may enable topological spintronics but is not yet well understood. Here the authors demonstrate that the directional photocurrent is due to the asymmetric optical transitions between topological surface states and bulk states.

Electrically tunable spin polarization of chiral edge modes in a quantum anomalous Hall insulator

In the quantum anomalous Hall effect, chiral edge modes are expected to conduct spin polarized current without dissipation and thus hold great promise for future electronics and spintronics with low energy consumption. However, spin polarization of chiral edge modes has never been established in experiments. In this work, we theoretically study spin polarization of chiral edge modes in the quantum anomalous Hall effect, based on both the effective model and more realistic tight-binding model constructed from the first principles calculations. We find that spin polarization can be manipulated by tuning either a local gate voltage or the Fermi energy. We also propose to extract spin information of chiral edge modes by contacting the quantum anomalous Hall insulator to a ferromagnetic (FM) lead. The establishment of spin polarization of chiral edge modes, as well as the manipulation and detection in a fully electrical manner, will pave the way to the applications of the quantum anomalous Hall effect in spintronics.

Electrically tunable multiple Dirac cones in thin films of the (LaO)2(SbSe2)2 family of materials.

Two-dimensional Dirac physics has aroused great interests in condensed matter physics ever since the discovery of graphene and topological insulators. The ability to control the properties of Dirac cones, such as bandgap and Fermi velocity, is essential for various new phenomena and the next-generation electronic devices. On the basis of first-principles calculations and an analytical effective model, we propose a new Dirac system with eight Dirac cones in thin films of the (LaO)2(SbSe2)2 family of materials, which has the advantage in its tunability: the existence of gapless Dirac cones, their positions, Fermi velocities and anisotropy all can be controlled by an experimentally feasible electric field. We identify layer-dependent spin texture induced by spin-orbit coupling as the underlying physical reason for electrical tunability of this system. Furthermore, the electrically tunable quantum anomalous Hall effect with a high Chern number can be realized by introducing magnetization into this system.

Reentrant quantum anomalous Hall effect with in-plane magnetic fields in HgMnTe quantum wells

Quantum anomalous Hall effect has been predicted in HgMnTe quantum wells with an out-of-plane magnetization of Mn atoms. However, since HgMnTe quantum wells are paramagnetic, an out-of-plane magnetic field is required to polarize magnetic moments of Mn atoms, which inevitably induces Landau levels and makes it difficult to identify the origin of the quantized Hall conductance experimentally. In this work, we study the quantum anomalous Hall effect in the presence of an in-plane magnetic field in Mn doped HgTe quantum wells. For a small out-of-plane magnetic field, the in-plane magnetic field can drive the system from a normal insulating state to a quantum anomalous Hall state. When the out-of-plane magnetic field is slightly above the transition point, the system shows a reentrant behavior of Hall conductance, varying from

Heavy Dirac fermions in a graphene/topological insulator hetero-junction

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