Chinmay Khandekar

Giant frequency-selective near-field energy transfer in active–passive structures

We apply a fluctuation electrodynamics framework in combination with semianalytical (dipolar) approximations to study amplified spontaneous energy transfer (ASET) between active and passive bodies. We consider near-field energy transfer between semi-infinite planar media and spherical structures (dimers and lattices) subject to gain, and show that the combination of loss compensation and near-field enhancement (achieved by the proximity, enhanced interactions, and tuning of subwavelength resonances) in these structures can result in orders of magnitude ASET enhancements below the lasing threshold. We examine various possible geometric configurations, including realistic materials, and describe optimal conditions for enhancing ASET, showing that the latter depends sensitively on both geometry and gain, enabling efficient and tunable gain-assisted energy extraction from structured surfaces.

Radiative heat transfer in nonlinear Kerr media

We obtain a fluctuation--dissipation theorem describing thermal electromagnetic fluctuation effects in nonlinear media that we exploit in conjunction with a stochastic Langevin framework to study thermal radiation from Kerr (

Thermal radiation from optically driven Kerr (χ(3)) photonic cavities

\chi^{(3)}

Near-field thermal upconversion and energy transfer through a Kerr medium

) photonic cavities coupled to external environments at and out of equilibrium. We show that that in addition to thermal broadening due to two-photon absorption,the emissivity of such cavities can exhibit asymmetric,non-Lorentzian lineshapes due to self-phase modulation. When the local temperature of the cavity is larger than that of the external bath, we find that the heat transfer into the bath exceeds the radiation from a corresponding linear black body at the same local temperature. We predict that these temperature-tunable thermal processes can be observed in practical, nanophotonic cavities operating at relatively small temperatures.

Amplified and directional spontaneous emission from arbitrary composite bodies: A self-consistent treatment of Purcell effect below threshold

We describe thermal radiation from nonlinear (χ(3)) photonic cavities coupled to external channels and subject to incident monochromatic light. Our work extends related work on nonlinear mechanical oscillators to the problem of thermal radiation, demonstrating that bistability can enhance thermal radiation by orders of magnitude and result in strong lineshape alternations, including “super-narrow spectral peaks” occurring at the onset of kinetic phase transitions. We show that when the cavities are designed to exhibit perfect linear emissivity (rate matching), such thermally activated transitions can be exploited to dramatically tune the output power and radiative properties of the cavity, leading to a kind of Kerr-mediated thermo-optic effect. Finally, we demonstrate that in certain parameter regimes, the output radiation exhibits Stokes and anti-Stokes side peaks whose relative magnitudes can be altered by tuning the internal temperature of the cavity relative to its surroundings, a consequence of stron...

Near-field refrigeration and tunable heat exchange through four-wave mixing

We present an approach for achieving large Kerr χ(3)-mediated thermal energy transfer at the nanoscale that exploits a general coupled-mode description of triply resonant, four-wave mixing processes. We analyze the efficiency of thermal upconversion and energy transfer from mid- to near-infrared wavelengths in planar geometries involving two slabs supporting far-apart surface plasmon polaritons and separated by a nonlinear χ(3) medium that is irradiated by externally incident light. We study multiple geometric and material configurations and different classes of intervening mediums-either bulk or nanostructured lattices of nanoparticles embedded in nonlinear materials-designed to resonantly enhance the interaction of the incident light with thermal slab resonances. We find that even when the entire system is in thermodynamic equilibrium (at room temperature) and under typical drive intensities ~ W/μm2, the resulting upconversion rates can approach and even exceed thermal flux rates achieved in typical symmetric and non-equilibrium configurations of vacuum-separated slabs. The proposed nonlinear scheme could potentially be exploited to achieve thermal cooling and refrigeration at the nanoscale, and to actively control heat transfer between materials with dramatically different resonant responses.

Thermal bistability through coupled photonic resonances

We study amplified spontaneous emission (ASE) from wavelength-scale composite bodies--complicated arrangements of active and passive media--demonstrating highly directional and tunable radiation patterns, depending strongly on pump conditions, materials, and object shapes. For instance, we show that under large enough gain,

Near-field thermal upconversion through a Kerr medium

\mathcal{PT}

Giant frequency-selective near-field heat transfer in

symmetric dielectric spheres radiate mostly along either active or passive regions, depending on the gain distribution. Our predictions are based on a recently proposed fluctuating volume--current (FVC) formulation of electromagnetic radiation that can handle inhomogeneities in the dielectric and fluctuation statistics of active media, e.g. arising from the presence of non-uniform pump or material properties, which we exploit to demonstrate an approach to modelling ASE in regimes where Purcell effect (PE) has a significant impact on the gain, leading to spatial dispersion and/or changes in power requirements. The nonlinear feedback of PE on the active medium, captured by the Maxwell--Bloch equations but often ignored in linear formulations of ASE, is introduced into our linear framework by a self-consistent renormalization of the (dressed) gain parameters, requiring the solution of a large system of nonlinear equations involving many linear scattering calculations.

\mathcal{PT}

We modify and extend a recently proposed four-wave mixing scheme [Opt. Express 25 (19),23164 (2017)] for achieving near-field thermal upconversion and energy transfer, to demonstrate efficient thermal refrigeration at low intensities