Christian H. Schunck

Condensation of Pairs of Fermionic Atoms near a Feshbach Resonance

We have observed Bose-Einstein condensation of pairs of fermionic atoms in an ultracold 6Li gas at magnetic fields above a Feshbach resonance, where no stable 6Li2 molecules would exist in vacuum. We accurately determined the position of the resonance to be 822+/-3 G. Molecular Bose-Einstein condensates were detected after a fast magnetic field ramp, which transferred pairs of atoms at close distances into bound molecules. Condensate fractions as high as 80% were obtained. The large condensate fractions are interpreted in terms of preexisting molecules which are quasistable even above the two-body Feshbach resonance due to the presence of the degenerate Fermi gas.

Observation of bose-einstein condensation of molecules

We have observed Bose-Einstein condensation of molecules, created from a spin mixture of fermionic 6Li atoms. The condensate realizes the limit of tightly bound fermion pairs in the crossover between BCS and BEC superfluidity

Vortices and superfluidity in a strongly interacting Fermi gas

Quantum degenerate Fermi gases provide a remarkable opportunity to study strongly interacting fermions. In contrast to other Fermi systems, such as superconductors, neutron stars or the quark-gluon plasma of the early Universe, these gases have low densities and their interactions can be precisely controlled over an enormous range. Previous experiments with Fermi gases have revealed condensation of fermion pairs. Although these and other studies were consistent with predictions assuming superfluidity, proof of superfluid behaviour has been elusive. Here we report observations of vortex lattices in a strongly interacting, rotating Fermi gas that provide definitive evidence for superfluidity. The interaction and therefore the pairing strength between two 6Li fermions near a Feshbach resonance can be controlled by an external magnetic field. This allows us to explore the crossover from a Bose–Einstein condensate of molecules to a Bardeen–Cooper–Schrieffer superfluid of loosely bound pairs. The crossover is associated with a new form of superfluidity that may provide insights into high-transition-temperature superconductors.

Fermionic Superfluidity with Imbalanced Spin Populations

We established superfluidity in a two-state mixture of ultracold fermionic atoms with imbalanced state populations. This study relates to the long-standing debate about the nature of the superfluid state in Fermi systems. Indicators for superfluidity were condensates of fermion pairs and vortices in rotating clouds. For strong interactions, near a Feshbach resonance, superfluidity was observed for a broad range of population imbalances. We mapped out the superfluid regime as a function of interaction strength and population imbalance and characterized the quantum phase transition to the normal state, known as the Pauli limit of superfluidity.

Observation of Phase Separation in a Strongly-Interacting Imbalanced Fermi Gas

We have observed phase separation between the superfluid and the normal component in a strongly interacting Fermi gas with imbalanced spin populations. The in situ distribution of the density difference between two trapped spin components is obtained using phase-contrast imaging and 3D image reconstruction. A shell structure is clearly identified where the superfluid region of equal densities is surrounded by a normal gas of unequal densities. The phase transition induces a dramatic change in the density profiles as excess fermions are expelled from the superfluid.

Radio-Frequency Spectroscopy of Ultracold Fermions

Radio-frequency techniques were used to study ultracold fermions. We observed the absence of mean-field “clock” shifts, the dominant source of systematic error in current atomic clocks based on bosonic atoms. This absence is a direct consequence of fermionic antisymmetry. Resonance shifts proportional to interaction strengths were observed in a three-level system. However, in the strongly interacting regime, these shifts became very small, reflecting the quantum unitarity limit and many-body effects. This insight into an interacting Fermi gas is relevant for the quest to observe superfluidity in this system.

Phase diagram of a two-component Fermi gas with resonant interactions.

The pairing of fermions lies at the heart of superconductivity and superfluidity. The stability of these pairs determines the robustness of the superfluid state, and the quest for superconductors with high critical temperature equates to a search for systems with strong pairing mechanisms. Ultracold atomic Fermi gases present a highly controllable model system for studying strongly interacting fermions. Tunable interactions (through Feshbach collisional resonances) and the control of population or mass imbalance among the spin components provide unique opportunities to investigate the stability of pairing—and possibly to search for exotic forms of superfluidity. A major controversy has surrounded the stability of superfluidity against an imbalance between the two spin components when the fermions interact resonantly (that is, at unitarity). Here we present the phase diagram of a spin-polarized Fermi gas of 6Li atoms at unitarity, experimentally mapping out the superfluid phases versus temperature and density imbalance. Using tomographic techniques, we reveal spatial discontinuities in the spin polarization; this is the signature of a first-order superfluid-to-normal phase transition, and disappears at a tricritical point where the nature of the phase transition changes from first-order to second-order. At zero temperature, there is a quantum phase transition from a fully paired superfluid to a partially polarized normal gas. These observations and the implementation of an in situ ideal gas thermometer provide quantitative tests of theoretical calculations on the stability of resonant superfluidity.

Direct observation of the superfluid phase transition in ultracold Fermi gases.

Phase transitions are dramatic phenomena: water freezes into ice, atomic spins spontaneously align in a magnet, and liquid helium becomes superfluid. Sometimes, such a drastic change in behaviour is accompanied by a visible change in appearance. The hallmark of Bose–Einstein condensation and superfluidity in trapped, weakly interacting Bose gases is the sudden formation of a dense central core inside a thermal cloud. However, in strongly interacting gases—such as the recently observed fermionic superfluids—there is no longer a clear separation between the superfluid and the normal parts of the cloud. The detection of fermion pair condensates has required magnetic field sweeps into the weakly interacting regime, and the quantitative description of these sweeps presents a major theoretical challenge. Here we report the direct observation of the superfluid phase transition in a strongly interacting gas of 6Li fermions, through sudden changes in the shape of the clouds—in complete analogy to the case of weakly interacting Bose gases. By preparing unequal mixtures of the two spin components involved in the pairing, we greatly enhance the contrast between the superfluid core and the normal component. Furthermore, the distribution of non-interacting excess atoms serves as a direct and reliable thermometer. Even in the normal state, strong interactions significantly deform the density profile of the majority spin component. We show that it is these interactions that drive the normal-to-superfluid transition at the critical population imbalance of 70 ± 5 per cent (ref. 12).

Fiftyfold Improvement in the Number of Quantum Degenerate Fermionic Atoms

We have produced a quantum degenerate 6Li Fermi gas with up to 7 x 10(7) atoms, an improvement by a factor of 50 over all previous experiments with degenerate Fermi gases. This was achieved by sympathetic cooling with bosonic 23Na in the F=2, upper hyperfine ground state. We have also achieved Bose-Einstein condensation of F=2 sodium atoms by direct evaporation.

Decay of an ultracold fermionic lithium gas near a Feshbach resonance

We studied the magnetic field dependence of the inelastic decay of an ultracold, optically trapped fermionic /sup 6/Li gas of different spin compositions. The spin mixture of the two lowest hyperfine states showed two decay resonances at 550 G and 680 G, consistent with the predicted Feshbach resonances for elastic s-wave collisions. The observed lifetimes of several hundred milliseconds are much longer than the expected time for Cooper pair formation and the phase transition to superfluidity in the vicinity of the Feshbach resonance.