Christian Spielmann

Femtosecond solid-state lasers

The emergence of new ultrafast optical modulation techniques has opened the way towards a new femtosecond laser technology based on solid-state gain media. The authors address the requirements for stable ultrashort pulse generation in these novel femtosecond sources. The theoretical considerations are backed up by experimental results obtained with a number of different laser systems. The conclusions drawn from the presented theoretical and experimental investigations provide general guidelines for the design and optimization of a wide range of femtosecond solid-state laser oscillators. >

Ultrabroadband femtosecond lasers

The exploitation of soliton-like pulse shaping mechanisms and the optimization of phase dispersion in broadband self-modelocked solid state laser oscillators have led to unprecedented advances in ultrafast laser technology. This paper reviews the basic physical mechanisms governing pulse formation and addresses the requirements for optimum performance of these novel ultrashort pulse laser sources. These considerations together with the demonstration of /spl ap/10 fs pulse generation from a Ti:sapphire laser suggest that a family of solid-state laser oscillators with comparable performance can be developed. >

Laser ablation of dielectrics with pulse durations between 20 fs and 3 ps

Laser‐induced ablation has been extended down to a pulse duration of 20 fs generated by a Ti sapphire laser system at a wavelength of 780 nm. Barium aluminum borosilicate glass with an extremely high glass transformation temperature (∼600 °C) served as target material. The most significant observation was a substantial decrease of the ablation threshold fluence at pulse durations below 100 fs. All results indicate a dominant role of multiphoton absorption in addition to collisional ionization in this time domain.

Generation of 11-fs pulses from a Ti:sapphire laser without the use of prisms

The generation of highly stable optical pulses as short as 11 fs from a Kerr-lens mode-locked Ti:sapphire laser containing no intracavity prisms is demonstrated. In the femtosecond oscillator design reported, novel dielectric mirrors provide broadband dispersion control for solitonlike pulse formation.

X-ray absorption spectroscopy in the keV range with laser generated high harmonic radiation

By irradiating He and Ne atoms with 3mJ, 12fs, near infrared laser pulses from a tabletop laser system, the authors generated spatially and temporally coherent x rays up to a photon energy of 3.5keV. With this source it is possible to use high-harmonic radiation for x-ray absorption spectroscopy in the keV range. They were able to clearly resolve the L absorption edges of titanium and copper and the K edges of aluminum and silicon. From the fine structure of the x-ray absorption they estimated the interatomic distances.

Toward a terawatt-scale sub-10-fs laser technology

Powerful techniques for spectral broadening and ultrabroad-band dispersion control, which allow compression of high-energy femtosecond pulses to a duration of a few optical cycles, are analyzed. Spectral broadening in a gas-filled hollow fiber and compression by chirped mirrors with high-energy 20-fs input pulses are presented. Using 1-mJ seed pulses we have demonstrated the generation of 0.5-mJ 5-fs pulses at 0.8-/spl mu/m and 1-kHz repetition rate. General design criteria to scale the compression technique toward the terawatt level are presented.

Laser micromachining of barium aluminium borosilicate glass with pulse durations between 20 fs and 3 ps

Laser-micromachining of high-tech glass has been extended down to a pulse duration of 20 fs generated by a Ti sapphire laser system at a wavelength of 780 nm. A systematic electronmicroscopic study shows that, below 100 fs, an extreme precision and a substantial decrease of the ablation threshold fluence with respect to pulse laser processing with pulses in the picosecond and nanosecond range could be achieved. The technical relevance of this novel microtechnology is discussed. The morphology of the ablated areas is not determined by thermal processes, i.e. the heat affected zone. It is controlled by non-linear optical coupling effects. Multi-photon absorption becomes highly efficient below laser pulse durations of 100 fs so that light penetration is minimized and ablation cavities become smooth. At longer pulse durations, a higher light penetration due to a lower number of non-linearly absorbed photons allows mechanical relaxation processes in the glass material leading to roughening.

Dispersion control over 150 THz with chirped dielectric mirrors

Ultrabroad-band chirped multilayer dielectric mirrors providing nearly constant negative group delay dispersion over the wavelength range of 640-950 nm and high reflectance between 590 and 970 nm are demonstrated. A key to this performance has been an improved design method, which also substantially reduces the computing time needed for ultimate optimization. The presented devices constitute an enabling technology for producing high-quality terawatt pulses in the sub-10-fs regime. The generation of 5-fs 0.1-TW pulses by using exclusively these mirrors as negative delay line demonstrates this potential.

Submicron extreme ultraviolet imaging using high-harmonic radiation

We report on experiments using high-harmonic (HH) radiation for microscopy imaging at 13 nm wavelength. A simple setup using a zone plate as objective and a back-illuminated CCD as detector yields at moderate magnifications of M≈60 a spatial resolution of δx<0.8 μm demonstrated with a sample of mica. The HH radiation was monochromatized by means of a high-efficiency multilayer monochromator consisting of two Mo/Si-mirros.

Experimental study of additive-pulse mode locking in an Nd:glass laser

Self-starting additive-pulse mode locking (APM) has been investigated experimentally in a continuous-wave Nd:glass laser. Stress has been put on the study of the self-starting process and relaxation oscillation instabilities. An intensity threshold for self-starting APM is observed and related to the linewidth of the first beat note of the power spectrum of the free-running laser output. Under steady-state conditions, two distinct operating regimes are obtained: mode locking with repetitive self-Q switching and pure mode locking. Increasing the intracavity power gives rise to a strong chirp developing on the mode-locked pulses and to a simultaneous disappearance of self-Q switching. >