Christof Weitenberg

Single-atom-resolved fluorescence imaging of an atomic Mott insulator

The reliable detection of single quantum particles has revolutionized the field of quantum optics and quantum information processing. For several years, researchers have aspired to extend such detection possibilities to larger-scale, strongly correlated quantum systems in order to record in situ images of a quantum fluid in which each underlying quantum particle is detected. Here we report fluorescence imaging of strongly interacting bosonic Mott insulators in an optical lattice with single-atom and single-site resolution. From our images, we fully reconstruct the atom distribution on the lattice and identify individual excitations with high fidelity. A comparison of the radial density and variance distributions with theory provides a precise in situ temperature and entropy measurement from single images. We observe Mott-insulating plateaus with near-zero entropy and clearly resolve the high-entropy rings separating them, even though their width is of the order of just a single lattice site. Furthermore, we show how a Mott insulator melts with increasing temperature, owing to a proliferation of local defects. The ability to resolve individual lattice sites directly opens up new avenues for the manipulation, analysis and applications of strongly interacting quantum gases on a lattice. For example, one could introduce local perturbations or access regions of high entropy, a crucial requirement for the implementation of novel cooling schemes.

Single―spin addressing in an atomic Mott insulator

Ultracold atoms in optical lattices provide a versatile tool with which to investigate fundamental properties of quantum many-body systems. In particular, the high degree of control of experimental parameters has allowed the study of many interesting phenomena, such as quantum phase transitions and quantum spin dynamics. Here we demonstrate how such control can be implemented at the most fundamental level of a single spin at a specific site of an optical lattice. Using a tightly focused laser beam together with a microwave field, we were able to flip the spin of individual atoms in a Mott insulator with sub-diffraction-limited resolution, well below the lattice spacing. The Mott insulator provided us with a large two-dimensional array of perfectly arranged atoms, in which we created arbitrary spin patterns by sequentially addressing selected lattice sites after freezing out the atom distribution. We directly monitored the tunnelling quantum dynamics of single atoms in the lattice prepared along a single line, and observed that our addressing scheme leaves the atoms in the motional ground state. The results should enable studies of entropy transport and the quantum dynamics of spin impurities, the implementation of novel cooling schemes, and the engineering of quantum many-body phases and various quantum information processing applications.

Observation of Correlated Particle-Hole Pairs and String Order in Low-Dimensional Mott Insulators

Parity correlations in a one-dimensional Bose gas in an optical lattice reveal a hidden “string order.” Quantum phases of matter are characterized by the underlying correlations of the many-body system. Although this is typically captured by a local order parameter, it has been shown that a broad class of many-body systems possesses a hidden nonlocal order. In the case of bosonic Mott insulators, the ground state properties are governed by quantum fluctuations in the form of correlated particle-hole pairs that lead to the emergence of a nonlocal string order in one dimension. By using high-resolution imaging of low-dimensional quantum gases in an optical lattice, we directly detect these pairs with single-site and single-particle sensitivity and observe string order in the one-dimensional case.

Experimental reconstruction of the Berry curvature in a Floquet Bloch band

Cold atoms do geometry Electrons in solids populate energy bands, which can be simulated in cold atom systems using optical lattices. The geometry of the corresponding wave functions determines the topological properties of the system, but getting a direct look is tricky. Fläschner et al. and Li et al. measured the detailed structure of the band wave functions in hexagonal optical lattices, one resembling a boron-nitride and the other a graphene lattice. These techniques will make it possible to explore more complex situations that include the effects of interactions. Science, this issue pp. 1091 and 1094 Berry curvature is engineered and measured in a simulated boron-nitride optical lattice filled with fermionic K atoms. Topological properties lie at the heart of many fascinating phenomena in solid-state systems such as quantum Hall systems or Chern insulators. The topology of the bands can be captured by the distribution of Berry curvature, which describes the geometry of the eigenstates across the Brillouin zone. Using fermionic ultracold atoms in a hexagonal optical lattice, we engineered the Berry curvature of the Bloch bands using resonant driving and show a full momentum-resolved measurement of the ensuing Berry curvature. Our results pave the way to explore intriguing phases of matter with interactions in topological band structures.

Observation of dynamical vortices after quenches in a system with topology

Topological phases constitute an exotic form of matter characterized by non-local properties rather than local order parameters1. The paradigmatic Haldane model on a hexagonal lattice features such topological phases distinguished by an integer topological invariant known as the first Chern number2. Recently, the identification of non-equilibrium signatures of topology in the dynamics of such systems has attracted particular attention3–6. Here, we experimentally study the dynamical evolution of the wavefunction using time- and momentum-resolved full state tomography for spin-polarized fermionic atoms in driven optical lattices7. We observe the appearance, movement and annihilation of dynamical vortices in momentum space after sudden quenches close to the topological phase transition. These dynamical vortices can be interpreted as dynamical Fisher zeros of the Loschmidt amplitude8, which signal a so-called dynamical phase transition9,10. Our results pave the way to a deeper understanding of the connection between topological phases and non-equilibrium dynamics.Non-equilibrium signatures of topology—the appearance, movement and annihilation of vortices in a cold-atom system—are identified, showing that topological phase can emerge dynamically from a non-topological state.Phase transitions are a fundamental concept in science describing diverse phenomena ranging from, e.g., the freezing of water to Bose-Einstein condensation. While the concept is well-established in equilibrium, similarly fundamental concepts for systems far from equilibrium are just being explored, such as the recently introduced dynamical phase transition (DPT). Here we report on the first observation of a DPT in the dynamics of a fermionic many-body state after a quench between two lattice Hamiltonians. With time-resolved state tomography in a system of ultracold atoms in optical lattices, we obtain full access to the evolution of the wave function. We observe the appearance, movement, and annihilation of vortices in reciprocal space. We identify their number as a dynamical topological order parameter, which suddenly changes its value at the critical times of the DPT. Our observation of a DPT is an important step towards a more comprehensive understanding of non-equilibrium dynamics in general.

Quench-induced supercurrents in an annular Bose gas.

We create supercurrents in annular two-dimensional Bose gases through a temperature quench of the normal-to-superfluid phase transition. We detect the magnitude and the direction of these supercurrents by measuring spiral patterns resulting from the interference of the cloud with a central reference disk. These measurements demonstrate the stochastic nature of the supercurrents. We further measure their distribution for different quench times and compare it with predictions based on the Kibble-Zurek mechanism.

Protein adsorption on tailored substrates: long-range forces and conformational changes

Adsorption of proteins onto solid surfaces is an everyday phenomenon that is not yet fully understood. To further the current understanding, we have performed in situ ellipsometry studies to reveal the adsorption kinetics of three different proteins, lysozyme, α-amylase and bovine serum albumin. As substrates we offer Si wafers with a controlled Si oxide layer thickness and a hydrophilic or hydrophobic surface functionalization, allowing the tailoring of the influence of short- and long-range interactions. Our studies show that not only the surface chemistry determines the properties of an adsorbed protein layer but also the van der Waals contributions of a composite substrate. We compare the experimental findings to results of a colloidal Monte Carlo approach that includes conformational changes of the adsorbed proteins induced by density fluctuations.

Emergence of coherence via transverse condensation in a uniform quasi-two-dimensional Bose gas

Phase transitions are ubiquitous in our three-dimensional world. By contrast, most conventional transitions do not occur in infinite uniform low-dimensional systems because of the increased role of thermal fluctuations. The crossover between these situations constitutes an important issue, dramatically illustrated by Bose-Einstein condensation: a gas strongly confined along one direction of space may condense along this direction without exhibiting true long-range order in the perpendicular plane. Here we explore transverse condensation for an atomic gas confined in a novel trapping geometry, with a flat in-plane bottom, and we relate it to the onset of an extended (yet of finite-range) in-plane coherence. By quench crossing the transition, we observe topological defects with a mean number satisfying the universal scaling law predicted by Kibble-Zurek mechanism. The approach described can be extended to investigate the topological phase transitions that take place in planar quantum fluids.

Coherent Light Scattering from a Two-Dimensional Mott Insulator

We experimentally demonstrate coherent light scattering from an atomic Mott insulator in a two-dimensional lattice. The far-field diffraction pattern of small clouds of a few hundred atoms was imaged while simultaneously laser cooling the atoms with the probe beams. We describe the position of the diffraction peaks and the scaling of the peak parameters by a simple analytic model. In contrast to Bragg scattering, scattering from a single plane yields diffraction peaks for any incidence angle. We demonstrate the feasibility of detecting spin correlations via light scattering by artificially creating a one-dimensional antiferromagnetic order as a density wave and observing the appearance of additional diffraction peaks.

Quantum computation architecture using optical tweezers

We present a complete architecture for scalable quantum computation with ultracold atoms in optical lattices using optical tweezers focused to the size of a lattice spacing. We discuss three different two-qubit gates based on local collisional interactions. The gates between arbitrary qubits require the transport of atoms to neighboring sites. We numerically optimize the nonadiabatic transport of the atoms through the lattice and the intensity ramps of the optical tweezer in order to maximize the gate fidelities. We find overall gate times of a few 100 μs, while keeping the error probability due to vibrational excitations and spontaneous scattering below 10−3. The requirements on the positioning error and intensity noise of the optical tweezer and the magnetic field stability are analyzed and we show that atoms in optical lattices could meet the requirements for fault-tolerant scalable quantum computing.