Christopher A. Ebbers

Second-harmonic generation in zinc tris(thiourea) sulfate

The linear and second-order nonlinear optical properties of single-crystal zinc tris(thiourea) sulfate, or ZTS, are determined. The deduced nonlinear coefficients are |d(31)| = 0.31, |d(32)| = 0.35, and |d(33)| = 0.23 pm/V compared with a |d(14)| value of 0.39 pm/V for potassium dihydrogen phosphate. Because it exhibits a low angular sensitivity (deltaDeltak/deltatheta), ZTS may prove useful for type-II second-harmonic generation from 1.06 to 1.027 microm. We present the phase-matching measurement data for ZTS and compare the calculated frequency conversion efficiency for ZTS with that of several other well-characterized materials.

L-Histidine tetrafluoroborate: a solution-grown semiorganic crystal for nonlinear frequency conversion

The crystal structure, refractive indices, and phase-matching conditions for a new nonlinear optical material, L-histidine tetrafluoroborate (HFB), are reported. HFB grows readily, displays favorable mechanical characteristics, and has adequate birefringence to permit phase-matched parametric processes over much of its transparency range (250 nm to 1300 nm). The phase-matching loci and angular sensitivity for second-harmonic generation of 1064-nm light in single crystals of HFB were measured. The effective nonlinearity for HFB is comparable with that of beta-barium borate (~2 pm/V), and its angular sensitivity [delta(Deltak)/deltatheta] is somewhat smaller.

Demonstration of a 1.1 petawatt laser based on a hybrid optical parametric chirped pulse amplification/mixed Nd:glass amplifier

We present the design and performance of the Texas Petawatt Laser, which produces a 186 J 167 fs pulse based on the combination of optical parametric chirped pulse amplification (OPCPA) and mixed Nd:glass amplification. OPCPA provides the majority of the gain and is used to broaden and shape the seed spectrum, while amplification in Nd:glass accounts for >99% of the final pulse energy. Compression is achieved with highly efficient multilayer dielectric gratings.

Optical parametric chirped-pulse amplifier as an alternative to Ti:sapphire regenerative amplifiers

We demonstrated a high-pulse energy, femtosecond-pulse source based on optical parametric chirped-pulse amplification. We successfully amplified 1-microm broadband oscillator pulses to 31 mJ and recompressed them to 310-fs pulse duration, at a 10-Hz repetition rate. The gain in our system is 6 x 10(7), achieved by the single passing of only 40 mm of gain material pumped by a commercial Q-switched Nd:YAG laser. This relatively simple system replaces a more complex Ti:sapphire regenerative-amplifier-based chirped-pulse amplification system. Numerous features in design and performance of optical parametric chirped-pulse amplifiers make them a preferred alternative to regenerative amplifiers based on Ti:sapphire in the front end of high-peak-power lasers.

High-average-power 1-/spl mu/m performance and frequency conversion of a diode-end-pumped Yb:YAG laser

Using a diode-end-pumped technology, a Yb:YAG laser capable of delivering up to 434 W of CW power has been demonstrated. The system incorporates a unique composite rod design which allows for high-average-power operation while simultaneously suppressing parasitic oscillations. Modeling and experimental data to support the quenching of parasitics are discussed. Beam quality measurements for CW operation with several cavity configurations are presented. In particular, beam quality measurements at 340-W CW yielded a beam quality factor of M/sup 2/=21. Predictions of a quasi-three-level model are compared with the experimental data for several output coupler reflectivities. An observed dependence of the cavity mode fill as a function of output coupler reflectivity is discussed. Employing a single acoustooptical switch, the system was Q-switched at 10 kHz and generated output powers up to 280 W with a measured beam quality of M/sup 2/=6.8 at 212 W, With an external dual-KTP crystal configuration, the Q-switched output was frequency converted to 515 nm and produced up to 76 W at 10 kHz in a 30-ns pulse length.

The mercury project : A high average power, gas-cooled laser for inertial fusion energy development

Abstract Hundred-joule, kilowatt-class lasers based on diode-pumped solid-state technologies, are being developed worldwide for laser-plasma interactions and as prototypes for fusion energy drivers. The goal of the Mercury Laser Project is to develop key technologies within an architectural framework that demonstrates basic building blocks for scaling to larger multi-kilojoule systems for inertial fusion energy (IFE) applications. Mercury has requirements that include: scalability to IFE beamlines, 10 Hz repetition rate, high efficiency, and 109 shot reliability. The Mercury laser has operated continuously for several hours at 55 J and 10 Hz with fourteen 4 × 6 cm2 ytterbium doped strontium fluoroapatite amplifier slabs pumped by eight 100 kW diode arrays. A portion of the output 1047 nm was converted to 523 nm at 160 W average power with 73 % conversion efficiency using yttrium calcium oxy-borate (YCOB).

High-average-power femto-petawatt laser pumped by the Mercury laser facility

The Mercury laser system is a diode-pumped solid-state laser that has demonstrated over 60 J at a repetition rate of 10 Hz (600 W) of near-infrared light (1047 nm). Using a yttrium calcium oxyborate frequency converter, we have demonstrated 31.7 J/pulse at 10 Hz of second harmonic generation. The frequency converted Mercury laser system will pump a high-average-power Ti:sapphire chirped pulse amplifier system that will produce a compressed peak power > 1 PW and peak irradiance > 1023W/cm2.

Hybrid chirped-pulse amplification

Conversion efficiency in optical parametric chirped-pulse amplification is limited by spatiotemporal characteristics of the pump pulse. We have demonstrated a novel hybrid chirped-pulse amplification scheme that uses a single pump pulse and combines optical parametric amplification and laser amplification to achieve high gain, high conversion efficiency, and high prepulse contrast without utilization of electro-optic modulators. We achieved an overall conversion efficiency of 37% from the hybrid amplification system at a center wavelength of 820nm. Generation of multiterawatt pulses is possible by use of this simple method and commercial Q -switched pump lasers.

Analysis of an intracavity-doubled diode-pumped Q-switched Nd:YAG laser producing more than 100 W of power at 0.532 µm

A diode-pumped Nd:YAG laser was frequency doubled to 0.532 microm with an intracavity KTiOPO(4) crystal in a V-cavity arrangement, achieving an output power of 140 W. Acousto-optic Q switching was employed at repetition rates of 10-30 kHz, and the beam quality was assessed at M(2) approximately 50. It was deduced on the basis of our model that the strength of the nonlinear frequency conversion is the main parameter determining the pulse width.

Nonlinear optical properties of LaCa(4)O(BO(3))(3).

We have grown LaCa(4)O (BO(3))(3) (LaCOB), an isostructural member of GdCa(4)O(BO(3))(3) (GdCOB) family and characterized its nonlinear optical properties. At 1064nm, d(eff) of 0.52+/-0.05 pm /V and an angular sensitivity of 1224+/-184(cm rad)(-1) for type I frequency doubling in LaCOB were determined relative to those of KTiOPO(4) , beta-BaB(2)O(4) , KD(2)PO(4) , LiB(3)O(5) , YCa(4)O(BO(3))(3) (YCOB), and GdCOB. The d(alphabetabeta) and d(gammabetabeta) coefficients of the nonlinear optical tensor for LaCOB, GdCOB, and YCOB were determined to be equivalent within the experimental uncertainty and have values of ?0.26+/-0.04?pm/V and ?1.69+/-0.17?pm /V , respectively. From phase-matching angle measurements at 1064 and 1047nm, we predict that LaCOB is noncritically phase matched at 1042+/-1.5 nm .