D. English

Controlling atomic vapor density in paraffin-coated cells using light-induced atomic desorption

Atomic-vapor density change due to light induced atomic desorption (LIAD) is studied in paraffincoated rubidium, cesium, sodium and potassium cells. In the present experiment, low-intensity probe light is used to obtain an absorption spectrum and measure the vapor density, while light from an argon-ion laser, array of light emitting diodes, or discharge lamp is used for desorption. Potassium is found to exhibit significantly weaker LIAD from paraffin compared to Rb and Cs, and we were unable to observe LIAD with sodium. A simple LIAD model is applied to describe the observed vapor-density dynamics, and the role of the cell’s stem is explored through the use of cells with lockable stems. Stabilization of Cs vapor density above its equilibrium value over 25 minutes is demonstrated. The results of this work could be used to assess the use of LIAD for vapor-density control in magnetometers, clocks, and gyroscopes utilizing coated cells.

Spectroscopic Test of Bose-Einstein Statistics for Photons

Using Bose-Einstein-statistics-forbidden two-photon excitation in atomic barium, we have limited the rate of statistics-violating transitions, as a fraction ν of an equivalent statistics-allowed transition rate, to ν<4.0×10{-11} at the 90% confidence level. This is an improvement of more than 3 orders of magnitude over the best previous result. Additionally, hyperfine-interaction enabling of the forbidden transition has been observed, to our knowledge, for the first time.

Progress towards fundamental symmetry tests with nonlinear optical rotation

Magneto-optical (Faraday) rotation is a process in which the plane of light polarization rotates as light propagates through a medium along the direction of a magnetic field. In atomic vapors where ground state atomic polarization relaxes very slowly (relaxation rates ≳1 Hz), there arise ultranarrow, light-power-dependent (nonlinear) features in the magnetic field dependence of Faraday rotation. The shot-noise-limited sensitivity of a magnetometer based on nonlinear Faraday rotation can exceed 10−11 G/Hz, corresponding to a sensitivity of ∼10−6 Hz/Hz to Zeeman sublevel shifts. Here we discuss recent progress in magnetometry based on nonlinear optical rotation and consider the application of these methods to searches for fundamental-symmetry-violating interactions.

Hyperfine-interaction- and magnetic-field-induced Bose-Einstein-statistics suppressed two-photon transitions

Two-photon transitions between atomic states of total electronic angular momentum Ja = 0 and Jb = 1 are forbidden when the photons are of the same energy. This selection rule is analogous to the Landau-Yang theorem in particle physics that forbids decays of vector particle into two photons. It arises because it is impossible to construct a total angular momentum J2γ = 1 quantum-mechanical state of two photons that is permutation symmetric, as required by Bose-Einstein statistics. In atoms with non-zero nuclear spin, the selection rule can be violated due to hyperfine interactions. Two distinct mechanisms responsible for the hyperfine-induced two-photon transitions are identified, and the hyperfine structure of the induced transitions is evaluated. The selection rule is also relaxed, even for zero-nuclear-spin atoms, by application of an external magnetic field. Once again, there are two similar mechanisms at play: Zeeman splitting of the intermediate-state sublevels, and off-diagonal mixing of states with different total electronic angular momentum in the final state. The present theoretical treatment is relevant to the ongoing experimental search for a possible Bose-Einsteinstatistics violation using two-photon transitions in barium, where the hyperfine-induced transitions have been recently observed, and the magnetic-field-induced transitions are being considered both as a possible systematic effect, and as a way to calibrate the measurement.

Atomic parity violation inJ=0→0two-photon transitions

We present a method for measuring atomic parity violation in the absence of static external electric and magnetic fields. Such measurements can be achieved by observing the interference of parity conserving and parity violating two-photon transition amplitudes between energy eigenstates of zero electronic angular momentum. General expressions for induced two-photon transition amplitudes are derived. The signal-to-noise ratio of a two-photon scheme using the 6s^2 1S0 to 6s6p 3P0 transition in ytterbium is estimated.

Atomic tests of discrete symmetries at Berkeley

Recent and ongoing experiments testing various fundamental discrete symmetries are discussed, including search for parity nonconservation in dysprosium and ytterbium, investigation of possibilities of searches for parity and time-reversal invariance violation in samarium, and a test of permutation properties of photons in a two-photon transition in barium.