Dave Kielpinski

Anomalous Fluorescence Enhancement from Double Heterostructure 3D Colloidal Photonic Crystals--A Multifunctional Fluorescence-Based Sensor Platform.

Augmenting fluorescence intensity is of vital importance to the development of chemical and biochemical sensing, imaging and miniature light sources. Here we report an unprecedented fluorescence enhancement with a novel architecture of multilayer three-dimensional colloidal photonic crystals self-assembled from polystyrene spheres. The new technique uses a double heterostructure, which comprises a top and a bottom layer with a periodicity overlapping the excitation wavelength (E) of the emitters, and a middle layer with a periodicity matching the fluorescence wavelength (F) and a thickness that supports constructive interference for the excitation wavelength. This E-F-E double heterostructure displays direction-dependent light trapping for both excitation and fluorescence, coupling the modes of photonic crystal with multiple-beam interference. The E-F-E double heterostructure renders an additional 5-fold enhancement to the extraordinary FL amplification of Rhodamine B in monolithic E CPhCs, and 4.3-fold acceleration of emission dynamics. Such a self-assembled double heterostructue CPhCs may find significant applications in illumination, laser, chemical/biochemical sensing, and solar energy harvesting. We further demonstrate the multi-functionality of the E-F-E double heterostructure CPhCs in Hg (II) sensing.

Efficient generation of >2 W of green light by single-pass frequency doubling in PPMgLN

We report 32% efficient frequency doubling of single-frequency 1029 nm light to green light at 514.5 nm using a single-pass configuration. A congruent composition, periodically poled magnesium-doped lithium niobate (PPMgLN) crystal of 50 mm length was used to generate a second-harmonic power of 2.3 W. To our knowledge, this is the highest reported power and efficiency achieved in the second-harmonic generation of single-frequency green light in a single-pass configuration.

Benchmarking attosecond physics with atomic hydrogen

We have performed the first experiment on the interaction of intense few-cycle laser pulses with atomic hydrogen. Experimental data is compared with an advanced ab initio simulation and agrees quantitatively with simulations at the 10% level.