David R. Carlson

Ultrafast electro-optic light with subcycle control

Making ultrafast cycles of light The ability to generate coherent optical frequency combs has had a huge impact on precision metrology, imaging, and sensing applications. On closer inspection, the broadband “white light” generated through the interaction of femtosecond mode-locked laser pulses is composed of billions or trillions of precisely spaced wavelengths of light. Carlson et al. demonstrate an alternative to the mode-locked laser approach—the electro-optic modulation of a continuous-wave laser light source can also generate optical frequency combs (see the Perspective by Torres-Company). The electro-optic modulation techniques can operate at much higher repetition rates than mode-locked lasers, which means they could potentially yield even more precise measurements. Science, this issue p. 1358; see also p. 1316 Electro-optic modulation of a continuous-wave laser is used to produce ultrafast and ultrastable optical frequency combs. Light sources that are ultrafast and ultrastable enable applications like timing with subfemtosecond precision and control of quantum and classical systems. Mode-locked lasers have often given access to this regime, by using their high pulse energies. We demonstrate an adaptable method for ultrastable control of low-energy femtosecond pulses based on common electro-optic modulation of a continuous-wave laser light source. We show that we can obtain 100-picojoule pulse trains at rates up to 30 gigahertz and demonstrate sub–optical cycle timing precision and useful output spectra spanning the near infrared. Our source enters the few-cycle ultrafast regime without mode locking, and its high speed provides access to nonlinear measurements and rapid transients.

Photonic-Chip Supercontinuum with Tailored Spectra for Counting Optical Frequencies

Supercontinuum generation using chip-integrated photonic waveguides is a powerful approach for spectrally broadening pulsed laser sources with very low pulse energies and compact form factors. When pumped with a mode-locked laser frequency comb, these waveguides can coherently expand the comb spectrum to more than an octave in bandwidth to enable self-referenced stabilization. However, for applications in frequency metrology and precision spectroscopy, it is desirable to not only support self-referencing, but also to generate low-noise combs with customizable broadband spectra. In this work, we demonstrate dispersion-engineered waveguides based on silicon nitride that are designed to meet these goals and enable precision optical metrology experiments across large wavelength spans. We perform a clock comparison measurement and report a clock-limited relative frequency instability of

High-harmonic generation in periodically poled waveguides

3.8\times10^{-15}

On-chip waveguides for self-referencing low-power and high-repetition-rate laser frequency combs

at

Self-referenced frequency combs using high-efficiency silicon-nitride waveguides

\tau = 2

Dual-comb interferometry via repetition rate switching of a single frequency comb

seconds between a 1550 nm cavity-stabilized reference laser and NISTs calcium atomic clock laser at 657 nm using a two-octave waveguide-supercontinuum comb.

Photonic-chip supercontinuum with tailored spectra for precision frequency metrology

Optical waveguides made from periodically poled materials provide high confinement of light and enable the generation of new wavelengths via quasi-phase-matching, making them a key platform for nonlinear optics and photonics. However, such devices are not typically employed for high-harmonic generation. Here, using 200-fs, 10-nJ-level pulses of 4100 nm light at 1 MHz, we generate high harmonics up to the 13th harmonic (315 nm) in a chirped, periodically poled lithium niobate (PPLN) waveguide. Total conversion efficiencies into the visible--ultraviolet region are as high as 10 percent. We find that the output spectrum depends on the waveguide poling period, indicating that quasi-phase-matching plays a significant role. In the future, such periodically poled waveguides may enable compact sources of ultrashort pulses at high repetition rates and provide new methods of probing the electronic structure of solid-state materials.

Ultrabroadband Supercontinuum Generation and Frequency-Comb Stabilization Using On-Chip Waveguides with Both Cubic and Quadratic Nonlinearities

Using silicon nitride and aluminum nitride chip-integrated waveguides, we demonstrate supercontinuum spanning 500-4000 nm. We detect the carrier-envelope-offset frequency using total optical power below 15 mW, or, alternatively, directly from the waveguide output.