David Zueco

Circuit quantum electrodynamics in the ultrastrong-coupling regime

T. Niemczyk, F. Deppe, 2 H. Huebl, E. P. Menzel, F. Hocke, M. J. Schwarz, J. J. Garcia-Ripoll, D. Zueco, T. Hümmer, E. Solano, 7 A. Marx, and R. Gross 2 Walther-Meißner-Institut, Bayerische Akademie der Wissenschaften, D-85748 Garching, Germany∗ Physik-Department, Technische Universität München, D-85748 Garching, Germany Instituto de F́ısica Fundamental, CSIC, Serrano 113-bis, 28006 Madrid, Spain Instituto de Ciencia de Materiales de Aragón y Departamento de F́ısica de la Materia Condensada, CSIC-Universidad de Zaragoza, E-50012 Zaragoza, Spain. Institut für Physik, Universität Augsburg, Universitätsstraße 1, D-86135 Augsburg, Germany Departamento de Qúımica F́ısica, Universidad del Páıs Vasco Euskal Herriko Unibertsitatea, Apdo. 644, 48080 Bilbao, Spain IKERBASQUE, Basque Foundation for Science, Alameda Urquijo 36, 48011 Bilbao, Spain (Dated: December 24, 2010)

Molecular prototypes for spin-based CNOT and SWAP quantum gates

We show that a chemically engineered structural asymmetry in [Tb2] molecular clusters renders the two weakly coupled Tb3+ spin qubits magnetically inequivalent. The magnetic energy level spectrum of these molecules meets then all conditions needed to realize a universal CNOT quantum gate. A proposal to realize a SWAP gate within the same molecule is also discussed. Electronic paramagnetic resonance experiments confirm that CNOT and SWAP transitions are not forbidden.

Bringing Entanglement to the High Temperature Limit

Decoherence due to contact with a hot environment typically restricts quantum phenomena to the low temperature limit, k_{B}T/ℏω≪1 (ℏω is the typical energy of the system). Here we report the existence of a nonequilibrium state for two coupled, parametrically driven, dissipative harmonic oscillators which, contrary to generalized intuition, has stationary entanglement at high temperatures. This clarifies the role of temperature and could lighten the burden on quantum experiments requiring delicate precooling setups.

Modified Ehrenfest Formalism for Efficient Large-Scale ab initio Molecular Dynamics.

We present in detail the recently derived ab initio molecular dynamics (AIMD) formalism [Alonso et al. Phys. Rev. Lett. 2008, 101, 096403], which due to its numerical properties, is ideal for simulating the dynamics of systems containing thousands of atoms. A major drawback of traditional AIMD methods is the necessity to enforce the orthogonalization of the wave functions, which can become the bottleneck for very large systems. Alternatively, one can handle the electron-ion dynamics within the Ehrenfest scheme where no explicit orthogonalization is necessary, however the time step is too small for practical applications. Here we preserve the desirable properties of Ehrenfest in a new scheme that allows for a considerable increase of the time step while keeping the system close to the Born-Oppenheimer surface. We show that the automatically enforced orthogonalization is of fundamental importance for large systems because not only it improves the scaling of the approach with the system size but it also allows for an additional very efficient parallelization level. In this work, we provide the formal details of the new method, describe its implementation, and present some applications to some test systems. Comparisons with the widely used Car-Parrinello molecular dynamics method are made, showing that the new approach is advantageous above a certain number of atoms in the system. The method is not tied to a particular wave function representation, making it suitable for inclusion in any AIMD software package.

Weak and strong coupling regimes in plasmonic QED

We present a quantum theory for the interaction of a two-level emitter with surface plasmon polaritons confined in single-mode waveguide resonators. Based on the Green’s function approach, we develop the conditions for the weak and strong coupling regimes by taking into account the sources of dissipation and decoherence: radiative and nonradiative decays, internal loss processes in the emitter, as well as propagation and leakage losses of the plasmons in the resonator. The theory is supported by numerical calculations for several quantum emitters, GaAs and CdSe quantum dots, and nitrogen vacancy (NV) centers together with different types of resonators constructed of hybrid, cylindrical, or wedge waveguides. We further study the role of temperature and resonator length. Assuming realistic leakage rates, we find the existence of an optimal length at which strong coupling is possible. Our calculations show that the strong coupling regime in plasmonic resonators is accessible within current technology when working at very low temperatures (4 K). In the weak coupling regime, our theory accounts for recent experimental results. By further optimization we find highly enhanced spontaneous emission with Purcell factors over 1000 at room temperature for NV centers. We finally discuss more applications for quantum nonlinear optics and plasmon-plasmon interactions.

Coupling single-molecule magnets to quantum circuits

In this work we study theoretically the coupling of single-molecule magnets (SMMs) to a variety of quantum circuits, including microwave resonators with and without constrictions and flux qubits. The main result of this study is that it is possible to achieve strong and ultrastrong coupling regimes between SMM crystals and the superconducting circuit, with strong hints that such a coupling could also be reached for individual molecules close to constrictions. Building on the resulting coupling strengths and the typical coherence times of these molecules ( µs), we conclude that SMMs can be used for coherent storage and manipulation of quantum information, either in the context of quantum computing or in quantum simulations. Throughout the work we also discuss in detail the family of molecules that are most suitable for such operations, based not only on the coupling strength, but also on the typical energy

Qubit-oscillator dynamics in the dispersive regime: Analytical theory beyond the rotating-wave approximation

We generalize the dispersive theory of the Jaynes-Cummings model beyond the frequently employed rotating-wave approximation (RWA) in the coupling between the two-level system and the resonator. For a detuning sufficiently larger than the qubit-oscillator coupling, we diagonalize the non-RWA Hamiltonian and discuss the differences to the known RWA results. Our results extend the regime in which dispersive qubit readout is possible. If several qubits are coupled to one resonator, an effective qubit-qubit interaction of Ising type emerges, whereas RWA leads to isotropic

Employing circuit QED to measure non-equilibrium work fluctuations

XY

Tunable coupling engineering between superconducting resonators: From sidebands to effective gauge fields

interaction. This impacts on the entanglement characteristics of the qubits.

Scattering in the ultrastrong regime: nonlinear optics with one photon.

We study an interferometric method for measuring the statistics of work performed on a driven quantum system, which has been put forward recently (Dorner et al 2013 Phys. Rev. Lett. 110 230601, Mazzola et al 2013 Phys. Rev. Lett. 110 230602). This method allows the replacement of two projective measurements of the energy of the driven system with qubit tomography of an ancilla that is appropriately coupled to it. We highlight that this method could be employed to obtain the work statistics of closed as well as open driven system, even in the strongly dissipative regime. We then illustrate an implementation of the method in a circuit QED setup, which allows one to experimentally obtain the work statistics of a parametrically driven harmonic oscillator. Our implementation is an extension of the original method, in which two ancilla-qubits are employed and the work statistics are retrieved through two-qubit state tomography. Our simulations demonstrate the experimental feasibility.