E. M. Motoyama

Spin correlations in the electron-doped high-transition-temperature superconductor Nd2- xCexCuO4±δ

High-transition-temperature (high-Tc) superconductivity develops near antiferromagnetic phases, and it is possible that magnetic excitations contribute to the superconducting pairing mechanism. To assess the role of antiferromagnetism, it is essential to understand the doping and temperature dependence of the two-dimensional antiferromagnetic spin correlations. The phase diagram is asymmetric with respect to electron and hole doping, and for the comparatively less-studied electron-doped materials, the antiferromagnetic phase extends much further with doping and appears to overlap with the superconducting phase. The archetypal electron-doped compound Nd2-xCexCuO4±δ (NCCO) shows bulk superconductivity above x ≈ 0.13 (refs 3, 4), while evidence for antiferromagnetic order has been found up to x ≈ 0.17 (refs 2, 5, 6). Here we report inelastic magnetic neutron-scattering measurements that point to the distinct possibility that genuine long-range antiferromagnetism and superconductivity do not coexist. The data reveal a magnetic quantum critical point where superconductivity first appears, consistent with an exotic quantum phase transition between the two phases. We also demonstrate that the pseudogap phenomenon in the electron-doped materials, which is associated with pronounced charge anomalies, arises from a build-up of spin correlations, in agreement with recent theoretical proposals.

A universal relationship between magnetic resonance and superconducting gap in unconventional superconductors

A comprehensive survey of the cuprate, heavy-fermion and iron-based superconductors shows a universal linear relationship between their magnetic resonance energy and superconducting gap. This result suggests that antiferromagnetic fluctuations might have a similar role in the unconventional superconductivity of these seemingly different classes of materials.

Asymmetry of collective excitations in electron- and hole-doped cuprate superconductors

Cuprate superconductors are created by adding electrons or holes to a ‘parent’ compound. They have dissimilar phase diagrams and the asymmetry is further highlighted by unexpected collective modes measured using resonant inelastic X-ray scattering.

Magnetic field effect on the superconducting magnetic gap of Nd1.85Ce0.15CuO4

Inelastic neutron-scattering measurements on the archetypical electron-doped material Nd1.85Ce0.15CuO4 up to a high relative magnetic-field strength, H/H(c2) approximately 50%, reveal a simple linear magnetic-field effect on the superconducting magnetic gap and the absence of field-induced in-gap states. The extrapolated gap-closing field value is consistent with the upper critical field H(c2), and the high-field response resembles that of the paramagnetic normal state.