E. Papandrea

Seeking sprite-induced signatures in remotely sensed middle atmosphere NO2: latitude and time variations

Recent research on sprites shows these and other transient luminous events can exert a local impact on atmospheric chemistry, although with minor effects at global scales. In particular, both modelling and remote sensing work suggest perturbations to the background NOx up to a few tens of per cent can occur above active sprite-producing thunderstorms. In this study we present a detailed investigation of MIPAS/ENVISAT satellite measurements of middle atmospheric NO2 in regions of high likelihood of sprite occurrence during the period August to December 2003. As a proxy of sprite activity we used ground based WWLLN detections of large tropospheric thunderstorms. By investigating the sensitivity of the analysis to the characteristics of the adopted strategy, we confirm the indication of sprite-induced NO2 enhancements of about 10% at 52 km height and tens of per cent at 60 km height immediately after thunderstorm activity, as previously reported by Arnone et al (2008b Geophys. Res. Lett. 35 5807). A further analysis showed the enhancement to be dominated by the contribution from regions north of the Equator (5 ◦ Nt o 20 ◦ N) during the first 30 to 40 days of the sample (i.e. the tail of Northern Hemisphere summer) and in coincidence with low background winds. (Some figures in this article are in colour only in the electronic version)

Two-dimensional tomographic retrieval of MIPAS/ENVISAT measurements of ozone and related species

Observations from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) were analysed with the two-dimensional GMTR retrieval system in order to obtain fields of ozone and several molecular species related to ozone chemistry: HNO3, N2O, NO2, N2O5, ClONO2, COF2, CFC-11 and CFC-12. MIPAS measures mid-infrared emission of the atmosphere both during the day and at night time with global coverage. Observing the atmosphere with limb viewing geometries, the instrument is able to resolve finer vertical structures than with nadir instruments, thus enabling the investigation of ozone height-dependent processes. With the currently planned mission extended up to 2014, MIPAS can provide both short-term resolution and long-term trends needed for studying ozone. The adopted GMTR algorithm permits us to resolve the horizontal inhomogeneities of the atmosphere that are modelled using a two-dimensional discretization of the atmosphere. It is therefore especially suitable for analysing portions of the atmosphere where strong gradients such as at the ozone hole may be poorly reproduced by common horizontal homogeneous one-dimensional retrievals. The adopted strategy is well suited for a refined analysis and a correct monitoring of the ozone recovery, as required by the Montreal Protocol and successive amendments.

Assessment of the horizontal resolution of retrieval products derived from MIPAS observations

We report the results of a study aimed at the assessment of the trade-off between precision and horizontal resolution of the retrieval products of MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) operating onboard the ENVIronmental SATellite. By exploiting different observation setups we could perform the study by acting on both the retrieval and the sampling grids. Our results are compared with those previously obtained on simulated observations [Appl. Opt. 43, 1-11 (2004)]. We show that the horizontal sampling of the atmosphere operated by the spectrometer cannot be pushed beyond some limits without inducing unacceptable correlations among the retrieved profiles. These correlations show-up only when using a two-dimensional retrieval algorithm and can be evaluated through the instabilities that they trigger in the horizontal distribution of the retrieval products. In order to reduce these instabilities we compare the strategy of degrading the retrieval grid with the strategy of applying horizontal regularization. We discuss the different trade-off between precision and spatial resolution connected with the two strategies. The method adopted in this study, is applicable to any orbiting limb sounder measuring along the orbit track.

Retrieving cloud geometrical extents from MIPAS/ENVISAT measurements with a 2-D tomographic approach

Clouds represent a critical factor in regulating the Earths atmosphere and its energy balance. Satellite instruments can measure the energy balance and global atmospheric properties only through an accurate knowledge of the vertical profile of cloudiness, which is as yet one of the key shortages in atmospheric science. The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on-board the ENVISAT satellite, designed to infer the amount of atmospheric trace-gases, demonstrated also sensitivity to the radiation emitted from clouds. In order to model the effect of the geometrical extent of a cloud on MIPAS measurements, we developed a retrieval model capable to simulate cloud effects on broad spectral intervals accounting for the two-dimensional (2-D) variability of the atmosphere in the satellite orbit plane. The 2-D analysis revealed a sensitivity of MIPAS spectra to both the vertical and horizontal extents and the position of clouds along the instrument line of sight. One-dimensional models were found to underestimate Cloud Top Height (CTH) by approximating clouds as an infinite horizontal layer with a finite vertical extents. With the 2-D approach, we showed it is possible, for optically thin Polar Stratospheric Clouds (PSCs), to retrieve both CTH and horizontal dimension by analyzing simultaneously all the limb observations that come across the cloud with their field of view. For a selected case study we found a very good agreement for both PSC CTH and horizontal extents retrieved from MIPAS measurements and those retrieved from coincident CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarisation) measurements.

OCCUR—Study of the Chemistry−Climate Coupling in the UTLS Region with Satellite Measurements

This study, performed in the frame of the Changing Earth Science Network initiative, aims at investigating in particular the Upper Troposphere-Lower Stratosphere (UTLS) region with measurements acquired from satellite instruments and the aid of a chemical transport model. It is related to the “Challenge 4 of the Atmosphere” of the ESA Living Planet Program. The Challenge 4 addresses the following topic: Observe, monitor and understand the chemistry-dynamics coupling of the stratospheric and upper tropospheric circulations, and the apparent changes in these circulations. To contribute to this scientific challenge this study investigated the stratosphere and the UTLS region through the analysis of satellite observations using a tomographic approach, capable to take into account inhomogeneities of the atmosphere’s constituents. In this context, evidence of non-physical day-night differences in 1D retrievals has been found in a previous study performed on MIPAS spectra. These differences almost disappear using a tomographic approach, confirming that a 2D retrieval describes a more realistic picture of the atmosphere. These evidences have been confirmed with a 2D retrieval algorithm that has been expressly set up to analyse SCIAMACHY observations. The results of the study have also provided a new scientific understanding and support the definition of requirements for future Earth Explorers missions (i.e. an advanced imaging MIPAS spectrometer such as PREMIER).