E. Pelucchi

Growth and characterization of single quantum dots emitting at 1300 nm

We have optimized the molecular-beam epitaxy growth conditions of self-organized InAs∕GaAs quantum dots (QDs) to achieve a low density of dots emitting at 1300 nm at low temperature. We used an ultralow InAs growth rate, lower than 0.002ML∕s, to reduce the density to 2dots∕μm2 and an InGaAs capping layer to achieve longer emission wavelength. Microphotoluminescence spectroscopy at low-temperature reveals emission lines characteristic of exciton-biexciton behavior. We also study the temperature dependence of the photoluminescence, showing clear single QD emission up to 90 K. With these results, InAs∕GaAs QDs appear as a very promising system for future applications of single photon sources in fiber-based quantum cryptography.

Towards quantum-dot arrays of entangled photon emitters

An array of pyramidal site-controlled InGaAs1−δNδ quantum dots is grown on a GaAs substrate to reduce the fine-structure splitting of the intermediate single-exciton energy levels to less than 4 μeV. The quantum dots emit polarization-entangled photons at a maximum fidelity of 0.721 ± 0.043 without external manipulation of the electronic states.

Probing carrier dynamics in nanostructures by picosecond cathodoluminescence

Picosecond and femtosecond spectroscopy allow the detailed study of carrier dynamics in nanostructured materials. In such experiments, a laser pulse normally excites several nanostructures at once. However, spectroscopic information may also be acquired using pulses from an electron beam in a modern electron microscope, exploiting a phenomenon called cathodoluminescence. This approach offers several advantages. The multimode imaging capabilities of the electron microscope enable the correlation of optical properties (via cathodoluminescence) with surface morphology (secondary electron mode) at the nanometre scale. The broad energy range of the electrons can excite wide-bandgap materials, such as diamond- or gallium-nitride-based structures that are not easily excited by conventional optical means. But perhaps most intriguingly, the small beam can probe a single selected nanostructure. Here we apply an original time-resolved cathodoluminescence set-up to describe carrier dynamics within single gallium-arsenide-based pyramidal nanostructures with a time resolution of 10 picoseconds and a spatial resolution of 50 nanometres. The behaviour of such charge carriers could be useful for evaluating elementary components in quantum computers, optical quantum gates or single photon sources for quantum cryptography.

Single photon emission from site-controlled pyramidal quantum dots

We demonstrate that a single photoexcited InGaAs semiconductor quantum dot (QD) grown by organo-metallic chemical vapor deposition on prepatterned substrates emits one photon at a time, with no uncontrolled background photon emission, making it an excellent single photon emitter. Moreover, our fabrication technique offers complete site control and small inhomogeneous broadening of QD arrays, which is essential for the practical implementation of QDs in efficient solid-state single photon emitting devices.

High Uniformity of Site-Controlled Pyramidal Quantum Dots Grown on Prepatterned Substrates

We studied the uniformity of site-controlled, pyramidal InGaAs/AlGaAs semiconductor quantum dots (QDs) grown by organometallic chemical vapor deposition on prepatterned substrates. The inhomogeneous broadening of the QD ground state emission has been determined to be 7.6 meV by statistical single QD photoluminescence spectroscopy on a set of 120 individual QD structures. Taking into account the ground-to-excited state separation of 55 meV, such a small value has not yet been observed in QD systems where other growth mechanisms are employed. Moreover, a high reproducibility of the sharp QD emission features in the single exciton regime has been observed.

A site-controlled quantum dot system offering both high uniformity and spectral purity

In this letter we report on the optical properties of site-controlled InGaAs quantum dots with GaAs barriers grown in pyramidal recesses by metalorganic vapor phase epitaxy. The inhomogeneous broadening of excitonic emission from an ensemble of quantum dots is found to be unusually narrow, with a standard deviation of 1.19 meV and the spectral purity of emission lines from individual dots is found to be very high (18–30 μeV), in contrast with other site-controlled dot systems.

Dense uniform arrays of site-controlled quantum dots grown in inverted pyramids

We report on the growth and optical properties of homogeneous, dense arrays of site-controlled, single GaAs/AlGaAs quantum dot (QD) heterostructures with periodicities as small as 300 nm. The samples were grown by organometallic chemical vapor deposition on (111)B GaAs substrates containing dense inverted pyramid recess patterns prepared by electron beam lithography and wet chemical etching. Low-temperature microphotoluminescence spectra of the samples show distinct luminescence from the QDs with 1–3 meV linewidth. Low-temperature cathodoluminescence spectrally resolved images reveal uniform emission energy within an ensemble of 900 QDs.

Optical polarization anisotropy and hole states in pyramidal quantum dots

The authors present a polarization-resolved photoluminescence study of single semiconductor quantum dots (QDs) interconnected to quantum wires, measured both in a top geometry, and in a less conventional cleaved-edge geometry. Strong polarization anisotropy is revealed for all observed transitions, and it is deduced that closely spaced QD hole states exhibit nearly pure heavy-or light-hole character. These effects are attributed to the large aspect ratio of the dot shape.

Decomposition, diffusion, and growth rate anisotropies in self-limited profiles during metalorganic vapor-phase epitaxy of seeded nanostructures

We present a model for the interplay between the fundamental phenomena responsible for the formation of nanostructures by metalorganic vapor phase epitaxy on patterned (001)/(111)B GaAs substrates. Experiments have demonstrated that V-groove quantum wires and pyramidal quantum dots form as a consequence of a self-limiting profile that develops, respectively, at the bottom of V-grooves and inverted pyramids. Our model is based on a system of reaction-diffusion equations, one for each crystallographic facet that defines the pattern, and include the group III precursors, their decomposition and diffusion kinetics (for which we discuss the experimental evidence), and the subsequent diffusion and incorporation kinetics of the group-III atoms released by the precursors. This approach can be applied to any facet configuration, including pyramidal quantum dots, but we focus on the particular case of V-groove templates and offer an explanation for the self-limited profile and the Ga segregation observed in the V-groove. The explicit inclusion of the precursor decomposition kinetics and the diffusion of the atomic species revises and generalizes the earlier work of Biasiol et al. [Biasiol et al., Phys.Rev. Lett. 81, 2962 (1998); Phys. Rev. B 65, 205306 (2002)] and is shown to be essential for obtaining a complete description of self-limiting growth. The solution of the system of equations yields spatially resolved adatom concentrations, from which average facet growth rates are calculated. This provides the basis for determining the conditions that yield self-limiting growth. The foregoing scenario, previously used to account for the growth modes of vicinal GaAs(001) and the step-edge profiles on the ridges of vicinal surfaces patterned with V-grooves during metalorganic vapor-phase epitaxy, can be used to describe the morphological evolution of any template composed of distinct facets.

Luttinger-liquid behavior in weakly disordered quantum wires

We have measured the temperature dependence of the conductance in long V-groove quantum wires fabricated in GaAs/AlGaAs heterostructures. Our data are consistent with recent theories developed within the framework of the Luttinger-liquid model, in the limit of weakly disordered wires. We show that, for the relatively low level of disorder in our quantum wires, the value of the interaction parameter g congruent with 0.66, which is the expected value for GaAs. However, samples with a higher level of disorder show conductance with stronger temperature dependence, which does not allow their treatment in the framework of perturbation theory. Fitting such data with perturbation-theory models leads inevitably to wrong (lower) values of g.