Eider Berganza

Quantitative Nanoscale Magnetic Study of Isolated Diameter-Modulated FeCoCu Nanowires

The comprehension of the magnetic configuration in FeCoCu nanowires with a diameter-modulated cylindrical geometry will allow controlling the domain wall motion in this low-dimensional system under the application of magnetic fields and/or the injection of current pulses. Here we perform a quantitative magnetic characterization of isolated diameter-modulated FeCoCu nanowires by combining nanoscale magnetic characterization techniques such as electron holography, magnetic force microscopy, and micromagnetic simulations. Local reconstructions of the magnetic distribution show the diameter-modulated geometry of the wires induces the formation of vortex-like structures and magnetic charges in the regions where the diameter is varied. Vortex-like structures modify the axial alignment of the magnetization in large-diameter segments. Moreover, the magnetic charges control the demagnetizing field distribution, promoting a flux-closure stray field configuration around large-diameter segments and keeping the demagnetizing field parallel to the NWs magnetization around small diameter segments. The detailed description of the remanent state in diameter-modulated cylindrical FeCoCu nanowires allows us to provide a clear explanation of the origin of bright and dark contrast observed in magnetic force microscopy images, which have the same feature of magnetic domain walls. This work establishes the primary knowledge required for future magnetization reversal studies with the aim of searching efficient modulated geometries that allow an optimum and controlled domain wall propagation.

Spin configuration of cylindrical bamboo-like magnetic nanowires

The surface and the internal magnetic structure of bamboo-like cylindrical nanowires with tailored diameter modulations have been determined exploiting the direct photoemission and transmission contrasts using photoemission electron microscopy combined with X-ray magnetic circular dichroism, as well as complementary magnetic force microscopy and micromagnetic simulations. Bamboo-like cylindrical nanowires with diameters of 130 and 140 nm, and a modulation periodicity of 400 nm were electrochemically grown into the pores of alumina templates. FeCoCu and Co nanowires were selected to offer parallel and perpendicular magnetization easy axis, respectively. For FeCoCu nanowires, a main longitudinal magnetization configuration is found consistent with the predominant shape anisotropy. In addition, a weaker modulated contrast along the wires’ axis is observed that matches the position of each diameter modulation: vortex-like structures are observed at the ends of the wires and at the surface around the modulations. In Co nanowires, a multi-segmented vortex-like structure with alternating opposite chirality is found not matching the periodicity of the diameter modulations. Such a spin configuration is interpreted considering that Co nanowires exhibit hexagonal symmetry with c axis nearly perpendicular to the nanowires defining strong uniaxial transverse magnetocrystalline anisotropy.

Spin configuration in isolated FeCoCu nanowires modulated in diameter.

Cylindrical Fe28Co67Cu5 nanowires modulated in diameter between 22 and 35 nm are synthesized by electroplating into the nanopores of alumina membranes. High-sensitivity MFM imaging (with a detection noise of 1 μN m(-1)) reveals the presence of single-domain structures in remanence with strong contrast at the ends of the nanowires, as well as at the transition regions where the diameter is modulated. Micromagnetic simulations suggest that curling of the magnetization takes place at these transition sites, extending over 10-20 nm and giving rise to stray fields measurable with our MFM. An additional weaker contrast is imaged, which is interpreted to arise from inhomogeneities in the nanowire diameter.

Domain wall pinning in FeCoCu bamboo-like nanowires

The three dimensional nature of cylindrical magnetic nanowires has opened a new way to control the domain configuration as well as the magnetization reversal process. The pinning effect of the periodic diameter modulations on the domain wall propagation in FeCoCu individual nanowires is determined by Magnetic Force Microscopy, MFM. A main bistable magnetic configuration is firstly concluded from MFM images characterized by the spin reversal between two nearly single domain states with opposite axial magnetization. Complementary micromagnetic simulations confirm a vortex mediated magnetization reversal process. A non-standard variable field MFM imaging procedure allows us to observe metastable magnetic states where the propagating domain wall is pinned at certain positions with enlarged diameter. Moreover, it is demonstrated that it is possible to control the position of the pinned domain walls by an external magnetic field.

Customized MFM probes with high lateral resolution

Summary Magnetic force microscopy (MFM) is a widely used technique for magnetic imaging. Besides its advantages such as the high spatial resolution and the easy use in the characterization of relevant applied materials, the main handicaps of the technique are the lack of control over the tip stray field and poor lateral resolution when working under standard conditions. In this work, we present a convenient route to prepare high-performance MFM probes with sub-10 nm (sub-25 nm) topographic (magnetic) lateral resolution by following an easy and quick low-cost approach. This allows one to not only customize the tip stray field, avoiding tip-induced changes in the sample magnetization, but also to optimize MFM imaging in vacuum (or liquid media) by choosing tips mounted on hard (or soft) cantilevers, a technology that is currently not available on the market.

Direct observation of transverse and vortex metastable magnetic domains in cylindrical nanowires

The study has been performed under the framework of the Projects No. MAT2013-48054-C2-1-R, MAT2016-76824-C3-1-R, MAT-2015-68772-P, MAT2015-64110-C2-2-P supported by the MINECO from Spain and DURSI 2014SGR220 supported by the Catalan Government. J.A.F.-R. acknowledges financial support from MINECO and the ESF through the “Ayudas para contratos predoctorales para la formacion de doctores 2014.”

Multisegmented Nanowires: a Step towards the Control of the Domain Wall Configuration

Cylindrical nanowires synthesized by controlled electrodeposition constitute excellent strategic candidates to engineer magnetic domain configurations. In this work, multisegmented CoNi/Ni nanowires are synthesized for tailoring a periodic magnetic structure determined by the balance between magnetocrystalline and magnetostatic energies. High-resolution Transmission Electron Microscopy confirms the segmented growth and the sharp transition between layers. Although both CoNi and Ni segments have similar fcc cubic crystal symmetry, their magnetic configuration is quite different as experimentally revealed by Magnetic Force Microscopy (MFM) imaging. While the Ni segments are single domain with axial magnetization direction, the CoNi segments present two main configurations: a single vortex state or a complex multivortex magnetic configuration, which is further interpreted with the help of micromagnetic simulations. This original outcome is ascribed to the tight competition between anisotropies. The almost monocrystalline fcc structure of the CoNi segments, as revealed by the electron diffraction patterns, which is atypical for its composition, contributes to balance the magnetocrystalline and shape anisotropies. The results of MFM measurements performed under in-plane magnetic field demonstrate that it is possible to switch from the multivortex configuration to a single vortex configuration with low magnetic fields.

Magnetization Ratchet in Cylindrical Nanowires

The unidirectional motion of information carriers such as domain walls in magnetic nanostrips is a key feature for many future spintronic applications based on shift registers. This magnetic ratchet effect has so far been achieved in a limited number of complex nanomagnetic structures, for example, by lithographically engineered pinning sites. Here we report on a simple remagnetization ratchet originated in the asymmetric potential from the designed increasing lengths of magnetostatically coupled ferromagnetic segments in FeCo/Cu cylindrical nanowires. The magnetization reversal in neighboring segments propagates sequentially in steps starting from the shorter segments, irrespective of the applied field direction. This natural and efficient ratchet offers alternatives for the design of three-dimensional advanced storage and logic devices.