Eric Plum

Metamaterial with negative index due to chirality

Artificial magnetism, negative permeability and negative refractive index are demonstrated in 3D-chiral metamaterial that shows giant polarization rotation and circular dichroism. ∗ As presented at the Quantum Electronics and Laser Sciences Conference (CLEO/QELS 2008), San Jose, CA, USA, 5 May 2008, paper QMA4.

Giant optical gyrotropy due to electromagnetic coupling

The authors demonstrate a chiral photonic metamaterial with chirality provided by electromagnetic coupling between mutually twisted unconnected layers. In the visible and near-IR spectral ranges, the material exhibits polarization rotatory power of up to 2500°/mm and shows relatively low losses and negligible circular dichroism, making it a promising candidate for the development of chiral negative index media.

Terahertz metamaterial with asymmetric transmission

We show that a planar metamaterial, an array of coupled metal split-ring resonators with a unit cell lacking mirror symmetry, exhibits asymmetric transmission of terahertz radiation (0.25-2.5 THz) propagating through it in opposite directions. This intriguing effect, that is compatible with Lorentz reciprocity and time-reversal, depends on a directional difference in conversion efficiency of the incident circularly polarized wave into one of opposite handedness, that is only possible in lossy low-symmetry planar chiral metamaterials. We show that asymmetric transmission is linked to excitation of enantiomerically sensitive plasmons, these are induced charge-field excitations that depend on the mutual handedness of incident wave and metamaterial pattern. Various bands of positive, negative and zero phase and group velocities have been identified indicating the opportunity to develop polarization sensitive negative index and slow light media based on such metamaterials.

Reconfigurable photonic metamaterials

We demonstrate the first temperature driven mechanically reconfigurable photonic metamaterials (RPMs) providing tunability at optical frequencies.

An electromechanically reconfigurable plasmonic metamaterial operating in the near-infrared

Current efforts in metamaterials research focus on attaining dynamic functionalities such as tunability, switching and modulation of electromagnetic waves. To this end, various approaches have emerged, including embedded varactors, phase-change media, the use of liquid crystals, electrical modulation with graphene and superconductors, and carrier injection or depletion in semiconductor substrates. However, tuning, switching and modulating metamaterial properties in the visible and near-infrared range remain major technological challenges: indeed, the existing microelectromechanical solutions used for the sub-terahertz and terahertz regimes cannot be shrunk by two to three orders of magnitude to enter the optical spectral range. Here, we develop a new type of metamaterial operating in the optical part of the spectrum that is three orders of magnitude faster than previously reported electrically reconfigurable metamaterials. The metamaterial is actuated by electrostatic forces arising from the application of only a few volts to its nanoscale building blocks-the plasmonic metamolecules-that are supported by pairs of parallel strings cut from a flexible silicon nitride membrane of nanoscale thickness. These strings, of picogram mass, can be driven synchronously to megahertz frequencies to electromechanically reconfigure the metamolecules and dramatically change the transmission and reflection spectra of the metamaterial. The metamaterials colossal electro-optical response (on the order of 10(-5)-10(-6) m V(-1)) allows for either fast continuous tuning of its optical properties (up to 8% optical signal modulation at up to megahertz rates) or high-contrast irreversible switching in a device only 100 nm thick, without the need for external polarizers and analysers.

Multifold Enhancement of Quantum Dot Luminescence in Plasmonic Metamaterials

We report that hybridizing semiconductor quantum dots with plasmonic metamaterial leads to a multifold intensity increase and narrowing of their photoluminescence spectrum. The luminescence enhancement is a clear manifestation of the cavity quantum electrodynamics Purcell effect and can be controlled by the metamaterials design. This observation is an essential step towards understanding loss compensation in plasmonic metamaterials with gain media and for developing metamaterial-enhanced gain media.

Towards the lasing spaser: controlling metamaterial optical response with semiconductor quantum dots

We report the first experimental demonstration of compensating Joule losses in metallic photonic metamaterial using optically pumped PbS semiconductor quantum dots.

Optical activity in extrinsically chiral metamaterial

We demonstrate optical activity in an intrinsically non-chiral anisotropic planar metamaterial. The phenomenon is due to extrinsic chirality resulting from the mutual orientation of the metamaterial structure and the incident electromagnetic wave. The polarization effect, which has a resonant nature, features a spectral band where linear birefringence is practically absent and can be easily tuned by tilting the plane of the metamaterial relative to the incident beam.

Giant nonlinear optical activity in a plasmonic metamaterial

In 1950, a quarter of a century after his first-ever nonlinear optical experiment when intensity-dependent absorption was observed in uranium-doped glass, Sergey Vavilov predicted that birefringence, dichroism and polarization rotatory power should be dependent on light intensity. It required the invention of the laser to observe the barely detectable effect of light intensity on the polarization rotatory power of the optically active lithium iodate crystal, the phenomenon now known as the nonlinear optical activity, a high-intensity counterpart of the fundamental optical effect of polarization rotation in chiral media. Here we report that a plasmonic metamaterial exhibits nonlinear optical activity 30 million times stronger than lithium iodate crystals, thus transforming this fundamental phenomenon of polarization nonlinear optics from an esoteric phenomenon into a major effect of nonlinear plasmonics with potential for practical applications.

Reconfigurable nanomechanical photonic metamaterials

The changing balance of forces at the nanoscale offers the opportunity to develop a new generation of spatially reconfigurable nanomembrane metamaterials in which electromagnetic Coulomb, Lorentz and Ampère forces, as well as thermal stimulation and optical signals, can be engaged to dynamically change their optical properties. Individual building blocks of such metamaterials, the metamolecules, and their arrays fabricated on elastic dielectric membranes can be reconfigured to achieve optical modulation at high frequencies, potentially reaching the gigahertz range. Mechanical and optical resonances enhance the magnitude of actuation and optical response within these nanostructures, which can be driven by electric signals of only a few volts or optical signals with power of only a few milliwatts. We envisage switchable, electro-optical, magneto-optical and nonlinear metamaterials that are compact and silicon-nanofabrication-technology compatible with functionalities surpassing those of natural media by orders of magnitude in some key design parameters.