F Di Pompeo

Effects of Nitrogen contamination in liquid Argon

A dedicated test of the effects of Nitrogen contamination in liquid Argon has been performed at the INFN-Gran Sasso Laboratory (LNGS, Italy) within the WArP R&D program. A detector has been designed and assembled for this specific task and connected to a system for the injection of controlled amounts of gaseous Nitrogen into the liquid Argon. The purpose of the test is to detect the reduction of the Ar scintillation light emission as a function of the amount of the Nitrogen contaminant injected in the Argon volume. A wide concentration range, spanning from ~ 10?1 ppm up to ~ 103 ppm, has been explored. Measurements have been done with electrons in the energy range of minimum ionizing particles (?-conversion from radioactive sources). Source spectra at different Nitrogen contaminations are analyzed, showing sensitive reduction of the scintillation yield at increasing concentrations. Direct PMT signal acquisition exploiting high time resolution by fast waveform recording allowed high precision extraction of the main characteristics of the scintillation light emission in contaminated LAr. In particular, the decreasing behavior in lifetime and relative amplitude of the slow component is found to be appreciable starting from (1 ppm) of Nitrogen concentrations. The rate constant of the quenching process induced by Nitrogen in liquid Ar has been found to be kQ(N2) = 0.11 ? 0.01 ?s?1ppm?1, consistent with a previous measurement of this quantity but with significant improvement in precision. On the other hand, no evidence for absorption by N2 impurities has been found up to the higher concentrations here explored.

Oxygen contamination in liquid Argon: combined effects on ionization electron charge and scintillation light

A dedicated test of the effects of Oxygen contamination in liquid Argon has been performed at the INFN-Gran Sasso Laboratory (LNGS, Italy) within the WArP R&D program. Two detectors have been used: the WArP2.3 lt prototype and a small (0.7 lt) dedicated detector, coupled with a system for the injection of controlled amounts of gaseous Oxygen. O2 contamination in LAr leads to depletion of both the free electron charge (via attachment process) and the scintillation light (via quenching and absorption mechanisms) available for ionization signal detection. Purpose of the test with the 0.7 lt detector was to detect the reduction of the long-lived component lifetime of the Argon scintillation light emission and of the overall light yield at increasing O2 concentration. Data from the WArP prototype were used for determining the behavior of both the ionization electron lifetime and the scintillation long-lived component lifetime at decreasing O2 concentration by the purification process activated in closed loop during the acquisition run. The electron lifetime measurements allowed to infer the O2 content of the Argon and correlate it with the long-lived scintillation lifetime data. The effects of Oxygen contamination on the scintillation light have been thus extensively measured over a wide range of O2 concentration, spanning from ~ 10−3 ppm up to ~ 10 ppm.

Demonstration and comparison of photomultiplier tubes at liquid Argon temperature

Liquified noble gases are widely used as a target in direct Dark Matter searches. Signals from scintillation in the liquid, following energy deposition from the recoil nuclei scattered by Dark Matter particles (e.g. WIMPs), should be recorded down to very low energies by photosensors suitably designed to operate at cryogenic temperatures. Liquid Argon based detectors for Dark Matter searches currently implement photo multiplier tubes for signal read-out. In the last few years PMTs with photocathodes operating down to liquid Argon temperatures (87 K) have been specially developed with increasing Quantum Efficiency characteristics. The most recent of these, Hamamatsu Photonics Mod. R11065 with peak QE up to about 35%, has been extensively tested within the R&D program of the WArP Collaboration. During these testes the Hamamatsu PMTs showed superb performance and allowed obtaining a light yield around 7 phel/keVee in a Liquid Argon detector with a photocathodic coverage in the 12% range, sufficient for detection of events down to few keVee of energy deposition. This shows that this new type of PMT is suited for experimental applications, in particular for new direct Dark Matter searches with LAr-based experiments.

VUV-Vis optical characterization of Tetraphenyl-butadiene films on glass and specular reflector substrates from room to liquid Argon temperature

The use of efficient wavelength-shifters from the vacuum-ultraviolet to the photo-sensors range of sensitivity is a key feature in detectors for Dark Matter search and neutrino physics based on liquid argon scintillation detection. Thin film of Tetraphenyl-butadiene (TPB) deposited onto the surface delimiting the active volume of the detector and/or onto the photosensor optical window is the most common solution in current and planned experiments. Detector design and response can be evaluated and correctly simulated only when the properties of the optical system in use (TPB film + substrate) are fully understood. Characterization of the optical system requires specific, sometimes sophisticated optical methodologies. In this paper the main features of TPB coatings on different, commonly used substrates is reported, as a result of two independent campaigns of measurements at the specialized optical metrology labs of ENEA and University of Tor Vergata. Measured features include TPB emission spectra with lineshape and relative intensity variation recorded as a function of the film thickness and for the first time down to LAr temperature, as well as optical reflectance and transmittance spectra of the TPB coated substrates in the wavelength range of the TPB emission.

The WArP experiment

Cryogenic noble liquid detectors are presently considered one of the best options for WIMP Dark Matter searches, especially when extensions to multi ton scale sensitive masses are foreseen. The WArP experiment is the first one that exploits the unique characteristics of liquid Argon to make a highly sensitive search for WIMP Dark Matter candidates. In 2008, a double phase detector has been assembled in the Gran Sasso National Laboratory with 140 kg sensitive mass and a discovery potential in the range of 5 × 10−45 cm2 in the spin-independent WIMP-nucleon cross-section. In addition to standard neutrons and gamma-rays passive shields, WArP implements an 8 ton liquid Argon active shield with 4π coverage. The detector was commissioned and put into operation during the first half of 2009 for a first technical run. This first run lasted about three months and then it was stopped for some detector repairs and modifications in the summer of 2009. A second run was started at the beginning of 2010. Detector design, construction and assembly are described, together with the results of the technical run and the very first results of the 2010 run.

Tetraphenyl-butadiene films: VUV-Vis optical characterization from room to liquid argon temperature

A thin film of Tetraphenyl-butadiene (TPB) deposited onto the surface delimiting the active volume of the detector and/or onto the photosensors optical window is the most common solution to down convert argon VUV scintillation light in current and planned liquid argon based experiments for dark matter searches and neutrino physics. Characterization of the main features of TPB coatings on different, commonly used substrates is reported, as a result of measurements at the specialized optical metrology labs of ENEA and University of Tor Vergata. Measured features include TPB emission spectra with lineshape and relative intensity variation recorded as a function of the film thickness and for the first time down to LAr temperature, as well as optical reflectance and transmittance spectra of the TPB coated substrates in the wavelength range of the TPB emission.

Discovery of underground argon with a low level of radioactive 39Ar and possible applications to WIMP dark matter detectors

We report on the first measurement of 39Ar in argon from underground natural gas reservoirs. The gas stored in the US National Helium Reserve was found to contain a low level of 39Ar. The ratio of 39Ar to stable argon was found to be ≤4×10-17 (84% C.L.), less than 5% the value in atmospheric argon (39Ar/Ar=8×10-16). The total quantity of argon currently stored in the National Helium Reserve is estimated at 1000 tons. 39Ar represents one of the most important backgrounds in argon detectors for WIMP dark matter searches. The findings reported demonstrate the possibility of constructing large multi-ton argon detectors with low radioactivity suitable for WIMP dark matter searches.