F. Fras

Effects of Spin-Dependent Interactions on Polarization of Bright Polariton Solitons

We report on the spin properties of bright polariton solitons supported by an external pump to compensate losses. We observe robust circularly polarized solitons when a circularly polarized pump is applied, a result attributed to phase synchronization between nondegenerate TE and TM polarized polariton modes at high momenta. For the case of a linearly polarized pump, either σ+ or σ- circularly polarized bright solitons can be switched on in a controlled way by a σ+ or σ- writing beam, respectively. This feature arises directly from the widely differing interaction strengths between co- and cross-circularly polarized polaritons. In the case of orthogonally linearly polarized pump and writing beams, the soliton emission on average is found to be unpolarized, suggesting strong spatial evolution of the soliton polarization. The observed results are in agreement with theory, which predicts stable circularly polarized solitons and unstable linearly polarized solitons.

Strong exciton-photon coupling in open semiconductor microcavities

We present a method to implement 3-dimensional polariton confinement with in-situ spectral tuning of the cavity mode. Our tunable microcavity is a hybrid system consisting of a bottom semiconductor distributed Bragg reflector (DBR) with a cavity containing quantum wells (QWs) grown on top and a dielectric concave DBR separated by a micrometer sized gap. Nanopositioners allow independent positioning of the two mirrors and the cavity mode energy can be tuned by controlling the distance between them. When close to resonance, we observe a characteristic anticrossing between the cavity modes and the QW exciton demonstrating strong coupling. For the smallest radii of curvature concave mirrors of 5.6 μm and 7.5 μm, real-space polariton imaging reveals submicron polariton confinement due to the hemispherical cavity geometry.

Spin Textures of Exciton-Polaritons in a Tunable Microcavity with Large TE-TM Splitting.

We report an extended family of spin textures of zero-dimensional exciton-polaritons spatially confined in tunable open microcavity structures. The transverse-electric-transverse-magnetic (TE-TM) splitting, which is enhanced in the open cavity structures, leads to polariton eigenstates carrying quantized spin vortices. Depending on the strength and anisotropy of the cavity confining potential and of the TE-TM induced splitting, which can be tuned via the excitonic or photonic fractions, the exciton-polariton emissions exhibit either spin-vortex-like patterns or linear polarization, in good agreement with theoretical modeling.S. Dufferwiel, Feng Li, ∗ E. Cancellieri, L. Giriunas, A. A. P. Trichet, D. M. Whittaker, P. M. Walker, F. Fras, 3 E. Clarke, J. M. Smith, M. S. Skolnick, and D. N. Krizhanovskii † Department of Physics and Astronomy, University of Sheffield, Sheffield S3 7RH, UK Department of Materials, University of Oxford, Parks Road, Oxford OX1 3PH, UK IPCMS UMR 7504, CNRS and Université de Strasbourg, 67200 Strasbourg, France EPSRC National Centre for III-V Technologies, University of Sheffield, Sheffield S1 3JD, UK (Dated: April 10, 2015)

Effect of polariton-polariton interactions on the excitation spectrum of a nonequilibrium condensate in a periodic potential

Polariton condensates are investigated in periodical potentials created by surface acoustic waves (SAWs) using both coherent and incoherent optical excitation. Under coherent resonant pumping, condensates are formed due to polariton-parametric scattering from the pump. In this case, the excitation spectrum of the condensate shows a strong reduction of the energy gap arising from the acoustic modulation, indicating efficient screening of the SAW potential by spatial modulation of the polariton density. The observed results are in good agreement with a model based on generalized Gross-Pitaveskii equations, with account taken of the spatial dependence of the exciton energy landscape. In the case of incoherent pumping, coexisting nonequilibrium condensates with s -a nd p-type wavefunctions are observed, which have different energies, symmetry, and spatial coherence. The energy splitting between these condensate states is also reduced with respect to the gap of the one particle spectrum below threshold, but the screening effect is less pronounced than in the case of coherently pumped system due to weaker modulation of the pump state. DOI: 10.1103/PhysRevB.87.155423

Multi-wave coherent control of a solid-state single emitter

Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton transitions in semiconductor quantum dots (QDs) is less advanced, principally due to the sub-nanosecond dephasing. Conversely, owing to their robust coupling to light, one can apply tools of nonlinear spectroscopy to achieve all-optical command. Here, we report on the coherent manipulation of an exciton via multi-wave mixing. Specifically, we employ three resonant pulses driving a single InAs QD. The first two induce a four-wave mixing (FWM) transient, which is projected onto a six-wave mixing (SWM) depending on the delay and area of the third pulse, in agreement with analytical predictions. Such a switch enables to demonstrate the generation of SWM on a single emitter and to engineer the spectro-temporal shape of the coherent response originating from a TLS. These results pave the way toward multi-pulse manipulations of solid state qubits via implementing the NMR-like control schemes in the optical domain.

Giant light-harvesting nanoantenna for single-molecule detection in ambient light

Here, we explore the enhancement of single-molecule emission by a polymeric nanoantenna that can harvest energy from thousands of donor dyes to a single acceptor. In this nanoantenna, the cationic dyes are brought together, in very close proximity, using bulky counterions, thus enabling ultrafast diffusion of excitation energy (≤30 fs) with minimal losses. Our 60 nm nanoparticles containing >10,000 rhodamine-based donor dyes can efficiently transfer energy to 1–2 acceptors, resulting in an antenna effect of ~1,000. Therefore, single Cy5-based acceptors become 25-fold brighter than quantum dots QD655. This unprecedented amplification of the acceptor dye emission enables observation of single molecules at illumination powers (1–10 mW cm−2) that are >10,000-fold lower than typically required in single-molecule measurements. Finally, using a basic set-up, which includes a ×20 air objective and a scalable complementary metal-oxide–semiconductor camera, we could detect single Cy5 molecules by simply shining divergent light on the sample at powers equivalent to sunlight.Donor dye nanoparticles have been used to realize structures that are 25 times brighter than quantum dots. This enabled single-molecule imaging using ambient light.

Electron and hole spin cooling efficiency in InAs quantum dots: The role of nuclear field

The spin dynamics of a resident carrier, hole or electron, in singly charged InAs/GaAs quantum dots has been measured by pump-probe experiments. The relative strength of the hole to the electron hyperfine couplings with nuclei is obtained by studying the magnetic-field dependence of the resident-carrier spin polarization. We find, in good agreement with recent theoretical studies, that the hole hyperfine coupling is ten times smaller than the electron one.

Spatial patterns of dissipative polariton solitons in semiconductor microcavities

We report propagating bound microcavity polariton soliton arrays consisting of multipeak structures either along (x) or perpendicular (y) to the direction of propagation. Soliton arrays of up to five solitons are observed, with the number of solitons controlled by the size and power of the triggering laser pulse. The breakup along the x direction occurs when the effective area of the trigger pulse exceeds the characteristic soliton size determined by polariton-polariton interactions. Narrowing of soliton emission in energy-momentum space indicates phase locking between adjacent solitons, consistent with numerical modeling which predicts stable multihump soliton solutions. In the y direction, the breakup originates from inhomogeneity across the wave front in the transverse direction which develops into a stable array only in the solitonic regime via phase-dependent interactions of propagating fronts.

Optical pumping and reversal of hole spin in InAs/GaAs quantum dots

We have obtained the optical pumping of hole spins, in p-doped InAs/GaAs quantum dots, via the generation of an intermediate trion state by a train of circularly polarized pulses. We show that we can optically control the orientation of the initialized hole spin, independently of the orientation of the intermediate trion state, by choosing the excitation energy of the circularly polarized light. This brings a supplementary degree of freedom for hole-spin manipulations in quantum dots.

Hole and trion spin dynamics in quantum dots under excitation by a train of circularly polarized pulses

We have performed pump-probe experiments in p -doped InAs/GaAs quantum dots leading to the all-optical initialization and readout of hole spins. In order to describe these experiments, we have modelized the interconnected dynamics of the photoelectron spin and the resident hole spin, triggered through the optical excitation by a train of short pulses. A complete description of this spin dynamics is obtained by including the hyperfine coupling as the common decoherence mechanism for the electron and hole spins. Periodic excitation conditions for arbitrary values of the pump power and the external magnetic field are also included in the model. In particular, a good agreement concerning the temporal behavior of the photoinduced circular dichroism is obtained for zero or low magnetic fields. When the applied magnetic field screens the hole-hyperfine interaction, we show that the agreement between the experimental and calculated time-dependent curves requires an additional relaxation mechanism for holes with a characteristic time in the microsecond range.