F. Käppeler

Neutron Capture in Low-Mass Asymptotic Giant Branch Stars: Cross Sections and Abundance Signatures

Recently improved information on the stellar (n, γ) cross sections of neutron magic nuclei at N = 82, and in particular of 142Nd, turn out to represent a sensitive test for models of s-process nucleosynthesis. While these data were found to be incompatible with the classical approach based on an exponential distribution of neutron exposures, they provide significantly better agreement between the solar abundance distribution of s nuclei and the predictions of models for low-mass asymptotic giant branch (AGB) stars. The origin of this phenomenon is identified as lying in the high neutron exposures at low neutron density obtained between thermal pulses when 13C burns radiatively in a narrow layer of a few 10-4 M☉. This effect is studied in some detail, and the influence of the currently available nuclear physics data is discussed with respect to specific further questions. In this context, particular attention is paid to a consistent description of s-process branchings in the region of the rare earth elements. It is shown that, in certain cases, the nuclear data are sufficiently accurate that the resulting abundance uncertainties can be completely attributed to stellar modeling. Thus, the s-process becomes important for testing the role of different stellar masses and metallicities as well as for constraining the assumptions used in describing the low neutron density provided by the 13C source.

Isotopic Compositions of Strontium, Zirconium, Molybdenum, and Barium in Single Presolar SiC Grains and Asymptotic Giant Branch Stars

The strontium, zirconium, molybdenum, and barium isotopic compositions predicted in the mass-losing envelopes of asymptotic giant branch (AGB) stars of solar metallicity and mass 1.5, 3, and 5 M☉ are discussed and compared with recent measurements in single presolar silicon carbide (SiC) grains from the Murchison meteorite. Heavy-element nucleosynthesis via the s-process occurs in the helium intershell, the region between the helium-burning and hydrogen-burning shells, producing heavy elements beyond iron. After a limited number of thermal runaways of the helium shell (thermal pulses), at the quenching of each instability, the convective envelope penetrates into the top layers of the helium intershell (third dredge-up), mixing newly synthesized 12C and s-process material to the stellar surface. Eventually, the envelope becomes carbon-rich (C ≥ O), a necessary condition for SiC grains to condense. In the helium intershell, neutrons are released by (α, n) reactions on 13C and 22Ne during interpulse phases and the thermal pulses, respectively. A 13C pocket is assumed to form in a tiny region in the top layers of the helium intershell by injection of a small amount of protons from the envelope during each third dredge-up episode. This 13C then burns radiately during the interpulse phase. The average neutron density produced is low, but of long duration, so the total neutron exposure is high. We have explored a large range of possible 13C abundances in the pocket. In low-mass AGB stars (1.5 M☉ ≤ M ≤ 4 M☉), a second small burst of neutrons is released by marginal 22Ne burning in the thermal pulse. The neutron density reaches quite a high peak value but is of short duration, so the neutron exposure is low. In intermediate-mass AGB stars (4 M☉ < M ≤ 8 M☉), the 22Ne neutron source is more efficiently activated. The neutron capture process has been followed with a postprocessing code that considers all relevant nuclei from 4He to 210Po. The predicted isotopic compositions of strontium, zirconium, molybdenum, and barium in the envelopes of low-mass AGB stars of solar metallicity are in agreement with the isotopic ratios measured in individual presolar SiC grains, whereas predictions for intermediate-mass stars exclude them as the sources of these grains. A multiplicity of low-mass AGB stars with metallicity around solar, having different masses and experiencing different neutron exposures, are required to account for the measured spread in heavy-element isotopic compositions among single presolar SiC grains. The range of neutron exposures corresponds, on average, to a lower mean neutron exposure than that required to reproduce the s-process main component in the solar system.

THE WEAK s-PROCESS IN MASSIVE STARS AND ITS DEPENDENCE ON THE NEUTRON CAPTURE CROSS SECTIONS

The slow neutron capture process in massive stars (weak s process) produces most of the s-process isotopes between iron and strontium. Neutrons are provided by the 22Ne(?,n)25Mg reaction, which is activated at the end of the convective He-burning core and in the subsequent convective C-burning shell. The s-process-rich material in the supernova ejecta carries the signature of these two phases. In the past years, new measurements of neutron capture cross sections of isotopes beyond iron significantly changed the predicted weak s-process distribution. The reason is that the variation of the Maxwellian-averaged cross sections (MACS) is propagated to heavier isotopes along the s path. In the light of these results, we present updated nucleosynthesis calculations for a 25 M ? star of Population I (solar metallicity) in convective He-burning core and convective C-burning shell conditions. In comparison with previous simulations based on the Bao et?al. compilation, the new measurement of neutron capture cross sections leads to an increase of s-process yields from nickel up to selenium. The variation of the cross section of one isotope along the s-process path is propagated to heavier isotopes, where the propagation efficiency is higher for low cross sections. New 74Ge, 75As, and 78Se MACS result in a higher production of germanium, arsenic, and selenium, thereby reducing the s-process yields of heavier elements by propagation. Results are reported for the He core and for the C shell. In shell C-burning, the s-process nucleosynthesis is more uncertain than in the He core, due to higher MACS uncertainties at higher temperatures. We also analyze the impact of using the new lower solar abundances for CNO isotopes on the s-process predictions, where CNO is the source of 22Ne, and we show that beyond Zn this is affecting the s-process yields more than nuclear or stellar model uncertainties considered in this paper. In particular, using the new updated initial composition, we obtain a high s-process production (overproduction higher than 16O, ~100) for Cu, Ga, Ge, and As. Using the older abundances by Anders & Grevesse, also Se, Br, Kr, and Rb are efficiently produced. Our results have important implications in explaining the origin of copper in the solar abundance distribution, pointing to a prevailing contribution from the weak s-process in agreement with spectroscopic observations and Galactic chemical evolution calculations. Because of the improvement due to the new MACS for nickel and copper isotopes, the nucleosynthesis of copper is less affected by nuclear uncertainties compared to heavier s-process elements. An experimental determination of the 63Ni MACS is required for a further improvement of the abundance prediction of copper. The available spectroscopic observations of germanium and gallium in stars are also discussed, where most of the cosmic abundances of these elements derives from the s-process in massive stars.

Pulse shape analysis of liquid scintillators for neutron studies

The acquisition of signals from liquid scintillators with Flash ADC of high sampling rate ð 1G S=sÞ has been investigated. The possibility to record the signal waveform is of great advantage in studies with g’s and neutrons in a high count-rate environment, as it allows to easily identify and separate pile-up events. The shapes of pulses produced by g-rays and neutrons have been studied for two different liquid scintillators, NE213 and C6D6: A 1-parameter fitting procedure is proposed, which allows to extract information on the particle type and energy. The performance of this method in terms of energy resolution and n=g discrimination is analyzed, together with the capability to identify and resolve pile-up events. r 2002 Elsevier Science B.V. All rights reserved.

The s‐process in low‐metallicity stars – II. Interpretation of high‐resolution spectroscopic observations with asymptotic giant branch models

High-resolution spectroscopic observations of a hundred metal-poor Carbon and s-rich stars (CEMP-s) collected from the literature are compared with the theoretical nucleosynthesis models of asymptotic giant branch (AGB) presented in Paper I (M = 1.3, 1.4, 1.5, 2 Msun, -3.6 < [Fe/H] < -1.5). The s-process enhancement detected in these objects is associated to binary systems: the more massive companion evolved faster through the thermally pulsing AGB phase (TP-AGB), synthesising in the inner He-intershell the s-elements, which are partly dredged-up to the surface during the third dredge-up (TDU) episode. The secondary observed low mass companion became CEMP-s by mass transfer of C and s-rich material from the primary AGB. We analyse the light elements as C, N, O, Na and Mg, as well as the two s-process indicators, [hs/ls] (where ls = is the the light-s peak at N = 50 and hs = the heavy-s peak at N = 82), and [Pb/hs]. We distinguish between CEMP-s with high s-process enhancement, [hs/Fe] > 1.5 (CEMP-sII), and mild s-process enhanced stars, [hs/Fe] < 1.5 (CEMP-sI). To interpret the observations, .... . Detailed analyses for individual stars will be provided in Paper III.

s-Process in Low Metallicity Stars. I. Theoretical Predictions

A large sample of carbon enhanced metal-poor stars enriched in s-process elements (CEMP-s) have been observed in the Galactic halo. These stars of low mass (M � 0.9 M� ) are located on the main-sequence or the red giant phase, and do not undergo third dredge-up (TDU) episodes. The s-process enhancement is most plausibly due to accretion in a binary system from a more massive companion when on the asymptotic giant branch (AGB) phase (now a white dwarf). In order to interpret the spectroscopic observations, updated AGB models are needed to follow in detail the sprocess nucleosynthesis. We present nucleosynthesis calculations based on AGB stellar models obtained with FRANEC (Frascati Raphson-Newton Evolutionary Code) for low initial stellar masses and low metallicities. For a given metallicity, a wide spread in the abundances of the s-process elements is obtained by varying the amount of 13 C and its profile in the pocket, where the 13 C(�, n) 16 O reaction is the major neutron source, releasing neutrons in radiative conditions during the interpulse phase. We account also for the second neutron source 22 Ne(�, n) 25 Mg, partially activated during convective thermal pulses. We discuss the surface abundance of elements from carbon to bismuth, for AGB models of initial masses M = 1.3 – 2 M� , low metallicities ([Fe/H] from 1 down to 3.6) and for different 13 C-pockets efficiencies. In particular we analyse the relative behaviour of the three s-process peaks: light-s (ls at magic neutron number N = 50), heavy-s (hs at N = 82) and lead (N = 126). Two s-process indicators, [hs/ls] and [Pb/hs], are needed in order to characterise the s-process distribution. In the online material, we provide a set of data tables with surface predictions. Our final goal is to provide a full set of theoretical models of low mass low metallicity s-process enhanced stars. In a forthcoming paper, we will test our results through a comparison with observations of CEMP-s stars.

GALACTIC CHEMICAL EVOLUTION AND SOLAR s-PROCESS ABUNDANCES: DEPENDENCE ON THE 13C-POCKET STRUCTURE

We study the s-process abundances (A > 90) at the epoch of the solar-system formation. AGB yields are computed with an updated neutron capture network and updated initial solar abundances. We confirm our previous results obtained with a Galactic Chemical Evolution (GCE) model: (i) as suggested by the s-process spread observed in disk stars and in presolar meteoritic SiC grains, a weighted average of s-process strengths is needed to reproduce the solar s-distribution of isotopes with A > 130; (ii) an additional contribution (of about 25%) is required in order to represent the solar s-process abundances of isotopes from A = 90 to 130. Furthermore, we investigate the effect of different internal structures of the 13C-pocket, which may affect the efficiency of the 13C(a, n)16O reaction, the major neutron source of the s-process. First, keeping the same 13C profile adopted so far, we modify by a factor of two the mass involved in the pocket; second, we assume a flat 13C profile in the pocket, and we test again the effects of the variation of the mass of the pocket. We find that GCE s-predictions at the epoch of the solar-system formation marginally depend on the size and shape of the 13C-pocket once a different weighted range of 13C-pocket strengths is assumed. We ascertain that, independently of the internal structure of the 13C-pocket, the missing solar-system s-process contribution in the range from A = 90 to 130 remains essentially the same.

The origin of the heavy elements: The s process

Abstract The heavy elements with Z≥30 are made in about equal quantities by neutron capture reactions during stellar He burning and presumably in supernovae. This contribution deals mainly with the slow neutron capture ( s ) process which is responsible for about one half of the abundances in the mass region between Fe and Bi. The slow time scale implies that the reaction path of this process involves mostly stable isotopes which can be studied in detail in laboratory experiments. Based on these data, the quantitative interpretation of the natural abundances provides an exciting possibility for exploring a variety of problems related to stellar and Galactic evolution. The p process, which provides a very small but significant admixture to many of the s abundances, has recently attracted increasing interest as a possibility for supernova studies.

The s-process in low-metallicity stars – III. Individual analysis of CEMP-s and CEMP-s/r with asymptotic giant branch models

We provide an individual analysis of 94 carbon enhanced metal-poor stars showing an s-process enrichment (CEMP-s) collected from the literature. The s-process enhancement observed in these stars is ascribed to mass transfer by stellar winds in a binary system from a more massive companion evolving faster toward the asymptotic giant branch (AGB) phase. The theoretical AGB nucleosynthesis models have been presented in Paper I. Several CEMP-s stars show an enhancement in both s and r-process elements (CEMP-s/r). In order to explain the peculiar abundances observed in CEMP-s/r stars, we assume that the molecular cloud from which CEMP-s formed was previously enriched in r-elements by Supernovae pollution. A general discussion and the method adopted in order to interpret the observations have been provided in Paper II. We present in this paper a detailed study of spectroscopic observations of individual stars. We consider all elements from carbon to bismuth, with particular attention to the three s-process peaks, ls (Y, Zr), hs (La, Nd, Sm) and Pb, and their ratios [hs/ls] and [Pb/hs]. The presence of an initial r-process contribution may be typically evaluated by the [La/Eu] ratio. We found possible agreements between theoretical predictions and spectroscopic data. In general, the observed [Na/Fe] (and [Mg/Fe]) provide information on the AGB initial mass, while [hs/ls] and [Pb/hs] are mainly indicators of the s-process efficiency. A range of 13C-pocket strengths is required to interpret the observations. However, major discrepancies between models and observations exist. We highlight star by star the agreements and the main problems encountered and, when possible, we suggest potential indications for further studies. These discrepancies provide starting points of debate for unsolved problems ...

Sensitivity of p-process nucleosynthesis to nuclear reaction rates in a 25 M. supernova model

The astrophysical p-process, which is responsible for the origin of the proton-rich stable nuclei heavier than iron, was investigated using a full nuclear reaction network for a Type II supernova explosion when the shock front passes through the O/Ne layer. Calculations were performed with a multilayer model adopting the seed of a preexplosion evolution of a 25 M? star. The reaction flux was calculated to determine the main reaction path and branching points responsible for synthesizing the proton-rich nuclei. In order to investigate the impact of nuclear reaction rates on the predicted p-process abundances, extensive simulations with different sets of collectively and individually modified neutron-, proton-, and ?-capture and photodisintegration rates have been performed. These results are not only relevant to explore the nuclear-physics-related uncertainties in p-process calculations but are also important for identifying the strategy and planning of future experiments.