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Dive into the research topics where Fabian Single is active.

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Featured researches published by Fabian Single.


Chemsuschem | 2018

Identifying the Mechanism of Continued SEI Growth

Fabian Single; Arnulf Latz; Birger Horstmann

Continued growth of the solid-electrolyte interphase (SEI) is the major reason for capacity fade in modern lithium-ion batteries. This growth is made possible by a yet unidentified transport mechanism that limits the passivating ability of the SEI towards electrolyte reduction. We, for the first time, differentiate the proposed mechanisms by analyzing their dependence on the electrode potential. Our calculations are compared to recent experimental capacity-fade data. We show that the potential dependence of SEI growth facilitated by solvent diffusion, electron conduction, or electron tunneling qualitatively disagrees with the experimental observations. Only diffusion of Li interstitials results in a potential dependence matching the experiments. Therefore, we identify the diffusion of neutral radicals, such as Li interstitials, as the cause of long-term SEI growth.


Physical Chemistry Chemical Physics | 2016

Dynamics and morphology of solid electrolyte interphase (SEI)

Fabian Single; Birger Horstmann; Arnulf Latz


Journal of The Electrochemical Society | 2017

Revealing SEI Morphology: In-Depth Analysis of a Modeling Approach

Fabian Single; Birger Horstmann; Arnulf Latz


Archive | 2017

Predicting SEI Morphology from Transport and Reaction Kinetics

Arnulf Latz; Birger Horstmann; Fabian Single


Archive | 2017

Theory-based Investigation of SEI Formation

Fabian Single; Birger Horstmann; Arnulf Latz


231st ECS Meeting (May 28 - June 1, 2017) | 2017

Revealing SEI Morphology: A Novel Modelling Approach

Fabian Single; Birger Horstmann; Arnulf Latz


Archive | 2016

Simulation of SEI Formation: Revealing SEI Morphology

Fabian Single; Tobias Schmitt; Arnulf Latz; Birger Horstmann


Archive | 2016

Modeling Graphite Surfaces: Lithium Plating & Solid Electrolyte Interphase

Birger Horstmann; Fabian Single; Simon Hein; Tobias Schmitt; Arnulf Latz


Archive | 2016

Modeling Solid Electrolyte Interphase Formation and Morphology

Fabian Single; Birger Horstmann; Arnulf Latz; Tobias Schmitt


Archive | 2016

Modelling Solid Electrolyte Interphase growth, a Novel Description of Porous Layer Evolution

Fabian Single; Birger Horstmann; Arnulf Latz

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Arnulf Latz

German Aerospace Center

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Simon Hein

German Aerospace Center

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