Fabian Single
German Aerospace Center
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Publication
Featured researches published by Fabian Single.
Chemsuschem | 2018
Fabian Single; Arnulf Latz; Birger Horstmann
Continued growth of the solid-electrolyte interphase (SEI) is the major reason for capacity fade in modern lithium-ion batteries. This growth is made possible by a yet unidentified transport mechanism that limits the passivating ability of the SEI towards electrolyte reduction. We, for the first time, differentiate the proposed mechanisms by analyzing their dependence on the electrode potential. Our calculations are compared to recent experimental capacity-fade data. We show that the potential dependence of SEI growth facilitated by solvent diffusion, electron conduction, or electron tunneling qualitatively disagrees with the experimental observations. Only diffusion of Li interstitials results in a potential dependence matching the experiments. Therefore, we identify the diffusion of neutral radicals, such as Li interstitials, as the cause of long-term SEI growth.
Physical Chemistry Chemical Physics | 2016
Fabian Single; Birger Horstmann; Arnulf Latz
Journal of The Electrochemical Society | 2017
Fabian Single; Birger Horstmann; Arnulf Latz
Archive | 2017
Arnulf Latz; Birger Horstmann; Fabian Single
Archive | 2017
Fabian Single; Birger Horstmann; Arnulf Latz
231st ECS Meeting (May 28 - June 1, 2017) | 2017
Fabian Single; Birger Horstmann; Arnulf Latz
Archive | 2016
Fabian Single; Tobias Schmitt; Arnulf Latz; Birger Horstmann
Archive | 2016
Birger Horstmann; Fabian Single; Simon Hein; Tobias Schmitt; Arnulf Latz
Archive | 2016
Fabian Single; Birger Horstmann; Arnulf Latz; Tobias Schmitt
Archive | 2016
Fabian Single; Birger Horstmann; Arnulf Latz