G. Callsen

Structural and optical investigation of non-polar (1-100) GaN grown by the ammonothermal method

We studied the structural and optical properties of state-of-the-art non-polar bulk GaN grown by the ammonothermal method. The investigated samples have an extremely low dislocation density (DD) of less than 5 × 104u2009cm−2, which results in very narrow high-resolution x-ray rocking curves. The a and c lattice parameters of these stress-free GaN samples were precisely determined by using an x-ray diffraction technique based on the modified Bond method. The obtained values are compared to the lattice parameters of free-standing GaN from different methods and sources. The observed differences are discussed in terms of free-electron concentrations, point defects, and DD. Micro Raman spectroscopy revealed a very narrow phonon linewidth and negligible built-in strain in accordance with the high-resolution x-ray diffraction data. The optical transitions were investigated by cathodoluminescence measurements. The analysis of the experimental data clearly demonstrates the excellent crystalline perfection of ammonothe...

Recombination dynamics in ZnO nanowires: Surfaces states versus mode quality factor

In this work, we investigate the influence of finite size on the recombinations dynamics of ZnO nanowires. We demonstrate that diameter as well as length of nanowires determine the lifetime of the neutral donor bound excitons. Our findings suggest that while the length is mainly responsible for different mode quality factors of the cavity-like nanowires, the diameter determines the influence of surface states as alternative recombinations channels for the optical modes trapped in the nanocavity. In addition, comparing nanowires grown using different catalyst we show that the surfaces states strongly depend on each precursor characteristics.

Spatial mapping of exciton lifetimes in single ZnO nanowires

We investigate the spatial dependence of the exciton lifetimes in single ZnO nanowires. We have found that the free exciton and bound exciton lifetimes exhibit a maximum at the center of nanowires, while they decrease by 30% towards the tips. This dependence is explained by considering the cavity-like properties of the nanowires in combination with the Purcell effect. We show that the lifetime of the bound-excitons scales with the localization energy to the power of 3/2, which validates the model of Rashba and Gurgenishvili at the nanoscale.

Optical absorption edge broadening in thick InGaN layers: Random alloy atomic disorder and growth mode induced fluctuations

To assess the impact of random alloying on the optical properties of the InGaN alloy, high-quality InxGa1−xN (0u2009<u2009xu2009<u20090.18) epilayers grown on c-plane free-standing GaN substrates are characterized both structurally and optically. The thickness (25–100u2009nm) was adjusted to keep these layers pseudomorphically strained over the whole range of explored indium content as checked by x-ray diffraction measurements. The evolution of the low temperature optical absorption (OA) edge linewidth as a function of absorption energy, and hence the indium content, is analyzed in the framework of the random alloy model. The latter shows that the OA edge linewidth should not markedly increase above an indium content of 4%, varying from 17u2009meV to 30u2009meV for 20% indium. The experimental data initially follow the same trend with, however, a deviation from this model for indium contents exceeding only ∼2%. Complementary room temperature near-field photoluminescence measurements carried out using a scanning near-field optical mi...

Shielding Electrostatic Fields in Polar Semiconductor Nanostructures

Modern opto-electronic devices are based on semiconductor heterostructures employing the process of electron-hole pair annihilation. In particular polar materials enable a variety of classic and even quantum light sources, whose on-going optimisation endeavours challenge generations of researchers. However, the key challenge - the inherent electric crystal polarisation of such materials - remains unsolved and deteriorates the electron-hole pair annihilation rate. Here, our approach introduces a sequence of reverse interfaces to compensate these polarisation effects, while the polar, natural crystal growth direction is maintained provoking a boost in device performance. Former research approaches like growth on less-polar crystal planes or even the stabilization of unnatural phases never reached industrial maturity. In contrast, our solution allows the adaptation of all established industrial processes, while the polarisation becomes adjustable; even across zero. Hence, our approach marks the onset of an entire class of ultra-fast and efficient devices based on any polar material.

A quantum optical study of thresholdless lasing features in high-β nitride nanobeam cavities

Exploring the limits of spontaneous emission coupling is not only one of the central goals in the development of nanolasers, it is also highly relevant regarding future large-scale photonic integration requiring energy-efficient coherent light sources with a small footprint. These studies are accompanied by a vivid debate on how to prove and interpret lasing in the high-

Excited states of neutral donor bound excitons in GaN

beta

Optical absorption and oxygen passivation of surface states in III-nitride photonic devices

regime. We investigate close-to-ideal spontaneous emission coupling in GaN nanobeam lasers grown on silicon. Due to their high optical quality, such nanobeam cavities allow for efficient funneling of spontaneous emission from the quantum well gain material into the laser mode. By performing a comprehensive optical and quantum-optical characterization, supported by microscopic modeling of the nanolasers, we identify high-

Bound excitons in ZnO: Structural defect complexes versus shallow impurity centers

beta

Optical signatures of nitrogen acceptors in ZnO

lasing at room temperature and show a lasing transition in the absence of a threshold nonlinearity at 156 K. This peculiar characteristic is explained in terms of a temperature and excitation power dependent interplay between 0D and 2D gain contributions.Exploring the limits of spontaneous emission coupling is not only one of the central goals in the development of nanolasers, it is also highly relevant regarding future large-scale photonic integration requiring energy-efficient coherent light sources with a small footprint. Recent studies in this field have triggeredxa0a vivid debate on how to prove and interpret lasing in the high-β regime. We investigate close-to-ideal spontaneous emission coupling in GaN nanobeam lasers grown on silicon. Such nanobeam cavities allow for efficient funneling of spontaneous emission from the quantum well gain material into the laser mode. By performing a comprehensive optical and quantum-optical characterization, supported by microscopic modeling of the nanolasers, we identify high-β lasing at room temperature and show a lasing transition in the absence of a threshold nonlinearity at 156u2009K. This peculiar characteristic is explained in terms of a temperature and excitation power-dependent interplay between zero-dimensional and two-dimensional gain contributions.Here the authors present temperature dependent studies of GaN nanobeam lasers grown on a silicon substrate and demonstrate high-βlasing at room temperature. Comprehensive optical and quantum-optical characterization, complemented by microscopic modeling, of the nanolasers allow identification of lasing behavior.