G. Günter

Observing the Dynamics of Dipole-Mediated Energy Transport by Interaction-Enhanced Imaging

Imaging Excitations Complex processes such as chemical reactions and photosynthesis involve the transport of energy. The mechanisms of how the energy migrates, the influence of the surrounding environment, or the extent to which quantum mechanics affects the process remain unclear. Günter et al. (p. 954, published online 7 November; see the Perspective by Donley) found that a cloud of cold atoms suitably prepared and decorated with “impurity” Rydberg atoms could be used to image the transport of excitations between excited Rydberg atoms directly. This ability to tune the influence of the background environment may help in the study of the coherent transport of energy in complex many-body systems. An imaging technique based on a cloud of cold atoms provides a model system to study the coherent transport of energy. [Also see Perspective by Donley] Electronically highly excited (Rydberg) atoms experience quantum state–changing interactions similar to Förster processes found in complex molecules, offering a model system to study the nature of dipole-mediated energy transport under the influence of a controlled environment. We demonstrate a nondestructive imaging method to monitor the migration of electronic excitations with high time and spatial resolution, using electromagnetically induced transparency on a background gas acting as an amplifier. The continuous spatial projection of the electronic quantum state under observation determines the many-body dynamics of the energy transport.

Coherent population trapping with controlled interparticle interactions

Coherent population trapping (CPT) and the related phenomenon of Electromagnetically Induced Transparency (EIT) are paradigms for quantuminterference effects and have been studied intensely over the last decade [1]. Only recently, EIT involving Rydberg states has attracted much interest, with regard to nonlinear optics [2] as well as in the context of quantum information processing [3]. Whereas CPT and EIT are generally described within a singleatom framework, the situation becomes more involved when interparticle interactions have to be considered. To address the effect of interactions, we investigate CPT in a strongly interacting ultracold Rydberg gas [4]. In our experiment we tune the interaction strength by choosing different Rydberg states and control interactions effects by varying the ground state atom density. Even in the blockade regime we observe a resonance with sub-natural linewidth at the single-particle resonance frequency despite the strong van der Waals interactions among Rydberg atoms. Due to the correlations among the atoms the experimental observations cannot be explained within a meanfield model. A theoretical model that includes interparticle correlations is presented and nicely reproduces the observed features.

Full counting statistics of laser excited Rydberg aggregates in a one-dimensional geometry

We experimentally study the full counting statistics of few-body Rydberg aggregates excited from a quasi-one-dimensional atomic gas. We measure asymmetric excitation spectra and increased second and third order statistical moments of the Rydberg number distribution, from which we determine the average aggregate size. Estimating rates for different excitation processes we conclude that the aggregates grow sequentially around an initial grain. Direct comparison with numerical simulations confirms this conclusion and reveals the presence of liquidlike spatial correlations. Our findings demonstrate the importance of dephasing in strongly correlated Rydberg gases and introduce a way to study spatial correlations in interacting many-body quantum systems without imaging.

Interaction enhanced imaging of individual Rydberg atoms in dense gases.

We propose a new all-optical method to image individual Rydberg atoms embedded within dense gases of ground state atoms. The scheme exploits interaction-induced shifts on highly polarizable excited states of probe atoms, which can be spatially resolved via an electromagnetically induced transparency resonance. Using a realistic model, we show that it is possible to image individual Rydberg atoms with enhanced sensitivity and high resolution despite photon-shot noise and atomic density fluctuations. This new imaging scheme could be extended to other impurities such as ions, and is ideally suited to equilibrium and dynamical studies of complex many-body phenomena involving strongly interacting particles. As an example we study blockade effects and correlations in the distribution of Rydberg atoms optically excited from a dense gas.

Spontaneous Avalanche Ionization of a Strongly Blockaded Rydberg Gas

We report the sudden and spontaneous evolution of an initially correlated gas of repulsively interacting Rydberg atoms to an ultracold plasma. Under continuous laser coupling we create a Rydberg ensemble in the strong blockade regime, which at longer times undergoes an ionization avalanche. By combining optical imaging and ion detection, we access the full information on the dynamical evolution of the system, including the rapid increase in the number of ions and a sudden depletion of the Rydberg and ground state densities. Rydberg-Rydberg interactions are observed to strongly affect the dynamics of plasma formation. Using a coupled rate-equation model to describe our data, we extract the average energy of electrons trapped in the plasma, and an effective cross section for ionizing collisions between Rydberg atoms and atoms in low-lying states. Our results suggest that the initial correlations of the Rydberg ensemble should persist through the avalanche. This would provide the means to overcome disorder-induced heating, and offer a route to enter new strongly coupled regimes.

Correlated Exciton Transport in Rydberg-Dressed-Atom Spin Chains

We investigate the transport of excitations through a chain of atoms with nonlocal dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping, and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and entanglement. These results highlight the importance of nontrivial dissipation, correlations, and many-body effects in recent experiments on the dipole-mediated transport of Rydberg excitations.

Quantum interference in interacting three-level Rydberg gases : coherent population trapping and electromagnetically induced transparency

In this paper, we consider the effects of strong dipole-dipole interactions on three-level interference phenomena such as coherent population trapping and electromagnetically induced transparency. Experiments are performed on laser cooled rubidium atoms and the results compared to a many-body theory based on either a reduced many-body density matrix expansion or Monte Carlo simulations of many-body rate equations. We show that these approaches permit quantitative predictions of the experimentally observed excitation and transmission spectra. Based on the calculations, we moreover predict a universal scaling of the nonlinear response of cold Rydberg gases.

Sub-Poissonian statistics of Rydberg-interacting dark-state polaritons

We observe individual dark-state polaritons as they propagate through an ultracold atomic gas involving Rydberg states coupled via an electromagnetically induced transparency resonance. Strong long-range interactions between Rydberg excitations give rise to a blockade between polaritons, resulting in large optical nonlinearities and modified polariton number statistics. By combining optical imaging and high-fidelity detection of the Rydberg polaritons we investigate both aspects of this coupled atom-light system. We map out the full nonlinear optical response as a function of atomic density and follow the temporal evolution of polaritons through the atomic cloud. In the blockade regime, the statistical fluctuations of the polariton number drop well below the quantum noise limit. The low level of fluctuations indicates that photon correlations modified by the strong interactions have a significant backaction on the Rydberg atom statistics.

Density matrix reconstruction of three-level atoms via Rydberg electromagnetically induced transparency

We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg states. The observed optical transmission of a weak probe laser at the center of the coupling region exhibits a double peaked spectrum as a function of detuning, whilst the Rydberg atom number shows a comparatively narrow single resonance. By imaging the transmitted light onto a charge-coupled-device camera, we record hundreds of spectra in parallel, which are used to map out the spatial profile of Rabi frequencies of the coupling laser. Using all the information available we can reconstruct the full one-body density matrix of the three-level system, which provides the optical susceptibility and the Rydberg density as a function of spatial position. These results help elucidate the connection between three-level interference phenomena, including the interplay of matter and light degrees of freedom and will facilitate new studies of many-body effects in optically driven Rydberg gases.