G.S. Sahoo

Effects of neutron irradiation on optical and chemical properties of CR-39: Potential application in neutron dosimetry.

Effects of high-dose neutron irradiation on chemical and optical properties of CR-39 were studied using FTIR (Fourier Transform Infrared) and UV-vis (Ultraviolet-Visible) spectroscopy. The primary goal was to find a correlation between the neutron dose and the corresponding changes in the optical and chemical properties of CR-39 resulted from the neutron irradiation. The neutrons were produced by bombarding a thick Be target with 22-MeV protons. In the FTIR spectra, prominent absorbance peaks were observed at 1735cm(-1) (C=O stretching), 1230cm(-1)(C-O-C stretching), and 783cm(-1)(=C-H bending), the intensities of which decreased with increasing neutron dose. The optical absorbance in the visible range increased linearly with the neutron dose. Empirical relations were established to estimate neutron doses from these optical properties. This technique is particularly useful in measuring high doses, where track analysis with an optical microscope is difficult because of track overlapping.

Measurement of neutron spectra generated from bombardment of 4 to 24 MeV protons on a thick 9Be target and estimation of neutron yields

A systematic study on the measurement of neutron spectra emitted from the interaction of protons of various energies with a thick beryllium target has been carried out. The measurements were carried out in the forward direction (at 0° with respect to the direction of protons) using CR-39 detectors. The doses were estimated using the in-house image analyzing program autoTRAK_n, which works on the principle of luminosity variation in and around the track boundaries. A total of six different proton energies starting from 4 MeV to 24 MeV with an energy gap of 4 MeV were chosen for the study of the neutron yields and the estimation of doses. Nearly, 92% of the recoil tracks developed after chemical etching were circular in nature, but the size distributions of the recoil tracks were not found to be linearly dependent on the projectile energy. The neutron yield and dose values were found to be increasing linearly with increasing projectile energies. The response of CR-39 detector was also investigated at different beam currents at two different proton energies. A linear increase of neutron yield with beam current was observed.

Effects of high neutron doses and duration of the chemical etching on the optical properties of CR-39.

Effects of the duration of chemical etching on the transmittance, absorbance and optical band gap width of the CR-39 (Polyallyl diglycol carbonate) detectors irradiated to high neutron doses (12.7, 22.1, 36.0 and 43.5 Sv) were studied. The neutrons were produced by bombardment of a thick Be target with 12 MeV protons of different fluences. The unirradiated and neutron-irradiated CR-39 detectors were subjected to a stepwise chemical etching at 1h intervals. After each step, the transmission spectra of the detectors were recorded in the range from 200 to 900 nm, and the absorbances and optical band gap widths were determined. The effect of the etching on the light transmittance of unirradiated detectors was insignificant, whereas it was very significant in the case of the irradiated detectors. The dependence of the optical absorbance on the neutron dose is linear at short etching periods, but exponential at longer ones. The optical band gap narrows with increasing etching time. It is more significant for the irradiated dosimeters than for the unirradiated ones. The rate of the narrowing of the optical band gap with increasing neutron dose increases with increasing duration of the etching.

Measurement of Neutron Energy Distributions From p+Be Reaction at 20 MeV Using Threshold Activation Foils

Energy distributions of neutrons emitted from the interaction of 20 MeV protons incident on a thick Be target were estimated at two angles (0° and 90°) with respect to the incident beam using activation foils as threshold detectors. A recently developed unfolding code GAMCD based on Genetic Algorithm and Monte Carlo methods was used to estimate the neutron spectra by unfolding the counts obtained from the activation foils. These results were compared with the unfolding codes, MAXED and GRAVEL. In the GAMCD code, a guess spectrum as a-priori information need not be provided as input unlike in MAXED and GRAVEL. Results obtained from all these codes matched each other reasonably well. Out of 30 reactions studied experimentally only the selected 15 were found sufficient to generate acceptable spectra in the case of neutrons emitted from the p+Be reaction at 20 MeV. A peak in the energy distributions around 3 MeV at both the measured angles is contributed by the three body breakup process while a broad hump between 6 MeV and 10 MeV only in the forward direction suggests contribution from the pre-equilibrium emissions from the 9Be(p, n)9B channel, which also contributes to the small peak observed around 15 MeV. The code GAMCD was found to perform satisfactorily for the present data set.

Neutron dose estimation via LET spectrometry using CR-39 detector for the reaction 9 Be (p, n)

CR-39 detectors, widely used for neutron dosimetry in accelerator radiation environment, have also been applied in tissue microdosimetry by generating the linear energy transfer (LET) spectrum. In this work, the neutron dose has been estimated via LET spectrometry for 9Be (p, n) reaction which is useful for personnel monitoring around particle accelerators and accelerator based therapy facilities. Neutrons were generated by the interaction of protons of 6 different energies from 4–24 MeV with a thick Be target. The LET spectra were obtained from the major and minor radii of each track and the thickness of removed surface. From the LET spectra, the absorbed dose (DLET) and the dose equivalent (HLET) were estimated using Q-L relationship as given by International Commission on Radiological Protection (ICRP) 60. The track density in CR-39 detector and hence the neutron yield was found to be increasing with the increase in projectile (proton) energy. Similar observations were also obtained for absorbed dose (DLET) and dose equivalents (HLET).

Measurement of neutron energy spectrum from 241 Am-B source using CR-39 detectors and an in-house image analysis program (autoTRAK_n)

An attempt has been made in the present work to estimate the neutron spectrum of a standard 241 Am-B source using CR-39 solid polymeric track detector and an in-house image analysis program autoTRAK_n. The program works on the principle of greyscale variations in and around the recoil tracks and calculates the track parameters such as diameter, major, minor axes and estimates three dimensional parameters like recoil track depth and angular incidence. It is also capable of counting overlapping tracks without any segregation procedure. In the present study, the standard 241 Am-B neutron spectrum generated from the recoil track parameters with the autoTRAK_n program is compared with the reported values measured using the time of flight method and found to be matching well, mainly at the characteristic peak. The total neutron fluence and dose equivalents are also determined with the program and are compared with the standard source measurements. The results obtained from autoTRAK_n are found to be in close agreement with the standard measurements with less than 5% error for both the parameters. Hence, this methodology can be used as a backup technique for neutron spectrum measurements along with other techniques considering its low cost, small size, easy irradiation, and processing.