G. Tungate

Optical model analyses of 6,7Li + 208Pb elastic scattering near the Coulomb barrier

The elastic scattering of 6Li and 7Li by 208Pb has been measured at several energies near the Coulomb barrier and analysed in terms of the optical model. Previous reports have suggested that the normalization factor, NR, for the double-folded real potential is approximately 0.6 for both isotopes at bombarding energies well above the Coulomb barrier. In this paper we show that, whereas this low value for NR persists for 6Li at energies close to the barrier, for 7Li it is somewhat greater than unity, and indicates the existence of a threshold anomaly for this projectile.

Cooling and bunching of ion beams for collinear laser spectroscopy

A greatly increased sensitivity in collinear laser spectroscopy experiments has been achieved by the application of new on-line ion cooling and bunching techniques. Cooling of a low-energy ion beam to low emittance and low velocity spread is shown to increase the peak efficiency while bunching the beam results in highly efficient background suppression.

Nuclear charge radii of neutron deficient titanium isotopes 44Ti and 45Ti

Optical isotope shifts of the unstable 44,45Ti isotopes, as well as those of stable 46−50Ti, have been investigated by collinear laser spectroscopy on fast ion beams using an ion guide isotope separator with a cooler-buncher. Changes in mean square charge radii across the neutron 1f7/2 shell are deduced. The evolution of the even-N Ti nuclear radii shows a generally increasing tendency with decreasing neutron number. This behaviour is significantly different to that of the neighbouring Ca isotopes which exhibit a symmetric parabolic behaviour across the shell. The trend of the Ti nuclear radii is consistent with the predictions of the relativistic mean-field theory. The charge radius of 44Ti is also compared to predictions of a 40Ca + α cluster model.

Collinear laser spectroscopy of radioisotopes of zirconium

Isotope shifts and hyperfine structures have been measured for radioisotopes of ionic zirconium using on-line laser spectroscopy at the IGISOL facility in Jyvaskyla, where the installation of an ion beam cooler/buncher has significantly improved the experimental sensitivity. Measurements have been made on all the neutron-deficient isotopes from 87Zr to 90Zr, including the isomers 87m,89mZr, and the neutron-rich isotopes from 96Zr to 102Zr. The change in mean square charge radii between the isotopes and the nuclear moments of the odd isotopes have been extracted. The data show a sudden increase in the mean square charge radius at mass A = 100, consistent with an onset of nuclear deformation which has been observed in the gamma ray spectroscopy of isotope chains in this region of the nuclear chart.

Nuclear charge radii and electromagnetic moments of radioactive scandium isotopes and isomers

Collinear laser spectroscopy experiments with the Sc+ transition 3d4s 3D2 → 3d4p 3F3 at λ = 363.1 nm were performed on the 42–46Sc isotopic chain using an ion guide isotope separator with a cooler-buncher. Nuclear magnetic dipole and electric quadrupole moments as well as isotope shifts were determined from the hyperfine structure for five ground states and two isomers. Extensive multi-configurational Dirac–Fock calculations were performed in order to evaluate the specific mass-shift, MSMS, and field-shift, F, parameters which allowed evaluation of the charge radii trend of the Sc isotopic sequence. The charge radii obtained show systematics more like the Ti radii, which increase towards the neutron shell closure N = 20, than the symmetric parabolic curve for Ca. The changes in mean-square charge radii of the isomeric states relative to the ground states for 44Sc and 45Sc were also extracted. The charge radii difference between the ground and isomeric states of 45Sc is in agreement with the deformation effect estimated from the B(E2) measurements but is smaller than the deformation extracted from the spectroscopic quadrupole moments.

Nuclear moments and charge radii of the 171Hf ground state and isomer

The magnetic moment, quadrupole moment and mean-square charge radial changes, relative to 172Hf, have been measured for the 171Hf ground state and the ½-[521] isomeric state, using on-line laser spectroscopy. The magnetic moments of the isomer and ground states are found to be + 0.526(16)µn and -0.674(12)µn, respectively. The spectroscopic quadrupole moment of the ground state is found to be +3.463(27) b. No change in mean-square charge radius is observed between the ground state and isomeric state. The observation of an inversion in the odd-even staggering at 171Hf is consistent with the suggested deformation trends.

First collinear laser spectroscopy measurements of radioisotopes from an IGISOL ion source

Abstract The standard Doppler-free technique of collinear laser spectroscopy has been successfully applied to radioisotopes from the ion-guide isotope separator (IGISOL) at the University of Jyvaskyla. The laser resonance fluorescence signals for the 140,142,144 Ba radioisotopes show that the ion beam energy spread is less than 6 eV, allowing the laser technique to have both high resolution and a sensitivity comparable with the best obtained at conventional facilities.

Nuclear spin determination of 100mY by collinear laser spectroscopy of optically pumped ions

The nuclear spin of the τ1/2 = 0.94 s isomer in 100Y has been determined by collinear laser spectroscopy of optically pumped yttrium fission fragments at the IGISOL facility, JYFL. The isotopes 96, 98, 99, 100Y were produced by the proton-induced fission of natural uranium, and studied on the 4d5s 3D2 (1045 cm−1) → 4d5p 3P1 (32 124 cm−1) transition at 321.67 nm. Enhancement of the population of the metastable 3D2 level was achieved by optically pumping the ground state population via the 5s2 1S0 → 4d5p 1P1 transition at 363.31 nm while the ions were stored in a linear Paul trap. These data, when combined with previous spectroscopic results, give sufficient information for the nuclear spin of 100mY to be determined unambiguously as I = 4. This spin assignment reveals that 100mY has an unexpectedly large dynamic contribution to its quadrupole deformation.

208Pb(7Li,6Li)209Pb reaction at 33 MeV and its effect on elastic scattering

Abstract Angular distributions of the differential cross section and the second-rank tensor analysing power T 20 have been measured for the one-neutron transfer reaction induced by polarized 7 Li ions on 208 Pb at 33 MeV leading to five states in 209 Pb. The experimental data were analysed simultaneously with data for elastic and inelastic scattering of 7 Li by means of CCBA and CRC calculations. A strong effect of the transfer channels on the elastic scattering was found. Coupling to the transfer channels cancelled out the effect of projectile excitation on the elastic-scattering cross section but was unable to account fully for the renormalization factor of the double-folding potential found previously in an optical-model analysis of 7 Li+ 208 Pb elastic scattering. The second-rank tensor analysing power for the elastic scattering was strongly affected by the transfer channels.

Collinear laser spectroscopy of neutron-rich cerium isotopes near the N = 88 shape transition.

Laser spectroscopy has been used to measure the isotope shifts of 146Ce and 148Ce relative to 144Ce, Z = 58. The new data, in combination with existing optical data on the stable isotopes and radioactive 144Ce isotope, permits a study of charge radii variations for the even-N Ce nuclei from N = 78 to N = 90. This range covers both the N = 82 shell closure and the N = 88 shape transition region. A marked increase in deformation occurs at N = 88 for elements with Z ≥ 60 but not for those with Z ≤ 56. The new data for Ce (Z = 58) show an intermediate behaviour, resulting in a smooth increase in deformation with Z in the N = 88, 90 region.