G. Valiulis

Spontaneously Generated X-Shaped Light Bullets

We observe the formation of an intense optical wave packet fully localized in all dimensions, i.e., both longitudinally (in time) and in the transverse plane, with an extension of a few tens of fsec and microns, respectively. Our measurements show that the self-trapped wave is an X-shaped light bullet spontaneously generated from a standard laser wave packet via the nonlinear material response (i.e., second-harmonic generation), which extend the soliton concept to a new realm, where the main hump coexists with conical tails which reflect the symmetry of linear dispersion relationship.

Highly efficient parametric conversion of femtosecond Ti:sapphire laser pulses at 1 kHz

Pulses with energies as high as 150 microJ and durations as low as 60 f(s) were generated from 1.1 to 2.6 microm by a traveling-wave parametric converter pumped by femtosecond pulses of a Ti:sapphire laser with chirped-pulse amplification.

Parametric generation of high-energy 14.5-fs light pulses at 1.5??µm

High-energy light pulses that are tunable from 1.1 to 2.6 mum, with a duration as short as 14.5 fs were generated in a type II phase-matching beta-BaB(2)O(4) traveling-wave parametric converter pumped by 18-fs pulses obtained from a Ti:sapphire laser with chirped-pulse amplification, followed by a hollow-fiber compressor.

Ultrabroadband supercontinuum and third-harmonic generation in bulk solids with two optical-cycle carrier-envelope phase-stable pulses at 2 μm

We report on the generation of ultrabroadband supercontinuum (SC) by filamentation of two optical-cycle, carrier-envelope phase-stable pulses at 2 μm in fused silica, sapphire, CaF₂ and YAG. The SC spectra extend from 450 nm to more than 2500 nm, and their particular shapes depend on dispersive properties of the materials. Prior to spectral super-broadening, we observe third-harmonic generation, which occurs in the condition of large phase and group velocity mismatch and consists of free and driven components. A double-peaked third-harmonic structure coexists with the SC pulse as demonstrated by the numerical simulations and verified experimentally. The SC pulses have stable carrier envelope phase with short-term rms fluctuations of ∼ 300 mrad, as simultaneously measured in YAG crystal by f-2f and f-3f interferometry, where the latter makes use of intrinsic third-harmonic generation.

Colored conical emission by means of second-harmonic generation.

We predict that the combination of space and time modulational instabilities that occur by means of parametric wave mixing in quadratic media leads to colored conical emission. This phenomenon should be observed under conditions usually employed in second-harmonic experiments.

Highly efficient four-wave parametric amplification in transparent bulk Kerr medium

We report on highly efficient four-wave optical parametric amplification in a water cell pumped by an elliptically shaped, ultrashort pulsed laser beam under non-collinear phase-matching configuration. Energy conversion from pump to parametric waves as high as 25 % is obtained owing to the achievement of 1-dimensional spatial-soliton regime, which guarantees high intensity over a large interaction length and ensures high beam quality.

Effective lensing effects in parametric frequency conversion

We show that, in the high wave-vector-mismatch (cascading) limit, the well-known paraxial description of parametric frequency conversion in quadratic media entails effective lensing effects, which can have a self-focusing or a self-defocusing nature, critically depending on the mismatch sign, the selected wave, and the launching condition (second-harmonic generation or downconversion). Numerical and experimental evidence of this behavior is reported.

Two-photon absorbing properties of ultraviolet phase-matchable crystals at 264 and 211 nm

We investigated the intensity-dependent loss properties of nonlinear crystals by using subpicosecond laser pulses at 264 and 211 nm. Two-photon absorption coefficients for potassium dihydrogen phosphate, beta-barium borate, and lithium triborate crystals were obtained from the intensity-dependent transmission measurements.

Generation of femtosecond pulses through second-harmonic compression of the output of a Nd:YAG laser

We report a greater than 20-fold compression during second-harmonic generation from an active–passive mode-locked Nd:YAG laser controlled by passive negative feedback. A compression ratio of 32 times is achieved in the beam center, resulting in a pulse duration of 360 fs.

Nonlinear second-harmonic pulse compression with tilted pulses

We demonstrate that the group velocities of interacting pulses can be adjusted by pulse tilting to optimize second-harmonic pulse compression for a variety of nonlinear crystals and wavelengths. As an experimental proof we present results of ninefold compression of 1.3-ps Nd:glass laser pulses in beta -barium borate crystal.