Gregory J. Stein

Multi-mJ, kHz, 2.1 μm optical parametric chirped-pulse amplifier and high-flux soft x-ray high-harmonic generation.

We report on a multi-mJ 2.1 μm optical parametric chirped-pulse amplification (OPCPA) system operating at 1 kHz repetition rate, pumped by a picosecond cryogenic Yb:YAG laser, and the demonstration of soft x-ray high-harmonic generation (HHG) with a flux of ∼2×10(8)  photon/s/1% bandwidth at 160 eV in Ar. The 1 kHz cryogenic Yb:YAG pump laser amplifies pulses up to 56 mJ and delivers compressed 42 mJ, 17 ps pulses to the 2.1 μm OPCPA system. In the three-stage OPCPA chain, we have obtained up to 2.6 mJ of output energies at 2.1 μm and pulses compressed to 40 fs with good beam quality. Finally, we show cut-off extension of HHG driven by this 2.1 μm source in Ar and N2 gas cells to 190 eV with high photon flux. Our 3D propagation simulation confirms the generation of soft x-ray attosecond pulses from the experiment with Ar.

High-energy, kHz, picosecond hybrid Yb-doped chirped-pulse amplifier.

We report on a diode-pumped, hybrid Yb-doped chirped-pulse amplification (CPA) laser system with a compact pulse stretcher and compressor, consisting of Yb-doped fiber preamplifiers, a room-temperature Yb:KYW regenerative amplifier (RGA), and cryogenic Yb:YAG multi-pass amplifiers. The RGA provides a relatively broad amplification bandwidth and thereby a long pulse duration to mitigate B-integral in the CPA chain. The ~1030-nm laser pulses are amplified up to 70 mJ at 1-kHz repetition rate, currently limited by available optics apertures, and then compressed to ~6 ps with high efficiency. The near-diffraction-limited beam focusing quality is demonstrated with M(x)(2) = 1.1 and M(y)(2) = 1.2. The shot-to-shot energy fluctuation is as low as ~1% (rms), and the long-term energy drift and beam pointing stability for over 8 hours measurement are ~3.5% and <6 μrad (rms), respectively. To the best of our knowledge, this hybrid laser system produces the most energetic picosecond pulses at kHz repetition rates among rod-type laser amplifiers. With an optically synchronized Ti:sapphire seed laser, it provides a versatile platform optimized for pumping optical parametric chirped-pulse amplification systems as well as driving inverse Compton scattered X-rays.

Multi-mJ, kHz, ps deep-ultraviolet source

We demonstrate a 0.56-GW, 1-kHz, 4.2-ps, 2.74-mJ deep-ultraviolet (DUV) laser at ∼257.7  nm with a beam propagation factor (M2) of ∼2.54 from a frequency-quadrupled cryogenic multi-stage Yb-doped chirped-pulse amplifier. The frequency quadrupling is achieved using LiB3O5 and β-BaB2O4 crystals for near-infrared (NIR)-to-green and green-to-DUV conversion, respectively. An overall NIR-to-DUV efficiency of ∼10% has been achieved, which is currently limited by the thermal-induced phase mismatching and the DUV-induced degradation of transmittance. To the best of our knowledge, this is the highest peak-power picosecond DUV source from a diode-pumped solid-state laser operating at kHz repetition rates.

Water-window soft x-ray high-harmonic generation up to the nitrogen K-edge driven by a kHz, 2.1 mu m OPCPA source

We report the generation of coherent water-window soft x-ray harmonics in a neon-filled semi-infinite gas cell driven by a femtosecond multi-mJ mid-infrared optical parametric chirped-pulse amplification (OPCPA) system at a 1 kHz repetition rate. The cutoff energy was extended to ~450 eV with a 2.1 μm driver wavelength and a photon flux of photons/s/1% bandwidth was obtained at 350 eV. A comparable photon flux of photons/s/1% bandwidth was observed at the nitrogen K-edge of 410 eV. This is the first demonstration of water-window harmonic generation up to the nitrogen K-edge from a kHz OPCPA system. Finally, this system is suitable for time-resolved soft x-ray near-edge absorption spectroscopy. Further scaling of the driving pulses energy and repetition rate is feasible due to the availability of high-power picosecond Yb-doped pump laser technologies, thereby enabling ultrafast, tabletop water-window x-ray imaging.

Kagome-fiber-based pulse compression of mid-infrared picosecond pulses from a Ho:YLF amplifier

Over the last decade, the development of ultrafast laser pulses in the mid-infrared (MIR) region has led to important breakthroughs in attosecond science and strong-field physics. However, as most such broadband MIR laser sources are near-IR pumped, the generation of high-intensity, long-wavelength MIR pulses is still a challenge, especially starting from picosecond pulses. Here we report, both experimentally and numerically, nonlinear pulse compression of sub-millijoule picosecond pulses down to sub-300 fs at 2050 nm wavelength in gas-filled Kagome-type hollow-core photonic crystal fibers for driving MIR optical parametric amplifiers. The pump laser is comprised of a compact fiber laser-seeded 2 μm chirped pulse amplification system based on a Ho:YLF crystal at 1 kHz repetition rate. Spectral broadening is studied for different experimental conditions with variations of gas pressure and incident pulse energies. The spectrally broadened 1.8 ps pulses with a Fourier-limited duration of 250 fs are compressed using an external prism-based compressor down to 285 fs and output energy of 125 μJ.

Multi-mJ mid-infrared kHz OPCPA and Yb-doped pump lasers for tabletop coherent soft x-ray generation

We present our recent progress on the development of a mid-infrared (mid-IR), multi-mJ, kHz optical parametric chirped-pulse amplification (OPCPA) system, pumped by a homebuilt picosecond cryogenic Yb:YAG chirped-pulse amplifier, and its application to soft x-ray high-order harmonic generation. The cryogenic Yb:YAG laser operating at 1 kHz repetition rate delivers 42 mJ, 17 ps, 1.03 μm pulses to pump the OPCPA system. Efficient second and fourth harmonic generations from the Yb:YAG system are demonstrated, which provide the pumping capability for OPCPA at various wavelengths. The mid-IR OPCPA system produces 2.6 mJ, 39 fs, 2.1 μm pulses with good beam quality (M 2 = ~1.5) at 1 kHz repetition rate. The output pulses of the OPCPA are used to generate high-order harmonics in both gas cell and hollow-core fiber targets. A photon flux of ~2 × 108 photon/s/1% bandwidth at 160 eV in Ar is measured while the cutoff is 190 eV. The direct measurements of the photon flux from x-ray photodiodes have confirmed the generation of water-window soft x-ray photons with a flux ~106 photon/s/1% bandwidth at 330 eV in Ne. The demonstrated OPCPA and Yb:YAG pump laser technologies provide an excellent platform of energy and power scalable few-cycle mid-IR sources that are suitable for high-flux tabletop coherent soft x-ray generation.

Kagome-fiber-based pulse compression of mid-infrared picosecond pulses from a Ho:YLF amplifier: publisher’s note

This publisher’s note identifies an error in the published version of Fig. 1 of Optica3, 816 (2016)10.1364/OPTICA.3.000816.

Multi-mJ, kHz picosecond deep UV source based on a frequency-quadrupled cryogenic Yb:YAG laser

We report on the development of a 2.74-mJ, ~4.2 ps, ~258 nm deep-ultraviolet (DUV) source at 1 kHz based on frequency quadrupling of ~32 mJ, 8.4 ps, ~1030 nm near-infrared (NIR) laser pulses with an excellent beam profile, generated from a diode-pumped, ultrafast hybrid Yb-doped chirped-pulse amplification laser system. We have used a two-stage second harmonic generation scheme at LBO (NIR-to-green) and BBO crystals (green-to-DUV), respectively, to achieve the fourth-harmonic generation (FHG). The NIR-to-DUV conversion efficiency of ~10% in the FHG is obtained. The peak power of the produced DUV laser pulses is as high as 0.56 GW. The beam profiles at near-field and far-field are found to be excellent and the M2 value is measured as ~2.6. We also present the systematic parameter study on the optimization of DUV generation. To our best knowledge, this is the most energetic DUV generation from a diodepumped solid-state laser at kHz repetition rates.

Tunable and Near-Fourier-limited Few-Cycle Mid-IR Pulses via an Adiabatically Chirped Difference Frequency Grating

A μJ-level source of few-cycle, mid-IR pulses tunable over 2-4 microns is demonstrated based on adiabatic difference frequency generation. This opens up the possibility for single-cycle mid-IR pulses controllable by a near-IR phase shaper.

Water-Window Soft X-ray High-Harmonic Generation up to the Nitrogen K-edge Driven by a kHz, 2.1 μm OPCPA Source

Water-window soft X-ray harmonics up to ~450 eV are generated, with a kHz, multi-mJ mid-infrared optical parametric chirped-pulse amplifier (OPCPA) in a neon-filled gas cell. The photon flux at the nitrogen K-edge is ~1 × 106 photons/s/1% bandwidth.