Gregory Perret

Utilization of freshly induced high-energy gamma-ray activity as a measure of fission rates in re-irradiated burnt UO 2 fuel

In the frame of the LIFE@PROTEUS program, a measurement technique is being developed to measure fission rates in burnt fuel, following re-irradiation in a zero-power research reactor. In the presented approach, the fission rates are estimated by measuring high energy gamma-rays (above 2000 keV) emitted by short-lived fission products freshly produced in the fuel. Due to their high energies, these gamma-rays can be discriminated against the high intrinsic gamma-ray activity of the burnt fuel, which reaches energies up to ∼2000 keV. To demonstrate the feasibility of this approach, fresh and burnt fuel samples (with burn-ups varying from 36 to 64 MWd/kg) were irradiated in the PROTEUS reactor at the Paul Scherrer Institut, and their emitted gamma-ray spectra were recorded shortly after irradiation. It was possible, for the first time, to detect the short-lived gamma-ray activity in the high-energy region, even in the presence of the intrinsic gamma-ray background of the burnt fuel samples. Using the short-lived gamma-ray lines 142La (2542 keV), 89Rb (2570 keV), 95Y (2632 keV), 138Cs (2640 keV) and 95Y (3576 keV), relative fission rates between different core positions were derived for a fresh sample as well as for a burnt sample with a burn-up of 36 MWd/kg. It was shown that, for both the fresh and burnt fuel samples, the measured fission rate ratios agreed well, i.e. within the statistical uncertainties, with calculation results obtained by Monte Carlo simulations.

Neutron production and thermal moderation at the PSI UCN source

We report on gold foil activation measurements performed along a vertical channel along the tank of the ultracold neutron source at the Paul Scherrer Institute. The activities obtained at various distances from the spallation target are in very good agreement with MCNPX simulations which take into account the detailed description of the source as built.

On the combination of delayed neutron and delayed gamma techniques for fission rate measurement in nuclear fuel

Novel techniques to measure newly induced fissions in spent fuel after re-irradiation at low power have been developed and tested at the Proteus zero-power research reactor. The two techniques are based on the detection of high energy gamma-rays emitted by short-lived fission products and delayed neutrons. The two techniques relate the measured signals to the total fission rate, the isotopic composition of the fuel, and nuclear data. They can be combined to derive better estimates on each of these parameters. This has potential for improvement in many areas. Spent fuel characterisation and safeguard applications can benefit from these techniques for non-destructive assay of plutonium content. Another application of choice is the reduction of uncertainties on nuclear data. As a first application of the combination of the delayed neutron and gamma measurement techniques, this paper shows how to reduce the uncertainties on the relative abundances of the longest delayed neutron group for thermal fissions in 235U, 239Pu and fast fissions in 238U. The proposed experiments are easily achievable in zero-power research reactors using fresh UO2 and MOX fuel and do not require fast extraction systems. The relative uncertainties (1σ) on the relative abundances are expected to be reduced from 13% to 4%, 16% to 5%, and 38% to 12% for 235U, 238U and 239Pu, respectively.

FUTURE EXPERIMENTAL PROGRAMMES IN THE CROCUS REACTOR

CROCUS is a teaching and research zero-power reactor operated by the Laboratory for Reactor Physics and Systems Behaviour (LRS) at the Swiss Federal Institute of Technology (EPFL). Three new experimental programmes are scheduled for the forthcoming years. The first programme consists in an experimental investigation of mechanical noise induced by fuel rods vibrations. An in-core device has been designed for allowing the displacement of up to 18 uranium metal fuel rods in the core periphery. The vibration amplitude will be 6 mm in the radial direction (±3 mm around the central position), while the frequency can be tuned between 0.1 and 5 Hz. The experiments will be used to validate computational dynamic tools currently under development, which are based on DORT-TD and CASMO/S3K code systems. The second programme concerns the measurement of in-core neutron noise for axial void profile reconstruction. Simulations performed at Chalmers University have shown how the void fraction and velocity profiles can be reconstructed from noise measurements. The motivation of these experiments is to develop an experimental setup to validate in-core the method in partnership with Chalmers University. The third experimental programme aims at continuing the validation effort on the nuclear data required in the calculation of GEN-III PWR reactors with heavy steel reflectors. This is a collaboration with CEA Cadarache that extends the results of the PERLE experiments carried out in the EOLE reactor at CEA. Scattering cross sections at around 1 MeV will be studied separately by replacing successively the water reflector by sheets of stainless steel alloy and pure metals – iron, nickel, and chromium. Data will be extracted from the measured flux attenuation using foils in the metal reflector and from the criticality effects of these reflectors. In parallel to the three reactor experiments, we develop in-core detectors and measurement systems. Following the last development of a neutron noise measurement station in pulse mode, a second neutron noise station in current mode is being designed. In current mode the reactor can be used at higher power without dead time effects. It allows faster measurement time or lower results uncertainties. Finally, a joint development of a full new detection system based on chemical vapour deposited (sCVD) diamond has been started with the CIVIDEC instrumentation start-up company. A first prototype has been tested in November 2015 in CROCUS. One of the main purposes is to work on the discrimination of gammas, thermal and fast neutrons for demonstrating the interest of this detector type in a mixed neutron-gamma field.

Analysis of Pin Removal Experiments Conducted in a Supercritical Light Water Reactor-Like Test Lattice

A comprehensive program of integral experiments, largely based on the measurement of reaction rate distributions, was carried out recently in the PROTEUS zero-power research reactor at the Paul Scherrer Institute in Switzerland, employing a fuel lattice resembling that of a supercritical light water reactor. The present paper reports on the analysis of a complementary set of measurements, in which the reactivity effects of removing individual pins from the unperturbed, heterogeneously moderated reference lattice were investigated. It has been found that the detailed Monte Carlo modeling of the whole reactor using MCNPX is able - as in the case of the reaction rate distributions - to reproduce the experimental results for the pin removal worths within the achievable statistical accuracy. A comparison of reduced-geometry calculations between MCNPX and the deterministic light water reactor assembly code CASMO-4E has revealed certain discrepancies. On the basis of a reactivity decomposition analysis of the differences between the codes, it has been suggested that these could be due at least partly to CASMO-4E deficiencies in calculating the effect, upon pin removal, of the extra moderation in the neighboring fuel pins.

On the Combination of Delayed Neutron and Delayed Gamma Measurement Techniques for Nuclear Fuel and Its Application to Nuclear Data Uncertainty Reduction

Novel techniques to measure induced fissions in spent fuel after re-irradiation at low power have been developed and tested at the Proteus zero-power research reactor. The two techniques are based on the detection of high energy gamma-rays emitted by short-lived fission products and delayed neutrons.