Helder Crespo

Simultaneous compression and characterization of ultrashort laser pulses using chirped mirrors and glass wedges

We present a simple and robust technique to retrieve the phase of ultrashort laser pulses, based on a chirped mirror and glass wedges compressor. It uses the compression system itself as a diagnostic tool, thereby making unnecessary the use of complementary diagnostic tools. We used this technique to compress and characterize 7.1 fs laser pulses from an ultrafast laser oscillator.

Cascaded highly nondegenerate four-wave-mixing phenomenon in transparent isotropic condensed media

Broad-bandwidth light pulses with different frequencies, extending from the IR to the UV, are simultaneously generated when two noncollinear, ultrafast laser pulses from a visible dual-frequency laser propagate through bulk isotropic transparent media such as common glass. This phenomenon, which is believed to have been previously unreported, can be explained by a cascade of highly nondegenerate four-wave-mixing processes and corresponds to a coherent scattering effect with geometrically minimized phase mismatch. Frequency-upconverted beams were observed up to the 11th order.

Characterization of broadband few-cycle laser pulses with the d-scan technique

We present an analysis and demonstration of few-cycle ultrashort laser pulse characterization using second-harmonic dispersion scans and numerical phase retrieval algorithms. The sensitivity and robustness of this technique with respect to noise, measurement bandwidth and complexity of the measured pulses is discussed through numerical examples and experimental results. Using this technique, we successfully demonstrate the characterization of few-cycle pulses with complex and structured spectra generated from a broadband ultrafast laser oscillator and a high-energy hollow fiber compressor.

Cascaded nondegenerate four-wave-mixing technique for high-power single-cycle pulse synthesis in the visible and ultraviolet ranges

We present a new technique to synthesize high-power single-cycle pulses in the visible and ultraviolet ranges by coherent superposition of a multiband octave-spanning spectrum obtained by highly-nondegenerate cascaded four-wave mixing of femtosecond pulses in bulk isotropic nonresonant media. The generation of coherent spectra spanning over two octaves in bandwidth is experimentally demonstrated using a thin fused silica slide. Full characterization of the intervening multicolored fields using frequency-resolved optical gating, where multiple cascaded orders have been measured simultaneously for the first time, supports the possibility of direct synthesis of near-single-cycle 2.2 fs visible-UV pulses without recurring to complex amplitude or phase control, which should enable many applications in science and technology.

Sub-two-cycle pulses by soliton self-compression in highly nonlinear photonic crystal fibers

We demonstrate the direct generation of sub-two-cycle pulses by soliton self-compression of femtosecond pulses from a Ti:sapphire laser at 85 MHz using a 4.85-mm-long highly nonlinear photonic crystal fiber. Sub-nanojoule, 41 fs input pulses were compressed down to 4.6 fs without additional phase compensation schemes. To our knowledge, these are the shortest pulses obtained by soliton-effect compression of a laser oscillator. Efficient, near-dispersionless collimation of the fiber output was achieved with a simple lens and an octave-spanning double-chirped mirror pair. The full electric field of the compressed pulses was retrieved with a genetic algorithm applied to spectral and interferometric autocorrelation measurements, and the results are well described by numerical simulations.

Simultaneous compression, characterization and phase stabilization of GW-level 1.4 cycle VIS-NIR femtosecond pulses using a single dispersion-scan setup.

We have temporally characterized, dispersion compensated and carrier-envelope phase stabilized 1.4-cycle pulses (3.2 fs) with 160 µJ of energy at 722 nm using a minimal and convenient dispersion-scan setup. The setup is all inline, does not require interferometric beamsplitting, and uses components available in most laser laboratories. Broadband minimization of third-order dispersion using propagation in water enabled reducing the compressed pulse duration from 3.8 to 3.2 fs with the same set of chirped mirrors. Carrier-envelope phase stabilization of the octave-spanning pulses was also performed by the dispersion-scan setup. This unprecedentedly simple and reliable approach provides reproducible CEP-stabilized pulses in the single-cycle regime for applications such as CEP-sensitive spectroscopy and isolated attosecond pulse generation.

Compression of CEP-stable multi-mJ laser pulses down to 4?fs in long hollow fibers

Carrier envelope phase stable 4 fs near-IR pulses with 3 mJ energy were generated by spectral broadening of circularly polarized 8 mJ pulses in a differentially pumped 2 m long composite stretched exible hollow ber. The pulses were characterized using both second-harmonic generation frequency-resolved optical gating (SHG-FROG) and SHG d-scan methods

Nonintrusive phase stabilization of sub-two-cycle pulses from a prismless octave-spanning Ti:sapphire laser.

Carrier-envelope (CE) phase-stabilized sub-two-cycle pulses are generated from a 500 MHz compact prismless octave-spanning laser without extracavity nonlinear optical processes distorting the laser output. The necessary f and 2f spectral components are generated intracavity and coupled out independently from the main pulse through specially designed cavity mirrors, resulting in a 55 dB CE beat note (100 kHz resolution bandwidth). The in-loop CE phase error (integrated from 2.5 mHz to 10 MHz) is 67 mrad, equivalent to a timing jitter between carrier and envelope of 28 as at 790 nm.

Dynamics of Dispersion Managed Octave-Spanning Titanium:Sapphire Lasers

An extensive one-dimensional laser model based on dispersion managed mode locking is presented that accurately describes the pulse dynamics of octave-spanning titanium:sapphire lasers generating sub-two-cycle pulses. By including detailed characteristics for the intracavity elements (mirrors and output coupler), it is demonstrated that the spectral output and temporal pulse shape of these lasers can be predicted quantitatively in very good agreement with experimental results.

Sub-two-cycle soliton-effect pulse compression at 800 nm in photonic crystal fibers

The possibility of soliton self-compression of ultrashort laser pulses down to the few-cycle regime in photonic crystal fibers is numerically investigated. We show that efficient sub-two-cycle temporal compression of nanojoule-level 800 nm pulses can be achieved by employing short (typically 5 mm long) commercially available photonic crystal fibers and pulse durations of around 100 fs, regardless of initial linear chirp, and without the need of additional dispersion compensation techniques. We envision applications in a new generation of compact and efficient sub-two cycle laser pulse sources.